多因素共同作用对中温条件下污泥与餐厨垃圾联合厌氧发酵产H<sub>2</sub>的影响

王永萍; 方皓珏; 华若婷; 何雨恒; 张燕琼; 郑育毅; 刘常青; 甄广印

doi:10.13205/j.hjgc.202303014

多因素共同作用对中温条件下污泥与餐厨垃圾联合厌氧发酵产H₂的影响

doi: 10.13205/j.hjgc.202303014

1. 福建师范大学地理科学学院碳中和未来技术学院, 福州 350007;
2. 福建师范大学环境与资源学院碳中和现代产业学院福建省污染控制与资源循环利用重点实验室, 福州 350007;
3. 城市废物资源化技术与管理福建省高校工程研究中心, 福州 350007;
4. 华东师范大学生态与环境科学学院, 上海 200241

基金项目:

福建省科技厅公益类项目(2019R1015-1)

福建省科技厅对外合作项目(2021I0010)

福建省科技厅计划项目(2020N5015)

详细信息

作者简介:
王永萍(1996-),女,硕士研究生,主要研究方向为固体废物处理与资源化。2219362906@qq.com

通讯作者:
刘常青(1970-),女,博士,副教授,主要研究方向为固体废物处理与资源化。mylcq@yeah.net

计量
- 文章访问数: 110
- HTML全文浏览量: 16
- PDF下载量: 6
- 被引次数: 0
出版历程
- 收稿日期: 2022-04-12
- 网络出版日期: 2023-05-26
- 刊出日期: 2023-03-01

COMPREHENSIVE INFLUENCE OF MULTIPLE FACTORS ON HYDROGEN PRODUCTION FROM COMBINED ANAEROBIC FERMENTATION OF SLUDGE AND KITCHEN WASTE UNDER MEDIUM TEMPERATURE CONDITION

1. School of Geographical Sciences and School of Carbon Neutrality Future Technology, Fujian Normal University, Fuzhou 350007, China;
2. College of Environmental and Resource Sciences and College of Carbon Neutral Modern Industry, Fujian Key Laboratory of Pollution Control and Resource Reuse, Fujian Normal University, Fuzhou 350007, China;
3. Urban Waste Resource Technology and Management Fujian University Engineering Research Center, Fuzhou 350007, China;
4. School of Ecological and Environmental Science, East China Normal University, Shanghai 200241, China

摘要

摘要: 污泥与餐厨垃圾联合厌氧发酵产H₂既可减少环境污染,又可制备清洁能源,是一种理想的有机固废处理处置技术。通过4因素5水平正交设计的批式实验及产氢动力学,探究餐厨垃圾C/N、混合体系C/N、含水率、初始pH值4个主要因素共同作用对中温条件下污泥餐厨垃圾联合厌氧发酵产H₂的影响。极差与方差分析结果表明:4个主要因素对联合厌氧发酵产H₂结果影响较明显,而餐厨垃圾C/N和混合体系C/N的交互作用对产H₂结果的影响不显著。不考虑交互作用,以比氢气产量为产H₂效能主要表征指标,最终确定餐厨垃圾C/N 为20,联合发酵体系C/N为 10,初始pH值为7,含水率为90%时,产H₂效能最佳,此时的累积产氢量为1499.6 mL,比氢气产量为140.96 mL H₂/g DS,最大产氢速率为21.73 mL H₂/h,最大H₂浓度为55.79%。
- 污泥 /
- 餐厨垃圾 /
- 联合厌氧发酵 /
- 正交实验 /
- 产H₂ /
- 优化
Abstract: The combined anaerobic fermentation of sludge and kitchen waste under medium temperature to produce hydrogen is an ideal treatment and disposal technology for both reducing environmental pollution and generating clean energy. Through batch experiment with four factors and a five-level orthogonal design, the effects of four main factors, including kitchen waste C/N, system C/N, moisture content and initial pH value on the hydrogen production from the combined anaerobic fermentation of sludge and kitchen waste based on the hydrogen production performance, and the key factors optimization of conditions were studied under medium temperature condition. The analysis of range and variance showed that the four main factors had an obvious effect on hydrogen production performance, but neither did the interaction of kitchen waste C/N and system C/N. Meanwhile, ignoring the interaction effect, the optimal operational conditions obtained by orthogonal design with the maximum specific hydrogen yield as the dominant indication of biohydrogen performance were: a kitchen waste C/N of 20, combined anaerobic fermentation system C/N of 10, initial pH of 7 and moisture content of 90%, and the corresponding cumulative hydrogen production, specific hydrogen yield, maximum hydrogen production rate and maximum hydrogen concentration was 1499.6 mL, 140.96 mL H₂/g DS, 21.73 mL H₂/h and 55.79%, respectively.
- sludge /
- kitchen waste /
- combined anaerobic fermentation /
- orthogonal experiment /
- hydrogen production /
- optimization

HTML全文

参考文献(40)

[1]	JIN C X, SUN S Q, YANG D H, et al. Anaerobic digestion:an alternative resource treatment option for food waste in China[J]. Science of the Total Environment, 2021,779:146397.
[2]	TAO Z T, WANG D B, YAO F B, et al. The effects of thiosulfinates on methane production from anaerobic co-digestion of waste activated sludge and food waste and mitigate method[J]. Journal of Hazardous Materials, 2020, 384:121363.
[3]	YUN Y M, LEE M K, IM S W, et al. Biohydrogen production from food waste:current status, limitations, and future perspectives[J]. Bioresource Technology, 2018, 248:79-87.
[4]	ARAIN M, MAHAR R B, SAHITO A R, et al. Biohydrogen production from co-digestion of high carbohydrate containing food waste and combined primary and secondary sewage sludge[J]. Mehran University Research Journal of Engineering and Technology, 2018, 37(1).
[5]	SREELA-OR C, PLANGKLANG P, IMAI T, et al. Co-digestion of food waste and sludge for hydrogen production by anaerobic mixed cultures:statistical key factors optimization[J].International Journal of Hydrogen Energy, 2011, 36(21):14227-14237.
[6]	ALIBARDI L, COSSU R. Effects of carbohydrate, protein and lipid content of organic waste on hydrogen production and fermentation products[J]. Waste Management, 2015, 47(JAN.PT.A):69-77.
[7]	YANG G, WANG J L. Fermentative hydrogen production from sewage sludge[J]. Critical Reviews in Environmental Science & Technology, 2017,47(13/14/15/16/17/18):1219-1281.
[8]	HASSAN G K, HEMDON B A, EL-GOHARY F A. Utilization of food waste for bio-hydrogen and bio-methane production:influences of temperature, OLR, and in situ aeration[J]. Journal of Material Cycles and Waste Management, 2020, 22(4):1218-1226.
[9]	ZHANG P S, LIU C Q, ZHENG Y Y, et al. Statistical key factor optimization of conditions for biohydrogen production from sewage sludge and food waste by anaerobic Co-digestion[J]. Energy & Fuels, 2019, 33(11):11163-11172.
[10]	CHENG J, DIND L K, LIN R C, et al. Fermentative biohydrogen and biomethane co-production from mixture of food waste and sewage sludge:effects of physiochemical properties and mix ratios on fermentation performance[J]. Applied Energy, 2016, 184:1-8.
[11]	LI Z P, CHEN Z, YE H, et al. Anaerobic co-digestion of sewage sludge and food waste for hydrogen and VFA production with microbial community analysis[J]. Waste Management, 2018,78:789-799.
[12]	YIN D X, LIU W, ZHAI N N, et al. Influence of pH controlling on fermentation performance in kitchen waste and cow manure[J]. Energy Sources Part A Recovery Utilization and Environmental Effects, 2019,43(19/20/21/22/23/24):2339-2351.
[13]	CAPPAI G, GIOANNIS G D, FRIARGIU M, et al. An experimental study on fermentative H₂ production from food waste as affected Cappai G by pH[J]. Waste Management, 2014, 34(8):1510-1519.
[14]	蒲贵兵,吕波,尹洪军.餐厨垃圾发酵产氢中比产氢率与pH值的关系[J].重庆理工大学学报(自然科学版),2013,27(6):48-52.
[15]	ALZATE M E, MUOZ R, ROGALLA F, et al. Biochemical methane potential of microalgae:influence of substrate to inoculum ratio,biomass concentration and pretreatment[J].Bioresource Technology, 2012,123(none):488-494.
[16]	CAPSON-TOJO G, TRABLY E, ROUEZ M, et al. Cardboard proportions and total solids contents as driving factors in dry co-fermentation of food waste[J]. Bioresource Technology, 2018, 248, 229-237.
[17]	RAMOS C, BUITRON G, MORENO-Andrade I, et al. Effect of the initial total solids concentration and initial pH on the bio-hydrogen production from cafeteria food waste[J]. International Journal of Hydrogen Energy, 2012, 37(18):13288-13295.
[18]	ZUO W, E J Q, LIU X L, et al. Orthogonal Experimental Design and Fuzzy Grey Relational Analysis for emitter efficiency of the micro-cylindrical combustor with a step[J]. Applied Thermal Engineering, 2016, 103:945-951.
[19]	CHENG Z, YU L, LI H H, et al. Use of housefly (Musca domestica L.) larvae to bioconversion food waste for animal nutrition and organic fertilizer[J]. Environmental Science and Pollution Research, 2021,28(35):48921-48928.
[20]	周雨绮,许俊超,卓桂华,等.中温条件下污泥接种量对污泥-餐厨垃圾联合厌氧发酵产氢余物产甲烷的影响[J].环境工程, 2021, 39(6):144-149.
[21]	张庆军,谢颖,吴松.基于正交实验与回归分析的机载共形天线吸波涂层厚度预测[J].兵工学报,2021,42(12):2693-2699.
[22]	李迎新,王勇,李彤,等.温度和物料配比对餐厨垃圾与果蔬垃圾协同厌氧产氢的影响研究[J].环境污染与防治,2018,40(3):259-264.
[23]	李彤, 王勇, 李迎新,等. 餐厨垃圾与市政污泥协同厌氧制氢影响因素研究[J]. 太阳能学报, 2019, 40(8):2135-2142.
[24]	HO K S, CHU L M. Characterization of food waste from different sources in Hong Kong[J]. Journal of the Air & Waste Management Association, 2019, 69(3):277-288.
[25]	袁雨珍,肖利平,刘传平,等. pH对餐厨垃圾厌氧发酵产氢过程的影响[J].生态环境学报,2017,26(4):687-692.
[26]	陈宏, 吴军, 陈晨,等. 有机废弃物厌氧共发酵制氢研究进展[J]. 化工进展, 2021, 40(1):440-450.
[27]	LI Y Y, JIN Y Y, BORRION A, et al. Current status of food waste generation and management in China[J]. Bioresource Technology, 2019, 273:654-665.
[28]	JIANG J F, WU P W, SUN Y M, et al. Comparison of microbial communities during anaerobic digestion of kitchen waste:effect of substrate sources and temperatures[J]. Bioresource Technology, 2020, 317:124016.
[29]	ZHANG X T, JIANG D P, ZHANG H, et al. Enhancement of the biohydrogen production performance from mixed substrate by photo-fermentation:effects of initial pH and inoculation volume ratio[J]. Bioresource Technology, 2021, 319:124153.
[30]	ZAKA M, SOLANKI R, BHALE P V, et al. Experimental investigation on anaerobic co-digestion of food waste and water hyacinth in batch type reactor under mesophilic condition[J]. Biomass Conversion and Biorefinery, 2020, 10(2):707-714.
[31]	BLASIUS J P, CASTRO M, MAINYINGUER S I, et al. Effects of temperature, proportion and organic loading rate on the performance of anaerobic digestion of food waste[J]. Biotechnology Reports, 2020, 27:e00503.
[32]	JARUNGLUMLERT T, PROMMUAK C, PUTMAI N, et al. Scaling-up bio-hydrogen production from food waste:feasibilities and challenges[J]. International Journal of Hydrogen Energy, 2017, 43(2):634-648.
[33]	MAHATO R K, KUMAR D, RAJAGOPALAN G J R E. Biohydrogen production from fruit waste by Clostridium strain BOH₃[J]. Renewable Energy, 2020, 153:1368-1377.
[34]	岳远, 李兵, 王伟锋,等. 餐厨垃圾与市政污泥共消化厌氧产氢研究[J]. 宁波大学学报(理工版), 2018, 31(6):110-114.
[35]	宋庆彬, 李爱民, 鞠茂伟,等. 厨余和污泥不同混合比例碱处理产氢特性研究[J]. 太阳能学报, 2010, 31(3):396-400.
[36]	SHIN H S, KIM S H, PAIK B C. Characteristics of hydrogen production from food waste and waste activated sludge[J]. Journal of Water and Environment Technology, 2003.
[37]	ZHU H G, PARKER W, BASNAR R, et al. Biohydrogen production by anaerobic co-digestion of municipal food waste and sewage sludges[J]. International Journal of Hydrogen Energy, 2008, 33(14):3651-3659.
[38]	DEHERI C, MOHANTY A P, ACHARYA S K. An experimental approach to produce hydrogen from food waste, cow dung, and sludge solution[J]. Materials Today:Proceedings, 2020,41:242-246.
[39]	NAM J Y, KIM D H, KIM S H, et al. Harnessing dark fermentative hydrogen from pretreated mixture of food waste and sewage sludge under sequencing batch mode[J]. Environmental Science and Pollution Research, 2016, 23(8):7155-7161.
[40]	LIU X Y, LI R Y, JI M. Effects of two-stage operation on stability and efficiency in Co-digestion of food waste and waste activated sludge[J]. Energies, 2019, 12(14):1-21.