中文核心期刊
CSCD来源期刊(核心库)
中国科技核心期刊
RCCSE中国核心学术期刊
JST China 收录期刊

留言板

尊敬的读者、作者、审稿人, 关于本刊的投稿、审稿、编辑和出版的任何问题, 您可以本页添加留言。我们将尽快给您答复。谢谢您的支持!

姓名
邮箱
手机号码
标题
留言内容
验证码

吸附法去除水中典型药物及个人护理品的研究进展

卜庆伟 张鑫 余刚

卜庆伟, 张鑫, 余刚. 吸附法去除水中典型药物及个人护理品的研究进展[J]. 环境工程, 2021, 39(2): 1-9. doi: 10.13205/j.hjgc.202102001
引用本文: 卜庆伟, 张鑫, 余刚. 吸附法去除水中典型药物及个人护理品的研究进展[J]. 环境工程, 2021, 39(2): 1-9. doi: 10.13205/j.hjgc.202102001
BU Qing-wei, ZHANG Xin, YU Gang. RESEARCH PROGRESS IN REMOVAL OF TYPICAL PHARMACEUTICALS AND PERSONAL CARE PRODUCTS BY ADSORPTION METHOD[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(2): 1-9. doi: 10.13205/j.hjgc.202102001
Citation: BU Qing-wei, ZHANG Xin, YU Gang. RESEARCH PROGRESS IN REMOVAL OF TYPICAL PHARMACEUTICALS AND PERSONAL CARE PRODUCTS BY ADSORPTION METHOD[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(2): 1-9. doi: 10.13205/j.hjgc.202102001

吸附法去除水中典型药物及个人护理品的研究进展

doi: 10.13205/j.hjgc.202102001
基金项目: 

国家自然科学基金(21777188);中国矿业大学(北京)"越崎青年学者"计划(2017QN15)。

详细信息
    作者简介:

    卜庆伟(1983-),男,博士,副教授,主要研究方向为新兴污染物环境行为及控制技术。qingwei.bu@cumtb.edu.cn

    通讯作者:

    卜庆伟(1983-),男,博士,副教授,主要研究方向为新兴污染物环境行为及控制技术。qingwei.bu@cumtb.edu.cn

RESEARCH PROGRESS IN REMOVAL OF TYPICAL PHARMACEUTICALS AND PERSONAL CARE PRODUCTS BY ADSORPTION METHOD

  • 摘要: 吸附法是去除污水中典型药物及个人护理品(PPCPs)的重要手段之一。在梳理各类吸附剂对典型PPCPs去除效果的基础上,结合吸附剂类型和操作条件评述了不同吸附剂对典型PPCPs的去除效率、吸附机理,及影响其吸附效果的因素。总体而言,目前针对吸附法去除典型PPCPs的研究仍存在一些不足,吸附机理研究尚不成熟。关于吸附法去除水中典型PPCPs的研究主要集中在去除效率提升方面,有关典型PPCPs在吸附中的传质过程、发生机理及吸附的控制步骤是未来应该加强的重点研究领域。
  • [1] 赵迎新,王亚舒,季民,等. 吸附法去除水中药品及个人护理品(PPCPs)研究进展[J]. 工业水处理,2017,37(6):1-5.
    [2] 刘晓晖,董文平,乔光明,等. 水环境中药品和个人护理品的迁移转化转化、毒性效应及其风险评估[J]. 科技导报,2015,3(16):56-60.
    [3] 邹艳敏,吴向阳,仰榴青. 水环境中药品和个人护理用品污染现状及研究进展[J]. 环境监测管理与技术,2010,22(6):14-19.
    [4] CARBALLA M, OMIL F, TERNES T, et al. Fate of pharmaceutical and personal care products (PPCPs) during anaerobic digestion of sewage sludge[J]. Water Research,2007,41(10):2139-2150.
    [5] NARUMIYA M, NAKADA N, YAMASHITA N, et al. Phase distribution and removal of pharmaceuticals and personal care products during anaerobic sludge digestion[J]. Journal of Hazardous Materials,2013,260:305-312.
    [6] TERNES T A, STUBER J, HERRMANN N, et al. Ozonation:a tool for removal of pharmaceuticals, contrast media and musk fragrances from wastewater[J]. Water Research,2003,37(8):1976-1982.
    [7] 康杜. 生物膜光反应器去除污水中营养盐和药品及个人护理品的研究[D].武汉:中国地质大学,2018.
    [8] 王建龙. 废水中药品及个人护理用品(PPCPs)的去除技术研究进展[J]. 四川师范大学学报(自然科学版),2020,43(2):143-172.
    [9] YANG Y, OK Y S, KIM K H, et al. Occurrences and removal of pharmaceuticals and personal care products (PPCPs) in drinking water and water/sewage treatment plants:a review[J]. Science of the Total Environment,2017,596/597:303-320.
    [10] KUMAR R, SARMAH A K, PADHYE L P. Fate of pharmaceuticals and personal care products in a wastewater treatment plant with parallel secondary wastewater treatment train[J]. Journal of Environmental Management,2019,233:649-659.
    [11] 乔学兵,由佩骅. 城市污水中药品和个人护理用品(PPCPs)削减技术研究[J]. 能源与环境,2012(2):48-50.
    [12] KATSIGIANNIS A, NOUTSOPOULOS C, MANTZIARAS J, et al. Removal of emerging pollutants through granular activated carbon[J]. Chemical Engineering Journal,2015,280:49-57.
    [13] ANASTOPOULOS I, PASHALIDIS I, ORFANOS A G, et al. Removal of caffeine, nicotine and amoxicillin from (waste) waters by various adsorbents:a review[J]. Journal of Environmental Management,2020,261:110236.
    [14] PRASANNAMEDHA G, KUMAR P S. A review on contamination and removal of sulfamethoxazole from aqueous solution using cleaner techniques:present and future perspective[J]. Journal of Cleaner Production,2020,250:119553.
    [15] AHMED M J. Adsorption of quinolone, tetracycline, and penicillin antibiotics from aqueous solution using activated carbons:review[J]. Environ Toxicol Pharmacol,2017,50:1-10.
    [16] PRIYA S S, RADHA K V. A Review on the Adsorption studies of tetracycline onto various types of adsorbents[J]. Chemical Engineering Communications,2017,204(8):821-839.
    [17] AHMED M J. Adsorption of non-steroidal anti-inflammatory drugs from aqueous solution using activated carbons:review[J]. Journal of Environmental Management,2017,190:274-282.
    [18] MANSOUR F, AL-HINDI M, YAHFOUFI R, et al. The use of activated carbon for the removal of pharmaceuticals from aqueous solutions:a review[J]. Reviews in Environmental Science and Bio/Technology,2017,17(1):109-145.
    [19] RAKIĆ V, RAJIĆ N, DAKOVIĆ A, et al. The adsorption of salicylic acid, acetylsalicylic acid and atenolol from aqueous solutions onto natural zeolites and clays:clinoptilolite, bentonite and kaolin[J]. Microporous and Mesoporous Materials,2013,166(15):185-194.
    [20] SWARCEWICZ M K, SOBCZAK J, PAZDZIOCH W. Removal of carbamazepine from aqueous solution by adsorption on fly ash-amended soil[J]. Water Science and Technology,2013,67(6):1396-1402.
    [21] DELGADO N, CAPPARELLI A, NAVARRO A, et al. Pharmaceutical emerging pollutants removal from water using powdered activated carbon:study of kinetics and adsorption equilibrium[J]. Journal of Environmental Management,2019,236:301-308.
    [22] REAL F J, BENITEZ F J, ACERO J L, et al. Adsorption of selected emerging contaminants onto PAC and GAC:equilibrium isotherms, kinetics, and effect of the water matrix[J]. Journal of Environmental Science and Health, Part A,2017,52(8):727-734.
    [23] LAWAL I A, MOODLEY B. Fixed-bed and batch adsorption of pharmaceuticals from aqueous solutions on ionic liquid-modified montmorillonite[J]. Chemical Engineering & Technology,2018,41(5):983-993.
    [24] JAIN R, SIKARWAR S, GOYAL S. Kinetics and isotherm studies on the adsorption of an antiparkinsonism drug Entacapone from aqueous solutions using unsaturated polyester resin (UPR)[J]. Desalination and Water Treatment,2014,54(11):3169-3176.
    [25] 朱晟,朱家文,陈葵,等. 红霉素在大孔树脂SP825上的固定床吸附动力学研究[J]. 离子交换与吸附,2012,28(3):257-266.
    [26] MORADI S E, HAJI SHABANI A M, DADFARNIA S, et al. Effective removal of ciprofloxacin from aqueous solutions using magnetic metal-organic framework sorbents:mechanisms, isotherms and kinetics[J]. Journal of the Iranian Chemical Society,2016,13(9):1617-1627.
    [27] VLASOVA E A, NAIDENKO E V, GAINULINA E T, et al. Metal-organic frameworks as sorbents for purification of vegetable Oils[J]. Russian Journal of Applied Chemistry,2018,91(3):524-528.
    [28] VLASOVA E A, SHALUNOVA N K, MAKAROVA A S, et al. Metal-organic frameworks based on terephthalic acid:Sorbents of organic dyes[J]. Russian Journal of Applied Chemistry,2014,87(8):1065-1069.
    [29] MORADI S E, DADFARNIA S, SHABANI A M H, et al. Removal of congo red from aqueous solution by its sorption onto the metal organic framework MIL-100(Fe):equilibrium, kinetic and thermodynamic studies[J]. Desalination And Water Treatment,2015,56(3):709-721.
    [30] MOLAVI H, ZAMANI M, AGHAJANZADEH M, et al. Evaluation of UiO-66 metal organic framework as an effective sorbent for Curcumin's overdose[J]. Applied Organometallic Chemistry,2018,32(4).
    [31] LIU W C, SHEN X, HAN Y Y, et al. Selective adsorption and removal of drug contaminants by using an extremely stable Cu(Ⅱ)-based 3D metal-organic framework[J]. Chemosphere,2019,215:524-531.
    [32] LESSA E F, NUNES M L, FAJARDO A R. Chitosan/waste coffee-grounds composite:an efficient and eco-friendly adsorbent for removal of pharmaceutical contaminants from water[J]. Carbohydrate Polymers,2018,189:257-266.
    [33] MIHCIOKUR H, OGUZ M. Removal of oxytetracycline and determining its biosorption properties on aerobic granular sludge[J]. Environmental Toxicology Pharmacology,2016,46:174-182.
    [34] PEREIRA K A A, OSÓRIO L R, SILVA M P, et al. Chemical modification of chitosan in the absence of solvent for diclofenac sodium removal:pH and kinetics studies[J]. Materials Research,2014,17(suppl 1):141-145.
    [35] PRASERTKULSAK S, CHIEMCHAISRI C, CHIEMCHAISRI W, et al. Removals of pharmaceutical compounds at different sludge particle size fractions in membrane bioreactors operated under different solid retention times[J]. Journal of Hazardous Materials,2019,368:124-132.
    [36] IOVINO P, CANZANO S, CAPASSO S, et al. A modeling analysis for the assessment of ibuprofen adsorption mechanism onto activated carbons[J]. Chemical Engineering Journal,2015,277:360-367.
    [37] NIELSEN L, BANDOSZ T J. Analysis of sulfamethoxazole and trimethoprim adsorption on sewage sludge and fish waste derived adsorbents[J]. Microporous and Mesoporous Materials,2016,220:58-72.
    [38] MIHCIOKUR H, OGUZ M. Removal of oxytetracycline and determining its biosorption properties on aerobic granular sludge[J]. Environmental Toxicology and Pharmacology,2016,46:174-182.
    [39] RAKSHIT S, SARKAR D, PUNAMIYA P, et al. Kinetics of oxytetracycline sorption on magnetite nanoparticles[J]. International Journal of Environmental Science and Technology,2014,11(5):1207-1214.
    [40] JAIN S, VYAS R K, PANDIT P, et al. Adsorption of antiviral drug, acyclovir from aqueous solution on powdered activated charcoal:kinetics, equilibrium, and thermodynamic studies[J]. Desalination and Water Treatment,2014,52(25/26/27):4953-4968.
    [41] LONAPPAN L, ROUISSI T, KAUR B S, et al. An insight into the adsorption of diclofenac on different biochars:Mechanisms, surface chemistry, and thermodynamics[J]. Bioresource Technology,2018,249:386-394.
    [42] YAN B, NIU C H, WANG J. Kinetics, electron-donor-acceptor interactions, and site energy distribution analyses of norfloxacin adsorption on pretreated barley straw[J]. Chemical Engineering Journal,2017,330:1211-1221.
    [43] WONG S, LIM Y, NGADI N, et al. Removal of acetaminophen by activated carbon synthesized from spent tea leaves:equilibrium, kinetics and thermodynamics studies[J]. Powder Technology,2018,338:878-886.
    [44] PARK S H, KIM J H. Isotherm, kinetic, and thermodynamic characteristics for adsorption of 2,5-xylenol onto activated carbon[J]. Biotechnology and Bioprocess Engineering,2018,23(5):541-549.
    [45] ZHANG L, WANG Y, JIN S W, et al. Adsorption isotherm, kinetic and mechanism of expanded graphite for sulfadiazine antibiotics removal from aqueous solutions[J]. Environmental Technology,2017,38(20):2629-2638.
    [46] KHANDAY W A, MARRAKCHI E, ASIF M, et al. Mesoporous zeolite-activated carbon composite from oil palm ash as an effective adsorbent for methylene blue[J]. Journal of the Taiwan Institute of Chemical Engineers,2017,70:32-41.
    [47] ÇALIŞKAN E, GÖKTVRK S. Adsorption characteristics of sulfamethoxazole and metronidazole on activated carbon[J]. Separation Science and Technology,2010,45(2):244-255.
    [48] FUKAHORI S, FUJIWARA T, ITO R, et al. pH-dependent adsorption of sulfa drugs on high silica zeolite:modeling and kinetic study[J]. Desalination,2011,275(1/2/3):237-242.
    [49] QIN T T, WANG Z W, XIE X Y, et al. A novel biochar derived from cauliflower (brassica oleracea L.) roots could remove norfloxacin and chlortetracycline efficiently[J]. Water science and technology:a journal of the International Association on Water Pollution Research,2017,76(11/12):3307-3318.
    [50] LI Z H, CHANG P H, JIANG W T, et al. Removal of diphenhydramine from water by swelling clay minerals[J]. Journal of Colloid Interface Science,2011,360(1):227-232.
    [51] OH S, SHIN W S, KIM H T. Effects of pH, dissolved organic matter, and salinity on ibuprofen sorption on sediment[J]. Environmental Science and Pollution Research,2016,23(22):22882-22889.
    [52] ZHAO Y, LIU F, QIN X P. Adsorption of diclofenac onto goethite:adsorption kinetics and effects of pH[J]. Chemosphere,2017,180:373-378.
    [53] LIU L, HU S Q, SHEN G X, et al. Adsorption dynamics and mechanism of aqueous sulfachloropyridazine and analogues using the root powder of recyclable long-root eichhornia crassipes[J]. Chemosphere,2018,196:409-417.
    [54] ZHAO Y F, CHO C W, CUI L Z, et al. Adsorptive removal of endocrine-disrupting compounds and a pharmaceutical using activated charcoal from aqueous solution:kinetics, equilibrium, and mechanism studies[J]. Environmental Science Pollution Research,2018,26(33):33897-33905.
    [55] LIMBIKAI S S, DESHPANDE N A, KULKARNI R M, et al. Kinetics and adsorption studies on the removal of levofloxacin using coconut coir charcoal impregnated with Al2O3 nanoparticles[J]. Desalination and Water Treatment,2016,57(50):23918-23926.
    [56] JAIN S, VYAS R K, PANDIT P, et al. Adsorption of antiviral drug, acyclovir from aqueous solution on powdered activated charcoal:kinetics, equilibrium, and thermodynamic studies[J]. Desalination and Water Treatment,2013,52(25/26/27):4953-4968.
    [57] HOSSEINI-BANDEGHARAEI A, ALAHABADI A, RAHMANI-SANI A, et al. Effect of nitrate and amine functionalization on the adsorption properties of a macroporous resin towards tetracycline antibiotic[J]. Journal of the Taiwan Institute of Chemical Engineers,2016,66:143-153.
    [58] KONG Q, WANG Y N, SHU L, et al. Isotherm, kinetic, and thermodynamic equations for cefalexin removal from liquids using activated carbon synthesized from loofah sponge[J]. Desalination and Water Treatment,2016,57(17):7933-7942.
    [59] NAEIMI S, FAGHIHIAN H. Remediation of pharmaceutical contaminated water by use of magnetic functionalized metal organic framework. Physicochemical Study of Doxycycline Adsorption[J]. Water and Environment Journal,2018,32(3):422-432.
    [60] KAUR H, BANSIWAL A, HIPPARGI G, et al. Effect of hydrophobicity of pharmaceuticals and personal care products for adsorption on activated carbon:adsorption isotherms, kinetics and mechanism[J]. Environmental Science and Pollution Research,2018,25(21):20473-20485.
    [61] MESTRE A S, MACHUQUEIRO M, SILVA M, et al. Influence of activated carbons porous structure on iopamidol adsorption[J]. Carbon,2014,77:607-615.
    [62] DORDIO A V, MIRANDA S, PRATES RAMALHO J P, et al. Mechanisms of removal of three widespread pharmaceuticals by two clay materials[J]. Journal of Hazardrous Materials,2017,323(Part A):575-583.
    [63] SHAN D N, DENG S B, LI J, et al. Preparation of porous graphene oxide by chemically intercalating a rigid molecule for enhanced removal of typical pharmaceuticals[J]. Carbon,2017,119:101-109.
    [64] ALLEN S J, MCKAY G, PORTER J F. Adsorption isotherm models for basic dye adsorption by peat in single and binary component systems[J]. Journal of Colloid and Interface Science,2004,280(2):322-333.
    [65] AHMARUZZAMAN M. Adsorption of phenolic compounds on low-cost adsorbents:a review[J]. Advances in Colloid and Interface Science,2008,143(1/2):48-67.
    [66] RINGOT D, LERZY B, CHAPLAIN K, et al. In vitro biosorption of ochratoxin a on the yeast industry by-products:comparison of isotherm models[J]. Bioresource Technology,2007,98(9):1812-1821.
    [67] BOULINGUIEZ B, LE CLOIREC P, WOLBERT D. Revisiting tine determination of langnmir parameters-application to tetrahydriotlhiophene adsorption onto activated carbon[J]. Langmuir,2008,24(13):6420-6424.
    [68] KARADAG D, KOC Y, TURAN M, et al. A comparative study of linear and non-linear regression analysis for ammonium exchange by clinoptilolite zeolite[J]. Journal of Hazardous Materials,2007,144(1/2):432-437.
    [69] PEREZ-MARIN A B, ZAPATA V M, ORTUNO J F, et al. Removal of cadmium from aqueous solutions by adsorption onto orange waste[J]. Journal of Hazardous Materials,2007,139(1):122-131.
    [70] 王宜辰. Freundlich吸附等温式的理论推导[J]. 烟台师范学院学报(自然科学版),1993,9(4):76-78.
    [71] SELLAOUI L, MECHI N, LIMA ÉC, et al. Adsorption of diclofenac and nimesulide on activated carbon:statistical physics modeling and effect of adsorbate size[J]. Journal of Physics and Chemistry of Solids,2017,109:117-123.
    [72] PLAZINSKI W, RUDZINSKI W, PLAZINSKA A. Theoretical models of sorption kinetics including a surface reaction mechanism:a review[J]. Advances in Colloid and Interface Science,2009,152(1/2):2-13.
    [73] FEBRIANTO J, KOSASIH A N, SUNARSO J, et al. Equilibrium and kinetic studies in adsorption of heavy metals using biosorbent:A summary of recent studies[J]. Journal of Hazardous Materials,2009,162(2/3):616-645.
    [74] HO Y S, MCKAY G. Pseudo-second order model for sorption processes[J]. Process Biochemistry,1999,34(5):451-465.
    [75] NAGHIPOUR D, AMOUEI A, ESTAJI M, et al. Cephalexin adsorption from aqueous solutions by biochar prepared from plantain wood:equilibrium and kinetics studies[J]. Desalination and Water Treatment,2019,143:374-381.
    [76] de FRANCO M A E, de CARVALHO C B, BONETTO M M, et al. Diclofenac removal from water by adsorption using activated carbon in batch mode and fixed-bed column:isotherms, thermodynamic study and breakthrough curves modeling[J]. Journal of Cleaner Production,2018,181:145-154.
    [77] STYSZKO K, SZCZUROWSKI J, CZUMA N, et al. Adsorptive removal of pharmaceuticals and personal care products from aqueous solutions by chemically treated fly ash[J]. International Journal of Environmental Science and Technology,2017,15(3):493-506.
    [78] FOUNTOULI T V, CHRYSIKOPOULOS C V. Adsorption and thermodynamics of pharmaceuticals, acyclovir and fluconazole, onto quartz sand under static and dynamic conditions[J]. Environmental Engineering Science,2018,35(9):909-917.
    [79] ANTON-HERRERO R, GARCIA-DELGADO C, ALONSO-IZQUIERDO M, et al. Comparative adsorption of tetracyclines on biochars and stevensite:looking for for the most effective adsorbent[J]. Applied Clay Science,2018,160:162-172.
    [80] LAWAL I A, MOODLEY B. Sorption mechansim of pharmaceuticals from aqueous medium on ionic liquid modified biomass[J]. Journal of Chemical Technology & Biotechnology,2017,92(4):808-818.
    [81] SARKAR M, ACHARYA P K, BHATTACHARYA B. Modeling the adsorption kinetics of some priority organic pollutants in water from diffusion and activation energy parameters[J]. Journal of Colloid and Interface Science,2003,266(1):28-32.
    [82] TORRELLAS S A, RODRIGUEZ A R, ESCUDERO G O, et al. Comparative evaluation of adsorption kinetics of diclofenac and isoproturon by activated carbon[J]. Journal of Environmental Science and Health. Part A, Toxic Hazardous Substances Environmental Engineering,2015,50(12):1241-1248.
    [83] YU Z R, PELDSZUS S, HUCK H P. Adsorption of selected pharmaceuticals and an endocrine disrupting compound by granular activated carbon. 1. Adsorption capacity and kinetics[J]. Environmental Science & Technology,2009,43(5):1467-1473.
    [84] YU Z R, PELDSZUS S, HUCK H P. Adsorption of selected pharmaceuticals and an endocrine disrupting compound by granular activated carbon. 2. Model prediction[J]. Environmental Science & Technology,2009,43(5):1474-1479.
  • 加载中
计量
  • 文章访问数:  252
  • HTML全文浏览量:  39
  • PDF下载量:  14
  • 被引次数: 0
出版历程
  • 收稿日期:  2020-04-23
  • 网络出版日期:  2021-07-19

目录

    /

    返回文章
    返回