难降解含聚采出水处理技术研究进展

屈璇; 尹安伟; 方艾伦; 李春燕; 冯东磊; 李昂

doi:10.13205/j.hjgc.202111005

难降解含聚采出水处理技术研究进展

doi: 10.13205/j.hjgc.202111005

1. 哈尔滨工业大学城市水资源与水环境国家重点实验室, 哈尔滨 150090;
2. 扬州市海诚生物技术有限公司, 江苏扬州 225600

基金项目:

国家自然科学基金（51878212）。

详细信息

作者简介:
屈璇(1993-),女,博士研究生,主要研究方向为油气田废水处理技术。quxuana@163.com

通讯作者:
李昂(1980-),男,工学博士,教授,主要研究方向为环境生物技术。li.ang@hit.edu.cn

计量
- 文章访问数: 247
- HTML全文浏览量: 34
- PDF下载量: 25
- 被引次数: 0
出版历程
- 收稿日期: 2021-07-30
- 网络出版日期: 2022-01-26

RESEARCH PROGRESS ON TREATMENT TECHNOLOGY OF REFRACTORY POLYMER-CONTAINING OILFIELD PRODUCED WATER

1. State Key Laboratory of Urban Water Resource and Environment, Harbin Institute of Technology, Harbin 150090, China;
2. Yangzhou Haicheng Biotech Co., Ltd, Yangzhou 225600, China

摘要

摘要: 含聚采出水具有水质复杂、黏度大、乳化程度高、含油量高等特点，导致油水分离困难，对油田生产作业和环境带来严重影响。分析了含聚采出水的水质特性，对国内外含聚采出水处理技术进行了总结，如膜分离法、气浮法、高级氧化法、微生物法等，阐述了这些处理技术在油田的应用情况及存在的问题。简要说明了含聚采出水处理工艺及橇装一体化水处理装置开发问题，对今后的含聚采出水处理技术的研究进行了展望，以期为该类污水处理技术的研究和工程应用提供参考。
- 油田采出水 /
- 污水处理 /
- 聚合物驱 /
- 油水分离
Abstract: Produced water containing polymer has the characteristics of complex water quality, high viscosity, high degree of emulsification, and high oil content, which causes difficulty in oil-water separation and has serious impacts on oilfield production operations and the environment. This study analyzed the water quality characteristics of the polymer-containing produced water, and summarized the treatment technologies of the polymer-containing produced water, such as membrane separation method, air flotation method, advanced oxidation method, microbial method, etc., and explained the application of these treatment processes in various oil fields. The advantages and problems of various treatment technologies were described. This study also introduced the treatment technologies of polymer-containing produced water and the development of skid-mounted integrated water treatment equipment. Finally, some prospects were put forward for future research of polymer-containing produced water treatment technology, hoping to provide reference for the researches and engineering application of the sewage treatment technology.
- oilfield produced water /
- sewage treatment /
- polymer flooding /
- oil-water separation

HTML全文

参考文献(55)

[1]	李杰训,赵雪峰,田晶.高含水期大庆油田油气集输系统地面规划的做法与认识[J].石油规划设计,2017,28(4):8-11.
[2]	陈忠喜,舒志明.大庆油田采出水处理工艺及技术[J].工业用水与废水,2014,45(1):36-46.
[3]	何玉辉.大庆油田采出水处理新技术[J].油气田地面工程,2013,32(10):79-80.
[4]	付强.大庆油田采出水处理系统的优化简化[J].油气田地面工程,2013,32(2):52.
[5]	黄斌,王晨,傅程,等.三元复合驱采出水处理研究进展[J].化工进展,2020,39(10):4238-4247.
[6]	程杰成, 吴军政, 吴迪. 三元复合驱油技术[M]. 北京:石油工业出版社, 2013.
[7]	LI J X, LIU Y, WU D, et al. The synergistic effects of alkaline, surfactant, and polymer on the emulsification and destabilization of oilin-water crude oil emulsion produced by alkaline-surfactant-polymer flooding[J]. Petroleum Science and Technology, 2013, 31:399-407.
[8]	鞠野. 一元/二元/三元驱油体系微观驱油机理研究[D]. 大庆:大庆石油学院, 2006.
[9]	OREM W, TATU C, VARONKA M, et al. Organic substances in produced and formation water from unconventional natural gas extraction in coal and shale[J]. International Journal of Coal Geology, 2014, 126:20-31.
[10]	LESTER Y, FERRER I, THURMAN E M, et al. Characterization of hydraulic fracturing flowback water in Colorado:implications for water treatment[J]. Science of the Total Environment, 2015, 512-513:637-644.
[11]	STRINGFELLOW W T, DOMEN J K, CAMARILLO M K, et al. Physical, chemical, and biological characteristics of compounds used in hydraulic fracturing[J]. Journal of Hazardous Materials, 2014, 275:37-54.
[12]	THURMAN E M, FERRER I, BLOTEVOGEL J, et al. Analysis of hydraulic fracturing flowback and produced waters using accurate mass:identification of ethoxylated surfactants[J]. Analytical Chemistry, 2014, 86(19):9653-9661.
[13]	LAN D, CHEN M, LIU Y, et al. Development of shale gas in china and treatment options for wastewater produced from the exploitation:sustainability lessons from the united states[J]. Journal of Environmental Engineering, 2020, 146(9):04020103.
[14]	ZHANG Z Y, DU X W, CARLSON K H, et al. Effective treatment of shale oil and gas produced water by membrane distillation coupled with precipitative softening and walnut shell filtration[J]. Desalination, 2019, 454:82-90.
[15]	SHANG W, LIU Y H, HE Q P, et al. Efficient adsorption of organic matters and ions by porous biochar aerogel as pre-treatment of ultrafiltration for shale gas wastewater reuse[J]. Chemical Engineering Journal Advances, 2020, 2:100011.
[16]	梁毅, 李春光, 唐杨,等. 基于高效聚结技术的放射性油水分离系统改造[J]. 净水技术, 2019, 38(2):105-108 ,120.
[17]	ETCHEPARE R, OLIVEIRA H, AZEVEDO A, et al. Separation of emulsified crude oil in saline water by dissolved air flotation with micro and nanobubbles[J]. Separation and Purification Technology, 2017, 186:326-332.
[18]	WANG C Y, WANG Z X, WEI X Y, et al. A numerical study and flotation experiments of bicyclone column flotation for treating of produced water from ASP flooding[J]. Journal of Water Process Engineering, 2019, 32:100972.
[19]	李永丰, 刘敏, 王晓飞,等. 海上油田含聚生产水旋流气浮装置试验研究[J]. 油气田地面工程, 2016, 35(10):22-25.
[20]	TAWALBEH M, AL MOJJLY A, Al-OTHMAN A, et al. Membrane separation as a pre-treatment process for oily saline water[J]. Desalination, 2018, 447:182-202.
[21]	CHANG H Q, LI T, LIU B C, et al. Potential and implemented membrane-based technologies for the treatment and reuse of flowback and produced water from shale gas and oil plays:a review[J]. Desalination, 2019, 455:34-57.
[22]	CHANG H Q, LIU S, TONG T Z, et al. On-site treatment of shale gas flowback and produced water in Sichuan Basin by fertilizer drawn forward osmosis for irrigation[J]. Environmental Science & Technology, 2020, 54(17):10926-10935.
[23]	GUO C, CHANG H Q, LIU B C, et al. A combined ultrafiltration-reverse osmosis process for external reuse of Weiyuan shale gas flowback and produced water[J]. Environmental Science:Water Research & Technology, 2018, 4(7):942-955.
[24]	WESCHENFELDER S E, LOUVISSE A, BORGES C P, et al. Evaluation of ceramic membranes for oilfield produced water treatment aiming reinjection in offshore units[J]. Journal of Petroleum Science & Engineering, 2015, 131:51-57.
[25]	MILLER H, DIAS K, HARE H, et al. Reusing oil and gas produced water for agricultural irrigation:effects on soil health and the soil microbiome[J]. Science of the Total Environment, 2020, 722:137888.
[26]	KUSWORO T D, ARYANTI N, UTOMO D P. Oilfield produced water treatment to clean water using integrated activated carbon-bentonite adsorbent and double stages membrane process[J]. Chemical Engineering Journal, 2018, 347:462-471.
[27]	ZHANG B, YU S L, ZHU Y B, et al. Application of a polytetrafluoroethylene (PTFE) flat membrane for the treatment of pre-treated ASP flooding produced water in a Daqing oilfield[J]. RSC Advances, 2016, 6(67):62411-62419.
[28]	LAN D, CHEN M, LIU Y, et al. Development of shale gas in china and treatment options for wastewater produced from the exploitation:sustainability lessons from the united states[J]. Journal of Environmental Engineering, 2020, 146(9):04020103.
[29]	ZHONG C, ZOLFAGHARI A, HOU D, et al. Comparison of the hydraulic fracturing water cycle in china and north america:a critical review[J]. Environmental Science & Technology, 2021.
[30]	ZHANG Z J, ZHUANG Y L, LI J L, et al. Feasibility evaluation of the treatment and recycling of shale gas produced water:a case study of the first shale gas field in the Eastern Sichuan Basin, China[J]. Environmental Science:Water Research & Technology, 2019, 5(2):358-369.
[31]	OETJEN K, CHAN K E, GULMARK K, et al. Temporal characterization and statistical analysis of flowback and produced waters and their potential for reuse[J]. Science of the Total Environment, 2018, 619:654-664.
[32]	ROSENBLUM J, NELSON A W, RUYLE B, et al. Temporal characterization of flowback and produced water quality from a hydraulically fractured oil and gas well[J]. Science of the Total Environment, 2017, 596:369-377.
[33]	ZHANG W J, ZHANG M, XIAO F, et al. Pretreatment of high strength waste emulsions by combined vibratory shear enhanced process with Fenton oxidation[J]. International Journal of Environmental Science and Technology, 2014, 11(3):731-738.
[34]	尹立平,张浩男.磁分离技术在低含聚污水处理中的应用[J].油气田地面工程,2016,35(4):96-97.
[35]	MILLAR G J, LIN J, ARSHAD A, et al. Evaluation of electrocoagulation for the pre-treatment of coal seam water[J]. Journal of Water Process Engineering, 2014, 4:166-178.
[36]	ESMAEILIRAD N, CARLSON K, OZBEK P O. Influence of softening sequencing on electrocoagulation treatment of produced water[J]. Journal of Hazardous Materials, 2015, 283:721-729.
[37]	宋学峰,吴越强,许成君,王飞.电化学在三元复合驱采出水深度处理中的应用[J].油气田环境保护,2019,29(2):18-20 ,61.
[38]	ZHANG H, XIONG Z K, JI F Z, et al. Pretreatment of shale gas drilling flowback fluid (SGDF) by the microscale Fe⁰/persulfate/O₃ process (mFe⁰/PS/O₃)[J]. Chemosphere, 2017, 176:192-201.
[39]	陈春茂, 曹越, 胡景泽,等. 难降解石油化工废水臭氧氧化处理催化剂研究进展[J]. 工业水处理, 2020, 40(4):1-5 ,88.
[40]	CHEN C, YOZA B A, CHEN H, et al. Manganese sand ore is an economical and effective catalyst for ozonation of organic contaminants in petrochemical wastewater[J]. Water, Air, & Soil Pollution, 2015, 226(6):1-11.
[41]	LIU P, REN Y, MA W, et al. Degradation of shale gas produced water by magnetic porous MFe₂O₄ (M=Cu, Ni, Co and Zn) heterogeneous catalyzed ozone[J]. Chemical Engineering Journal, 2018, 345:98-106.
[42]	廖传华, 廖玮, 朱跃钊,等. 一种用于稠油热采的超临界流体的制备系统和方法:中国,CN108251093A[P]. 2018.
[43]	廖玮,朱廷风,廖传华,等.超临界水氧化技术在能量转化中的应用[J].水处理技术,2019,45(3):14-17.
[44]	王存英, 张达志. 微波破乳-双旋流气浮处理含油污水试验[J]. 环境工程, 2016, 34(5):1-5.
[45]	刘岩, 刘东方, 高芳, 等. 酵母菌-水解酸化-MBR工艺处理三元驱采出水的研究[J]. 工业水处理, 2015, 35(4):41-44.
[46]	刘长莉, 王宝鑫, 李娜, 等. 弱碱三元采出水ABR生物处理工艺研究[J]. 环境科学与技术, 2015,38(增刊1):198-204.
[47]	郭东璞, 林永波, 李永峰. 不同类型油田采出水作为阳极底物对MFC电压的影响[J]. 安徽农业科学, 2014, 42(2):523-526.
[48]	黄雪松, 王晓颖, 张丽. 中原油田复杂采出水"微生物+膜"处理研究及现场试验[J]. 安全.健康和环境, 2021,21(2):25-29.
[49]	周勇, 郭靖, 梁家豪,等. 三元复合驱含油污水处理技术研究进展[J]. 工业水处理, 2020,40(8):7-10.
[50]	ZHOU X Y, ZHANG H R, LONG Y, et al. Sustainable and clean oilfield development:optimal operation of wastewater treatment and recycling system[J]. Journal of Cleaner Production, 2020, 252:119819.
[51]	杨欢,赵华,陈腾巍. 油气地面管线内结垢固体颗粒沉积影响因素的实验研究[J]. 科学技术与工程,2016,16(9):80-85.
[52]	张立伟. 三元复合驱含油污水"双膜"深度处理集成技术研究[D]. 长春:吉林大学,2018.
[53]	唐洪明,龚小平,唐浩轩,等.页岩敏感性损害评价方法及损害机理[J]. 中南大学学报(自然科学版),2016,47(4):1227-1236.
[54]	王庆吉.油田含硫采出水橇装一体化处理装置设计及应用[J].工业水处理,2021,41(1):147-150.
[55]	UMAR A A, SAAID I B M, SULAIMON A A, et al. A review of petroleum emulsions and recent progress on water-in-crude oil emulsions stabilized by natural surfactants and solids[J]. Journal of Petroleum Science and Engineering, 2018, 165:673-690.