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畜禽养殖污水所含典型抗生素在人工湿地中的去除途径探讨

刘琳 辛宇 姚彤 韦莉莉 刘超翔

刘琳, 辛宇, 姚彤, 韦莉莉, 刘超翔. 畜禽养殖污水所含典型抗生素在人工湿地中的去除途径探讨[J]. 环境工程, 2020, 38(6): 102-107. doi: 10.13205/j.hjgc.202006016
引用本文: 刘琳, 辛宇, 姚彤, 韦莉莉, 刘超翔. 畜禽养殖污水所含典型抗生素在人工湿地中的去除途径探讨[J]. 环境工程, 2020, 38(6): 102-107. doi: 10.13205/j.hjgc.202006016
LIU Lin, XIN Yu, YAO Tong, WEI Li-li, LIU Chao-xiang. REMOVAL PATHWAYS OF TYPICAL ANTIBIOTICS FROM LIVESTOCK WASTEWATER BY CONSTRUCTED WETLAND[J]. ENVIRONMENTAL ENGINEERING , 2020, 38(6): 102-107. doi: 10.13205/j.hjgc.202006016
Citation: LIU Lin, XIN Yu, YAO Tong, WEI Li-li, LIU Chao-xiang. REMOVAL PATHWAYS OF TYPICAL ANTIBIOTICS FROM LIVESTOCK WASTEWATER BY CONSTRUCTED WETLAND[J]. ENVIRONMENTAL ENGINEERING , 2020, 38(6): 102-107. doi: 10.13205/j.hjgc.202006016

畜禽养殖污水所含典型抗生素在人工湿地中的去除途径探讨

doi: 10.13205/j.hjgc.202006016
基金项目: 

中国科学院战略性先导科技专项(XDA23020500)

国家自然科学基金(51678553)。

福建省社会发展引导性项目(2018Y0083)

详细信息
    作者简介:

    刘琳,男,硕士,副研究员,主要研究方向为污水处理与资源化。lliu@iue.ac.cn

    通讯作者:

    刘超翔,男,博士,研究员,主要研究方向为污水生态处理与回用。cxliu@iue.ac.cn

REMOVAL PATHWAYS OF TYPICAL ANTIBIOTICS FROM LIVESTOCK WASTEWATER BY CONSTRUCTED WETLAND

  • 摘要: 人工湿地处理畜禽养殖污水过程中,吸附作用为土霉素、环丙沙星和磺胺二甲基嘧啶在系统内的首要去除途径,其在3种抗生素去除过程中所占相对贡献比例分别为75%、85%和62%。水解作用为土霉素和环丙沙星在湿地中去除的次要途径,其对两者去除的贡献比例分别为21%和19%;磺胺二甲基嘧啶的次要去除途径为微生物降解作用(23%),而水解作用贡献比例仅为13%。通过对比无传统污染物添加组别分析结果,研究发现传统污染物存在不会对抗生素吸附作用产生显著影响,但土霉素和环丙沙星水解去除途径的贡献度会分别降低7%和5%,微生物降解对磺胺二甲基嘧啶的去除作用比例会提升21%。
  • ZHOU L J, YING G G, LIU S, et al. Excretion masses and environmental occurrence of antibiotics in typical swine and dairy cattle farms in China[J]. Science of the Total Environment, 2013, 444(2):183-195.
    傅海霞, 刘怡, 董志英,等.抗生素与重金属复合污染的生态毒理效应研究进展[J]. 环境工程, 2016, 34(4):60-63

    ,104.
    LIU L, LIU Y H, WANG Z, et al. Behavior of tetracycline and sulfamethazine with corresponding resistance genes from swine wastewater in pilot-scale constructed wetlands[J]. Journal of Hazardous Materials, 2014, 278:304-310.
    张鹏飞, 刘晓文, 李杰,等. 养殖废水中抗生素去除处理工艺的研究现状[J]. 净水技术, 2018, 37(4):60-65.
    程宪伟, 梁银秀, 祝惠,等. 人工湿地处理水体中抗生素的研究进展[J]. 湿地科学, 2017, 15(1):128-134.
    ZHANG Q Q, YING G G, PAN C G, et al. Comprehensive evaluation of antibiotics emission and fate in the river basins of China: source analysis, multimedia modeling, and linkage to bacterial resistance[J]. Environmental Science & Technology, 2015, 49(11): 6772-6782.
    LIAO J, LIU C X, LIU L, et al. Influence of hydraulic retention time on behavior of antibiotics and antibiotic resistance genes in aerobic granular reactor treating biogas slurry[J]. Frontiers of Environmental Science & Engineering, 2019, 13(3):59-67.
    LIU L, LI J, FAN H Y, et al. Fate of antibiotics from swine wastewater in constructed wetlands with different flow configurations[J]. International Biodeterioration & Biodegradation, 2019, 140: 119-125.
    HIJOSA-VALSERO M, FINK G, SCHLVSENER M P, et al. Removal of antibiotics from urban wastewater by constructed wetland optimization[J]. Chemosphere, 2011, 83(5): 713-719.
    DAGHRIR R, DROGUI P. Tetracycline antibiotics in the environment: a review[J]. Environmental Chemistry Letters, 2013, 11(3): 209-227.
    LI B, ZHANG T. Biodegradation and adsorption of antibiotics in the activated sludge process[J]. Environmental Science & Technology, 2010, 44(9): 3468-3473.
    SONG X C, LIU D F, ZHANG G W, et al. Adsorption mechanisms and the effect of oxytetracycline on activated sludge[J]. Bioresource Technology, 2014, 151: 428-431.
    WU Q F, LI Z H, HONG H L, et al. Adsorption and intercalation of ciprofloxacin on montmorillonite[J]. Applied Clay Science, 2010, 50(2): 204-211.
    CHENG D M, FENG Y, LIU Y W, et al. Quantitative models for predicting adsorption of oxytetracycline, ciprofloxacin and sulfamerazine to swine manures with contrasting properties[J]. Science of the Total Environment, 2018, 634: 1148-1156.
    LI J, ZHANG H, YUAN G D. Phosphate affects adsorption and desorption of oxytetracycline in the seawater-sediment systems[J]. Environmental Science and Pollution Research, 2018, 25(28): 28160-28168.
    ZHAO Y P, GU X Y, GAO S X, et al. Adsorption of tetracycline (TC) onto montmorillonite: cations and humic acid effects[J]. Geoderma, 2012, 183/184: 12-18.
    WATERMAN K C, ADAMI R C, ALSANTE K M, et al. Hydrolysis in pharmaceutical formulations[J]. Pharmaceutical Development and Technology, 2002, 7(2): 113-146.
    DOI A M, STOSKOPF M K. The kinetics of oxytetracycline degradation in deionized water under varying temperature, pH, light, substrate, and organic matter[J]. Journal of Aquatic Animal Health, 2000, 12(3): 246-253.
    BIAŁK-BIELIŃSKA A, STOLTE S, MATZKE M, et al. Hydrolysis of sulphonamides in aqueous solutions[J]. Journal of Hazardous Materials, 2012, 221/222: 264-274.
    XUAN R C, ARISI L, WANG Q Q, et al. Hydrolysis and photolysis of oxytetracycline in aqueous solution[J]. Journal of Environmental Science and Health Part B, 2009, 45(1): 73-81.
    LIU L, LIU Y H, LIU C X, et al. Potential effect and accumulation of veterinary antibiotics in Phragmites australis under hydroponic conditions[J]. Ecological Engineering, 2013, 53: 138-143.
    DETTENMAIER E M, DOUCETTE W J, BUGBEE B. Chemical hydrophobicity and uptake by plant roots[J]. Environmental Science & Technology, 2008, 43(2): 324-329.
    DALTON H, STIRLING D I. Co-metabolism[J]. Philosophical Transactions of the Royal Society of London. Series B, Biological Sciences, 1982, 297(1088): 481-496.
    TOYAMA T, FURUKAWA T, MAEDA N, et al. Accelerated biodegradation of pyrene and benzo [a] pyrene in the Phragmites australis rhizosphere by bacteria-root exudate interactions[J]. Water Research, 2011, 45(4): 1629-1638.
    OLIVEIRA G H D, SANTOS-NETO A J, ZAIAT M. Evaluation of sulfamethazine sorption and biodegradation by anaerobic granular sludge using batch experiments[J]. Bioprocess and Biosystems Engineering, 2016, 39(1): 115-124.
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