环江尾砂库溃坝影响区农田土壤和蔬菜中重金属含量测定与健康风险评价
doi: 10.13205/j.hjgc.201510029
HEAVY METAL CONTENTS IN SOIL AND VEGETABLES OF A TAILING SPILL IN HUANJIANG AND HUMAN HEALTH RISKS ASSESSMENT
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摘要: 为了解广西大环江上游尾砂库溃坝对下游农田土壤和蔬菜中重金属含量的影响,本研究采集了104个蔬菜样品,74个蔬菜样品对应的土壤样品和13个背景土壤样品,分析其砷、铅、镉的含量特征,评估通过食用蔬菜途径摄入重金属的人体健康风险。结果表明,被淹土壤中的砷、铅、镉含量均值分别为46.72,442.6,1.760 mg/kg,未淹土壤分别为24.06,56.89,0.490 mg/kg,被淹土壤重金属含量显著高于未淹土壤。现场采集蔬菜与市场采购蔬菜中铅、镉含量差异显著;被淹土壤与未淹土壤种植的蔬菜铅含量差异显著。溃坝影响区居民中成人食用蔬菜而摄入砷、铅和镉的目标危险系数值(THQ)分别为0.029、0.190、0.120,儿童分别为0.044、0.290、0.183,危害系数均低于安全阈值。若考虑到当地生产的大米等其他食品的贡献,通过全膳食途径摄入的铅对溃坝居民存在健康风险。Abstract: In order to investigate the concentration of the heavy metals in farmland soil and vegetables below the Dahuanjiang River affected by upriver tailing dam collapse,As,Pb,Cd in 74 soil samples from gardens and fields used to grow vegetable,13 background soil samples and 104 vegetable samples were collected and analyzed to evaluate the health risks of heavy metals intaking by eating contaminated vegetables in investigated areas. The results showed that the geometric mean concentration of As, Pb,Cd in flooded soil was 46. 72,442. 6,1. 760 mg /kg,respectively. The concentration of As,Pb,Cd in non-flooded soil was 24. 06,56. 89,0. 490 mg /kg,respectively. Contamination of heavy metals in flooded soils was higher than that in the nonflooded. The concentrations of Pb and Cd have significant differences in vegetables collected from farmland and bought from market,but the concentrations of As and Cd have no differences between vegetable from flooded and non-flooded soil. Farmland soils were seriously contaminated by As,Pb and Cd. The target hazard quotients of As,Pb,Cd for adult were 0. 029,0. 190, 0. 120,for the children’s were 0. 044,0. 290,0. 183,respectively,for residents through consuming vegetables. According to the contribution of other local foods,such as rice,it will cause obvious health risk of Pb to the local resident through total diet.
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Key words:
- Dahuanjiang River /
- soil /
- vegetable /
- heavy metal
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