INACTIVATION OF E. COLI IN WATER BY NANOSECOND PULSED HIGH VOLTAGE AIR DISCHARGE
-
摘要: 采用自行研制的喷嘴-板-筒式反应器,研究了大气压纳秒负脉冲空气放电对水中大肠杆菌(Escherichia coli, E.coli)灭菌率的影响因素及规律。实验中空气自放电喷嘴电极进入反应器,气流带动放电生成的活性粒子流到达并作用于水中大肠杆菌。研究结果表明:本实验装置可有效实现对水中大肠杆菌的灭活,灭菌率随着放电电压和脉冲重复频率的增加、放电处理时间的延长而升高;随着鼓气速率的增大先增大后减小;随着喷嘴电极直径的增加先减小后增大。当采用1.30 mm喷嘴电极,在脉冲峰值电压为-32 kV、重复频率80 Hz,鼓气速率为80 mL/min时,连续放电处理12 min,灭菌率达到91%。
-
关键词:
- 喷嘴-板-筒式反应器 /
- 大气压 /
- 纳秒负脉冲 /
- 空气放电 /
- 杀菌
Abstract: In this paper, a nozzle-plate-cylinder reactor was developed and the effect of different factors on inactivation rate of the Escherichia coli(E. coli)in the water with the nanosecond negative pulsed air discharge at atmospheric pressure were investigated. The air flow was injected into the reactor through the discharge nozzle. The active species flow were produced in the discharge process and carried by the air flow to reach the the liquid. The results showed that the inactivation rate increased with the rise of discharge voltage, the pulse repetition rate and the discharge duration time. It increased firstly and then decreased with the air flow rate and decreased with the diameter of the electrode. The inactivation rate reached 91% when a 1.30 mm diameter electrode was adopted under the discharge duration time of 12 min, the disharge peak voltage of -32 kV, repeat frequenty of 80 Hz, and the air flow rate of 80 mL/min. -
RICARD ANDRE. Optical spectroscopy on processing plasmas:cathode magnetron sputtering and flowing post-discharges for elastomer activation and medical sterilization[J]. Thin Solid Films, 2005, 475(1):1-5. ZHANG H, ZHANG Q F, MIAO C G, et al. Degradation of 2, 4-dichlorophenol in aqueous solution by dielectric barrier discharge:effects of plasma-working gases, degradation pathways and toxicity assessment[J]. Chemosphere, 2018, 204:351-358. FATEMEH R, BABAK S, SHARIFIAN M. Atmospheric-pressure DBD plasma-assisted surface modification of polymethyl methacrylate:a study on cell growth/proliferation and antibacterial properties[J]. Estuarine, Coastal and Shelf Science, 2015, 164:471-481. MAY K. Atmospheric plasma discharge sterilization effects on whole cell fatty acid profiles of Escherichia coli and Staphylococcus aureus[J].Journal of Electrostatics, 2010, 68(6):508-512. SHANG K F, WANG X J, LI J, WANG H, et al. Synergetic degradation of Acid Orange 7(AO7) dye by DBD plasma and persulfate[J]. Chemical Engineering Journal, 2017,311:378-384. CHIANG M H, WU J Y, LI Y H, et al. Inactivation of E.coli and B. subtilis by a parallel-plate dielectric barrier discharge jet[J]. Surface and Coatings Technology, 2010, 204(21/22):3729-3737. KANG W S, HONG Y C, HONG Y B, et al. Atmospheric-pressure cold plasma jet for medical applications[J]. Surface and Coatings Technology, 2010, 205(1):S418-S421. NI W Y, JI L F, NIU J H, et al. Plasma inactivation of Escherichia coli cells by atmospheric pressure air brush-shape plasma[J]. Surface and Coatings Technology, 2013, 234:120-125. JAI H C, INHO H, HONG K B, et al. Analysis of sterilization effect by pulsed dielectric barrier discharge[J]. Journal of Electrostatics, 2005, 64(1):17-22. KIM H S, CHO Y I, HWANG I H, et al. Use of plasma gliding arc discharges on the inactivation of E.Coli in water[J]. Separation and Purification Technology, 2013, 120:423-428. OUALID B, ABED Z, ARUTIUN P, et al. Advantages of highly ionized pulse plasma magnetron sputtering (HIPIMS) of silver for improved E.coli inactivation[J]. Thin Solid Films, 2012, 520(9):3567-3573. MIAO H, YUN G. The sterilization of Escherichia coli by dielectric-barrier discharge plasma at atmospheric pressure[J]. Applied Surface Science, 2011, 257(16):7065-7070. 刘红霞,陈杰瑢. 远程氩等离子体表面灭菌研究[J]. 西安交通大学学报, 2010, 44(9):119-114. 邓康,胡小吐. 脉冲电弧液相放电等离子体污水消毒灭菌[J]. 环境工程学报, 2012, 6(10):3635-3638. WANG C H, WU Y, LI G F. Inactivation of E. coli with plasma generated by bipolar pulsed discharge in a three-phase discharge plasma reactor[J]. Journal of Electrostatics, 2007, 66(1):71-78. KOSTOV K G, ROCHA V, KOGA-ITO C Y, et al. Bacterial sterilization by a dielectric barrier discharge (DBD) in air[J]. Surface & Coatings Technology, 2010, 204(18/19):2954-2959. LI J, SHANG K F, WANG T C, et al. Inactivation mechanisms of escherichia coli in drinking water using reactive species generated from a surface discharge[J]. High Voltage Engineering, 2013, 39(9):2119-2124. 马跃,张冠军,石兴民,等. 介质阻挡放电用于细菌灭活的机理研究[J]. 高电压技术,2008, 34(2):363-367 王骁,李中坚,王小平,等. 电场与放电杀菌技术应用于饮用水安全消毒的研究[J]. 环境科学学报, 2013, 33(3):730-735 孙明,杜审言,徐海洋,等. 多相纳秒脉冲放电协同二氧化钛系统对大肠杆菌的灭活[J].高电压技术, 2016, 42(8):2487-2493. SUN M, YANG Y, LU X, et al. Diagnosis of discharge plasma using atmospheric pressure pulsed discharge in air[C]//ICOPS/BEAMS 2014-41st IEEE International Conference on Plasma Science and the 20th International Conference on High-Power Particle Beams. Washington DC, 2014. 董冰岩,聂亚林,宿雅威,等. 双极性高压脉冲介质阻挡放电降解甲醛及臭氧生成质量浓度控制[J]. 高电压技术,2016,42(5):1373-1378.
点击查看大图
计量
- 文章访问数: 90
- HTML全文浏览量: 10
- PDF下载量: 1
- 被引次数: 0