基于蒙特卡罗模拟的沈阳城市表层土壤中多环芳烃的健康风险评价

罗庆; 谷雷严; 单岳; 孙丽娜

doi:10.13205/j.hjgc.202005034

基于蒙特卡罗模拟的沈阳城市表层土壤中多环芳烃的健康风险评价

doi: 10.13205/j.hjgc.202005034

1. 沈阳建筑大学市政与环境工程学院, 沈阳 110168;
2. 沈阳大学环境学院区域污染环境生态修复教育部重点实验室, 沈阳 110044

基金项目:

辽宁省自然科学基金重点项目(20170520384)。

中国博士后科学基金项目(2018M630304)

国家自然科学基金项目(41807384)

详细信息

作者简介:
罗庆(1984-),男,博士,副教授,硕士生导师,主要研究方向为环境分析化学和污染控制化学。luoqingyt@126.com。

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出版历程
- 收稿日期: 2019-04-24

HEALTH RISK ASSESSMENT OF POLYCYCLIC AROMATIC HYDROCARBONS IN URBAN TOP SOIL OF SHENYANG BASED ON MONTE CARLO METHOD

1. School of Municipal and Environmental Engineering, Shenyang Jianzhu University, Shenyang 110168, China;
2. Key Laboratory of Regional Environment and Eco-Remediation of Ministry of Education, College of Environment, Shenyang University, Shenyang 110044, China

摘要

摘要: 为研究沈阳城市表层土壤中多环芳烃(PAHs)污染特征,于2017年9月采集了沈阳城区74个表层土壤样品,检测了土壤中16种优控PAHs的含量,并利用基于蒙特卡罗模拟的概率风险评价模型定量评估了其健康风险。结果表明:沈阳城市表层土壤中PAHs含量为283~21821 μg/kg,平均值为2370 μg/kg;与国内外其他城市土壤污染状况相比,沈阳城市表层土壤中PAHs的污染较为严重。健康风险评价结果表明,沈阳城市表层土壤中PAHs对儿童和成人造成的总致癌和非致癌风险均处于可接受的水平;其中,苯并[a]芘是致癌风险的最主要贡献物质,芘、荧蒽和菲是非致癌风险的最主要贡献物质。
- 多环芳烃 /
- 健康风险评价 /
- 蒙特卡罗模拟 /
- 城市土壤 /
- 沈阳
Abstract: In order to study the pollution characteristics of polycyclic aromatic hydrocarbons (PAHs) in urban top soil of Shenyang, 74 urban top soil samples were collected from the urban area of Shenyang in September 2017, the concentrations of 16 prior PAHs were determined, and the health risks were evaluated by probabilistic risk models based on Monte Carlo simulation. The results showed that, the concentrations of 16 PAHs ranged from 283 to 21821 μg/kg, with an average concentration of 2370 μg/kg. Compared with other researches, the pollution extent of PAHs in urban top soil of Shenyang was serious. The results of health risk assessment showed that, the total carcinogenic and non-carcinogenic risks caused by PAHs for children and adults were presented at an acceptable level. Among them, benzo[a]pyrene was the key contributor for carcinogenic risk, while pyrene, fluoranthene and phenanthrene were the key contributors for non-carcinogenic risk.
- polycyclic aromatic hydrocarbons /
- health risk assessment /
- Monte Carlo simulation /
- urban soils /
- Shenyang

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参考文献(21)

姚宏, 张士超, 刘明丽, 等. 基于城镇化进程表层土壤多环芳烃来源解析与风险评价[J]. 环境科学, 2018, 39(2):889-898.

GAN S, LAU E V, NG H K. Remediation of soils contaminated with polycyclic aromatic hydrocarbons (PAHs) [J]. Journal of Hazardous Materials, 2009, 172(2/3): 532-549.

GAO P, DA SILVA E, HOU L, et al. Human exposure to polycyclic aromatic hydrocarbons: metabolomics perspective [J]. Environment International, 2018, 119: 466-477.

郭凡嫡, 潘俊, 孙丽娜, 等. 辽河干流河岸带土壤中多环芳烃的污染特征与生态风险评价研究[J]. 环境工程, 2018, 36(7): 155-160.

JIANG Y F, YVES U J, SUN H, et al. Distribution, compositional pattern and sources of polycyclic aromatic hydrocarbons in urban soils of an industrial city, Lanzhou, China [J]. Ecotoxicology and Environmental Safety, 2016, 126: 154-162.

刘海珍, 刘道辰, 陈诗越. 东平湖表层沉积物中PAHs来源分析及生态风险评价[J]. 环境工程, 2014, 32(1): 126-129.

PENG C, CHEN W P, LIAO X L, et al. Polycyclic aromatic hydrocarbons in urban soils of Beijing: status, sources, distribution and potential risk [J]. Environmental Pollution, 2011, 159(3): 802-808.

CHEN S C, LIAO C M. Health risk assessment on human exposed to environmental polycyclic aromatic hydrocarbons pollution sources [J]. Science of the Total Environment, 2006, 366(1): 112-123.

佟瑞鹏, 杨校毅. 基于蒙特卡罗模拟的土壤环境健康风险评价:以PAHs为例[J]. 环境科学, 2017, 38(6): 2522-2529.

李嘉康, 宋雪英, 魏建兵, 等. 沈北新区土壤中多环芳烃污染特征及源解析[J]. 环境科学, 2018, 39(1): 379-388.

杨明明, 孙丽娜, 罗庆, 等. 沈阳市铁西区老工业搬迁区土壤多环芳烃的健康风险评价[J]. 生态学杂志, 2013, 32(3): 675-681.

CVETKOVIC J S, MITIC V D, JOVANOVIC-STANKOV V P, et al. Optimization of the QuEChERS extraction procedure for the determination of polycyclic aromatic hydrocarbons in soil by gas chromatography-mass spectrometry [J]. Analytical Methods, 2016, 8(7): 1711-1720.

CHEN J W, WANG S L, HSIEH D P H, et al. Carcinogenic potencies of polycyclic aromatic hydrocarbons for back-door neighbors of restaurants with cooking emissions [J]. Science of the Total Environment, 2012, 417/418: 68-75.

CHEN S C, LIAO C M. Health risk assessment on human exposed to environmental polycyclic aromatic hydrocarbons pollution sources [J]. Science of the Total Environment, 2006, 366(1): 112-123.

ZHANG P, CHEN Y G. Polycyclic aromatic hydrocarbons contamination in surface soil of China: a review [J]. Science of The Total Environment, 2017, 605/606:1011-1020.

MARINHO R A P, SHEPHERD T, NOWELL G, et al. Source and pathway analysis of lead and polycyclic aromatic hydrocarbons in Lisbon urban soils[J]. Science of The Total Environment, 2016, 573:324-336.

BORTEY-SAM N, IKENAKA Y, NAKAYAMA S M M, et al. Occurrence, distribution, sources and toxic potential of polycyclic aromatic hydrocarbons (PAHs) in surface soils from the Kumasi Metropolis, Ghana[J]. Science of The Total Environment, 2014, 496:471-478.

SINGH D P, GADI R, MANDAL T K. Levels, sources, and toxic potential of polycyclic aromatic hydrocarbons in urban soil of delhi, india[J]. Human and Ecological Risk Assessment, 2012, 18(2):393-411.

USEPA (United States Environmental Protection Agency). Exposure Factors Handbook 2011 Edition[EB/OL]. Washington, DC:U.S. Environmental Protection Agency. EPA/600/R-09/052F. http://www.epa.gov/ncea/efh/pdfs/efh-complete.pdf, 2011.

HOU W, ZHANG L, LI Y, et al. Distribution and health risk assessment of polycyclic aromatic hydrocarbons in soil from a typical contaminated urban coking sites in Shenyang city[J]. Bulletin of Environmental Contamination and Toxicology, 2015, 95(6):815-821.

YANG W, LANG Y H, BAI J, et al. Quantitative evaluation of carcinogenic and non-carcinogenic potential for PAHs in coastal wetland soils of China[J]. Ecological Engineering, 2015, 74:117-124.

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