全氟和多氟烷基物质对生物环境作用的研究进展

郭海荣; 刘庆玉; 杨婧; 贺莉

doi:10.13205/j.hjgc.202308033

全氟和多氟烷基物质对生物环境作用的研究进展

doi: 10.13205/j.hjgc.202308033

郭海荣^1,2,
刘庆玉²,
杨婧³,
贺莉^1, ,

1. 农业农村部沼气科学研究所, 成都 610041;
2. 沈阳农业大学工程学院, 沈阳 110161;
3. 中国环境监测总站国家环境保护环境监测质量控制重点实验室, 北京 100012

基金项目:

四川省科技支撑项目(2021ZDZX0012)

国家自然科学基金(31902208)

详细信息

作者简介:
郭海荣(1997-),博士研究生,主要从事废弃物资源化利用研究。2021200003@stu.syau.edu.cn

通讯作者:
贺莉(1981-),研究员,主要从事废弃物资源化利用的研究。heli@caas.cn

计量
- 文章访问数: 117
- HTML全文浏览量: 20
- PDF下载量: 7
- 被引次数: 0
出版历程
- 收稿日期: 2022-07-27
- 网络出版日期: 2023-11-15

RESEARCH PROGRESS ON EFFECTS OF PER- AND POLY-FLUOROALKYL SUBSTANCES ON BIOLOGICAL ENVIRONMENT

GUO Hairong^1,2,
LIU Qingyu²,
YANG Jing³,
HE Li^{1
, ,}

1. Biogas Institute of Ministry of Agriculture and Rural Affairs, Chengdu 610041, China;
2. College of Engineering, Shenyang Agricultural University, Shenyang 110161, China;
3. China National Environmental Monitoring Centre, State Environmental Protection Key Laboratory of Quality Control in Environmental Monitoring, Beijing 100012, China

摘要

摘要: 近年来,随着工业和制造业的高速发展,含有全氟和多氟烷基物质(PFAS)的产品已在人类活动的各个领域内被大量应用并传播至生物环境中。由于PFAS的强稳定性和累积毒性,PFAS已对生物的生存环境造成了众多消极影响。尽管对PFAS的研究已有数十年,但PFAS的全球传播和生态治理难题仍未有效解决。综述了关于PFAS化合物持续影响生物环境的5个重要问题:1)目前生物环境中PFAS的暴露状况和PFAS引起的社会关注;2)生物环境中PFAS化合物的来源及其传播途径;3)3种典型PFAS化合物对生物环境造成的威胁;4)在逐年递增的环境暴露度下,各国对于PFAS化合物的管控措施和研究阻碍;5)目前PFAS化合物的研究进展及未来研究学者需要克服的问题。针对上述问题总结了以往研究报道的结论与建议,根据目前PFAS化合物的探索程度以及研究方向提出了5条潜在的研究方向,旨在为科学研究和管理阶层创建联系,实现人类活动与生态循环的绿色协同发展。
- 全氟和多氟烷基物质 /
- 生物环境 /
- 生态循环 /
- 可持续发展 /
- 环境污染
Abstract: The global biological environment is in the harm caused by per- and poly-fluoroalkyl substances (PFAS). In recent decades, with the rapid development of industry and manufacturing, products containing PFAS have been widely used in various fields of human activities and spread to the biological environment. Due to the strong stability and cumulative toxicity of PFAS, it has caused many negative impacts on the living environment of organisms. Although PFAS has been studied for decades, the global communication and ecological governance problems of PFAS are still unresolved. In this paper, five important issues concerning the continuous impact of PFAS compounds on the biological environment are summarized: 1) the current exposure of PFAS in the biological environment and the social concerns of PFAS; 2) sources and transmission routes of PFAS compounds in the biological environment; 3) the threats of three typical PFAS compounds to the biological environment; 4) under the increasing environmental exposure, the control measures and research obstacles of PFAS compounds in various countries; 5) the current research progress of PFAS compounds and the problems that future researchers need to overcome. This paper summarizes the conclusions and suggestions from previous research reports on the above issues, and proposes five potential ways according to the current degree of exploration and research direction of PFAS compounds, aiming to create links between scientific research and management, and achieve the green and coordinated development of human activities and ecological cycle.
- PFAS /
- biological environment /
- ecological cycle /
- sustainable development /
- ecological pollution

HTML全文

参考文献(108)

[1]	张善宇,姚谦,施蓉,等.全氟与多氟烷基物质的生殖毒性研究进展[J].环境与职业医学,2021,38(10):1161-1168.
[2]	OLSEN G W,BURRIS J M,EHRESMAN D J,et al.Half-life of serum elimination of perfluorooctanesulfonate,perfluorohexanesulfonate,and perfluorooctanoate in retired fluorochemical production workers[J].Environ Health Perspect,2007,115(9):1298-1305.
[3]	YU C H,WEISEL C P,ALIMOKHTARI S,et al.Biomonitoring:a tool to assess PFNA body burdens and evaluate the effectiveness of drinking water intervention for communities in New Jersey[J].International Journal of Hygiene and Environmental Health,2021,235:113757.
[4]	EUN H,YAMAZAKI E,TANIYASU S,et al.Evaluation of perfluoroalkyl substances in field-cultivated vegetables[J].Chemosphere,2020,239:124750.
[5]	SEMERAD J,HORKA P,FILIPOVA A,et al.The driving factors of per- and polyfluorinated alkyl substance (PFAS) accumulation in selected fish species:the influence of position in river continuum,fish feed composition,and pollutant properties[J].The Science of the total environment,2022,816:151662.
[6]	Environmental Protection Agency(EPA).EPA’s PFAS action plan.(2019-02-14)[2020-05-15].https://www.epa.gov/sites/production/files/2019-02/documents/pfas_action_plan_021319_508compliant_1.pdf.
[7]	谢双蔚.我国全氟辛烷磺酸(PFOS)排放源识别与排放估算研究[D].北京:中国科学院大学,2013.
[8]	LIU L,QU Y,HUANG J,et al.Per- and polyfluoroalkyl substances (PFASs) in Chinese drinking water:risk assessment and geographical distribution[J].Environmental Sciences Europe,2021,33(1):1-12.
[9]	肖子冰,邢航,窦增培.自然环境中能否出现可有效降解碳氟链的微生物[J].日用化学工业,2021,51(12):1242-1249.
[10]	AL AMIN M,SOBHANI Z,LIU Y,et al.Recent advances in the analysis of per- and polyfluoroalkyl substances (PFAS)—A review[J].Environmental Technology & Innovation,2020,19:100879.
[11]	PREVEDOUROS K,COUSINS I T,BUCK R C,et al.Sources,fate and transport of perfluorocarboxylates[J].Environ Sci Technol,2006,40(1):32-44.
[12]	魏嘉勋,陈文.全氟辛烷磺酸水样的前处理技术及固相微萃取剂的研究进展[J].化学通报(印刷版),2022,85(3):331-340,296.
[13]	PULSTER E L,WICHTERMAN A E,SNYDER S M,et al.Detection of long chain per- and polyfluoroalkyl substances (PFAS) in the benthic Golden tilefish (Lopholatilus chamaeleonticeps) and their association with microscopic hepatic changes[J].Science of the Total Environment,2022,809:151143.
[14]	KABORE H A,GOEURY K,DESROSIERS M,et al.Novel and legacy per- and polyfluoroalkyl substances (PFAS) in freshwater sporting fish from background and firefighting foam impacted ecosystems in Eastern Canada[J].The Science of the total environment,2022,816:151563.
[15]	RUDEL H,RADERMACHER G,FLIEDNER A,et al.Tissue concentrations of per- and polyfluoroalkyl substances (PFAS) in German freshwater fish:Derivation of fillet-to-whole fish conversion factors and assessment of potential risks[J].Chemosphere,2022,292:133483.
[16]	DALE K,YADETIE F,HORVLI T,et al.Single PFAS and PFAS mixtures affect nuclear receptor- and oxidative stress-related pathways in precision-cut liver slices of Atlantic cod (Gadus morhua)[J].Science of the Total Environment,2022,814:152732.
[17]	WILSON T B,STEVENSON G,CROUGH R,et al.Evaluation of residues in hen eggs after exposure of laying hens to water containing per- and polyfluoroalkyl substances[J].Environmental Toxicology and Chemistry,2021,40(3):735-743.
[18]	BEALE D J,NILSSON S,BOSE U,et al.Bioaccumulation and impact of maternal PFAS offloading on egg biochemistry from wild-caught freshwater turtles (Emydura macquarii macquarii)[J].The Science of the Total Environment,2022,817:153019.
[19]	CHEN C L,LU Y L,ZHANG X,et al.A review of spatial and temporal assessment of PFOS and PFOA contamination in China[J].Chemistry and Ecology,2009,25(3):163-177.
[20]	SONG X,VESTERGREN R,SHI Y,et al.Emissions,transport,and fate of emerging per- and polyfluoroalkyl substances from one of the major fluoropolymer manufacturing facilities in China[J].Environmental Science & Technology,2018,52(17):9694-9703.
[21]	中华人民共和国生态环境部.关于禁止生产、流通、使用和进出口林丹等持久性有机污染物的公告.(2019-02-14)[2020-05-15].https://www.mee.gov.cn/xxgk2018/xxgk/xxgk01/201903/t20190312_695462.html.
[22]	GIESY J P,KANNAN K.Perfluorochemical surfactants in the environment[J].Environ Sci Technol,2002,36(7):146-152.
[23]	LUO Y R.Comprehensive Handbook of Chemical Bond Energies[M].2007.
[24]	KRAFFT M P,RIESS J G.Per- and polyfluorinated substances (PFASs):environmental challenges[J].Current Opinion in Colloid & Interface Science,2015,20(3):192-212.
[25]	PAN Y T,ZHANG H X,CUI Q Q,et al.Worldwide distribution of novel perfluoroether carboxylic and sulfonic acids in surface water[J].Environmental Science & Technology,2018,52(14):7621-7629.
[26]	TANG J X,ZHU Y L,XIANG B,et al.Multiple pollutants in groundwater near an abandoned Chinese fluorine chemical park:concentrations,correlations and health risk assessments[J].Scientific Reports,2022,12(1):3370.
[27]	O'CONNOR J,MICKAN B S,SIDDIQUE K H M,et al.Physical,chemical,and microbial contaminants in food waste management for soil application:a review[J].Environmental Pollution,2022,300:118860.
[28]	LIU Y,MENDOZA-PERILLA P,CLAVIER K A,et al.Municipal solid waste incineration (MSWI) ash co-disposal:influence on per- and polyfluoroalkyl substances (PFAS) concentration in landfill leachate[J].Waste Management (New York,N.Y.),2022,144:49-56.
[29]	ROHLER K,HALUSKA A A,SUSSET B,et al.Long-term behavior of PFAS in contaminated agricultural soils in Germany[J].Journal of Contaminant Hydrology,2021,241:1:10.
[30]	陆宏,周锦阳,杨帆,等.基于Meta分析的全氟化合物对鱼类生态毒性效应[J/OL].环境科学:1-16.[2022-07-27 ].
[31]	LENKA S P,KAH M,PADHYE L P.Occurrence and fate of poly- and perfluoroalkyl substances (PFAS) in urban waters of New Zealand[J].Journal of Hazardous Materials,2022,428:128257.
[32]	HEARON S E,ORR A A,MOYER H,et al.Montmorillonite clay-based sorbents decrease the bioavailability of per-and polyfluoroalkyl substances (PFAS) from soil and their translocation to plants[J].Environmental Research,2022,205:112433.
[33]	何强,颜正,智悦,等.植物对全(多)氟烷基化合物(PFAS)的生物富集机制研究进展[J].中国环境科学,2022,42(11):5395-5407.
[34]	JOHNSON G R.PFAS in soil and groundwater following historical land application of biosolids[J].Water Research,2022,211:118035.
[35]	BOLAN N,SARKAR B,VITHANAGE M,et al.Distribution,behaviour,bioavailability and remediation of poly- and per-fluoroalkyl substances (PFAS) in solid biowastes and biowaste-treated soil[J].Environment International,2021,155:106600.
[36]	WANG P,ZHANG M,LI Q F,et al.Atmospheric diffusion of perfluoroalkyl acids emitted from fluorochemical industry and its associated health risks[J].Environment International,2021,146:106247.
[37]	SHOEIB M,HARNER T,VLAHOS P.Perfluorinated Chemicals in the Arctic Atmosphere[J].Environmental Science &Technology,2006,40(24):7577-7583.
[38]	WANG X P,HALSALL C,CODLING G,et al.Accumulation of perfluoroalkyl compounds in tibetan mountain snow:temporal patterns from 1980 to 2010[J].Environmental Science & Technology,2014,48(1):173-181.
[39]	MURAKAMI M,SATO N,ANEGAWA A,et al.Multiple evaluations of the removal of pollutants in road runoff by soil infiltration[J].Water Research,2008,42(10/11):2745-2755.
[40]	LINDSTROM A B,STRYNAR M J,LIBELO E L.Polyfluorinated compounds:past,present,and future[J].Environmental Science &Technology,2011,45(19):7954-7961.
[41]	罗佳璐,邵兵,刘嘉颖.全氟/多氟烷基化合物的毒理学研究进展及新型替代物健康危害[J].食品安全质量检测学报,2022,13(18):5983-5991.
[42]	YU N Y,WANG X X,ZHANG B B,et al.Distribution of perfluorooctane sulfonate isomers and predicted risk of thyroid hormonal perturbation in drinking water[J].Water Research,2015,76:171-180.
[43]	熊围,倪梦梅,包汇慧,等.全氟辛酸和全氟辛烷磺酸的致癌性证据及机制研究进展[J].卫生研究,2022,51(2):336-341.
[44]	LEHMLER H J.Synthesis of environmentally relevant fluorinated surfactants:a review[J].Chemosphere,2005,58(11):1471-1496.
[45]	郝丽丽,张磊,宁钧宇,等.PFOS与PFOA的毒性效应及其在我国普通人群中的内暴露研究进展[J].中国食品卫生杂志,2022,34(5):1112-1121.
[46]	OLSEN G W,HANSEN K J,STEVENSON L A,et al.Human donor liver and serum concentrations of perfluorooctanesulfonate and other perfluorochemicals[J].Environmental Science &Technology,2003,37(5):888-891.
[47]	BEESOON S,MARTIN J W.Isomer-specific binding affinity of perfluorooctanesulfonate (PFOS) and perfluorooctanoate (PFOA) to serum proteins[J].Environmental Science &Technology,2015,49(9):5722-5731.
[48]	HARADA K H,HASHIDA S,KANEKO T,et al.Biliary excretion and cerebrospinal fluid partition of perfluorooctanoate and perfluorooctane sulfonate in humans[J].Environmental Toxicology and Pharmacology,2007,24(2):134-139.
[49]	LAU C,ANITOLE K,HODES C,et al.Perfluoroalkyl acids:a review of monitoring and toxicological findings[J].Toxicological Sciences,2007,99(2):366-394.
[50]	OLSEN G W,BURRIS J M,EHRESMAN D J,et al.Half-life of serum elimination of perfluorooctanesulfonate,perfluorohexanesulfonate,and perfluorooctanoate in retired fluorochemical production workers[J].Environmental Health Perspectives,2007,115(9):1298-1305.
[51]	YU N Y,WANG X X,ZHANG B B,et al.Distribution of perfluorooctane sulfonate isomers and predicted risk of thyroid hormonal perturbation in drinking water[J].Water Research,2015,76:171-180.
[52]	ALVES R N,MAULVAULT A L,BARBOSA V L,et al.Preliminary assessment on the bioaccessibility of contaminants of emerging concern in raw and cooked seafood[J].Food and Chemical Toxicology,2017,104:69-78.
[53]	QI X,ZHOU J,WANG M,et al.Perfluorinated compounds in poultry products from the Yangtze River Delta and Pearl River Delta regions in China[J].Science of the Total Environment,2019,689:1079-1086.
[54]	TORRES F B M,GUIDA Y,WEBER R,et al.Brazilian overview of per- and polyfluoroalkyl substances listed as persistent organic pollutants in the stockholm convention[J].Chemosphere,2022,291:132674.
[55]	陈绍良,成红燕,陈北洋,等.全氟和多氟烷基物质对健康、生态的影响和处理技术展望[J].华电技术,2021,43(12):1-9.
[56]	HÖLZER J,MIDASCH O,RAUCHFUSS K,et al.Biomonitoring of perfluorinated compounds in children and adults exposed to perfluorooctanoate-contaminated drinking water[J].Environmental Health Perspectives,2008,116(5):651-657.
[57]	王广胤,孙伟强,马新壮,等.芦丁对全氟辛酸所致的小鼠脂代谢紊乱及肾脏损伤的改善作用[J].广西医学,2022,44(17):1998-2002.
[58]	CUI L,LIAO C Y,ZHOU Q F,et al.Excretion of PFOA and PFOS in Male Rats During a Subchronic Exposure[J].Archives of Environmental Contamination and Toxicology,2010,58(1):205-213.
[59]	LIU Z Y,LU Y L,WANG P,et al.Pollution pathways and release estimation of perfluorooctane sulfonate (PFOS) and perfluorooctanoic acid (PFOA) in central and eastern China[J].Science of the Total Environment,2017,580:1247-1256.
[60]	GHISI R,VAMERALI T,MANZETTI S.Accumulation of perfluorinated alkyl substances (PFAS) in agricultural plants:a review[J].Environmental Research,2019,169:326-341.
[61]	BRUSSEAU M L,ANDERSON R H,GUO B.PFAS concentrations in soils:Background levels versus contaminated sites[J].Science of the Total Environment,2020,740:140017.
[62]	吕雪艳,李政宇,杜文超,等.萝卜对土中全氟辛酸赋存形态影响及吸收特征[J].农业环境科学学报,2022,41(3):464-471.
[63]	胡涛英,黄芳,周珊珊,等.光谱法联合分子对接和等温滴定微量热法研究全氟壬酸与人血清白蛋白的相互作用(英文)[J].光谱学与光谱分析,2016,36(12):4141-4147.
[64]	QIN P F,LIU R T,PAN X R,et al.Impact of carbon chain length on binding of perfluoroalkyl acids to bovine serum albumin determined by spectroscopic methods[J].Journal of Agricultural and Food ChemistrY,2010,58(9):5561-5567.
[65]	OHMORI K,KUDO N,KATAYAMA K,et al.Comparison of the toxicokinetics between perfluorocarboxylic acids with different carbon chain length[J].Toxicology,2003,184(2/3):135-140.
[66]	JENSEN T K,ANDERSEN L B,KYHL H B,et al.Association between perfluorinated compound exposure and miscarriage in danish pregnant women[J].PLoS One,2015,10(4):e0123496.
[67]	MAMSEN L S,JÖNSSON B A G,LINDH C H,et al.Concentration of perfluorinated compounds and cotinine in human foetal organs,placenta,and maternal plasma[J].Science of the Total Environment,2017,596/597:97-105.
[68]	FANG X,GAO G,XUE H,et al.Exposure of perfluorononanoic acid suppresses the hepatic insulin signal pathway and increases serum glucose in rats[J].Toxicology,2012,294(2):109-115.
[69]	PETRO E M L,D’HOLLANDER W,COVACI A,et al.Perfluoroalkyl acid contamination of follicular fluid and its consequence for in vitro oocyte developmental competence[J].Science of the Total Environment,2014,496:282-288.
[70]	PFOHL M,MARQUES E,AUCLAIR A,et al.An’omics approach to unraveling the paradoxical effect of diet on perfluorooctanesulfonic acid (PFOS) and perfluorononanoic acid (PFNA)-induced hepatic steatosis[J].Toxicological Sciences,2021,180(2):277-294.
[71]	Initial indicative list of perfluorohexane sulfonic acid (PFHxS),its salts and PFHxS-related compounds[R/OL].[2019-10-15].https://www.mee.gov.cn/ywgz/gtfwyhxpgl/gnlygz/dtdt/202203/W020220305457959661771.pdf.
[72]	中华人民共和国生态环境部.关于公开征集《关于持久性有机污染物的斯德哥尔摩公约》全氟己烷磺酸、其盐类及其相关化合物修正案提案有关信息的通知[R/OL].[2022-03-05].https://www.mee.gov.cn/ywgz/gtfwyhxpgl/gnlygz/dtdt/202203/t20220305_970686.shtml.
[73]	LI Y,FLETCHER T,MUCS D,et al.Half-lives of PFOS,PFHxS and PFOA after end of exposure to contaminated drinking water[J].Occupational and Environmental Medicine,2018,75(1):46.
[74]	HE X,JIANG J,ZHANG X X.Environmental exposure to low-dose perfluorohexanesulfonate promotes obesity and non-alcoholic fatty liver disease in mice fed a high-fat diet[J].Environmental Science and Pollution Research,2022,29(32):49279-49290.
[75]	XU M M,LEGRADI J,LEONARDS P.Using comprehensive lipid profiling to study effects of PFHxS during different stages of early zebrafish development[J].Science of the Total Environment,2022,808:151739.
[76]	MARTÍNEZ-QUEZADA R,GONZÁLEZ-CASTAÑEDA G,BAHENA I,et al.Effect of perfluorohexane sulfonate on pig oocyte maturation,gap-junctional intercellular communication,mitochondrial membrane potential and DNA damage in cumulus cells in vitro[J].Toxicology in Vitro,2021,70:105011.
[77]	ZHANG S Y,TAN R R,PAN R,et al.Association of perfluoroalkyl and polyfluoroalkyl substances with premature ovarian insufficiency in chinese women[J].The Journal of Clinical Endocrinology &Metabolism,2018,103(7):2543-2551.
[78]	JIN R,MCCONNELL R,CATHERINE C,et al.Perfluoroalkyl substances and severity of nonalcoholic fatty liver in Children:an untargeted metabolomics approach[J].Environment International,2020,134:105220.
[79]	MATILLA-SANTANDER N,VALVI D,LOPEZ-ESPINOSA M-J,et al.Exposure to perfluoroalkyl substances and metabolic outcomes in pregnant women:evidence from the spanish INMA birth cohorts[J].Environmental Health Perspectives,2017,125(11):117004.
[80]	RAMHøJ L,HASS U,BOBERG J,et al.Perfluorohexane sulfonate (PFHxS) and a mixture of endocrine disrupters reduce thyroxine levels and cause antiandrogenic effects in rats[J].Toxicological Sciences,2018,163(2):579-591.
[81]	CUI Q Q,PAN Y T,ZHANG H X,et al.Elevated concentrations of perfluorohexanesulfonate and other per- and polyfluoroalkyl substances in Baiyangdian Lake (China):source characterization and exposure assessment[J].Environmental Pollution,2018,241:684-691.
[82]	OLIVERO-VERBEL J,TAO L,JOHNSON-RESTREPO B,et al.Perfluorooctanesulfonate and related fluorochemicals in biological samples from the north coast of Colombia[J].Environmental Pollution,2006,142(2):367-372.
[83]	方程,张红平,罗云龙.全氟和多氟烷基化合物的分析检测[J].分析科学学报,2021,37(4):451-458.
[84]	PAULETTO P S,BANDOSZ T J.Activated carbon versus metal-organic frameworks:a review of their PFAS adsorption performance[J].Journal of Hazardous Materials,2022,425:127810.
[85]	VU C T,WU T.Recent progress in adsorptive removal of per- and poly-fluoroalkyl substances (PFAS) from water/wastewater[J].Critical Reviews in Environmental Science and Technology,2020,52(1):90-129.
[86]	O’CONNOR J,BOLAN N S,KUMAR M,et al.Distribution,transformation and remediation of poly- and per-fluoroalkyl substances (PFAS) in wastewater sources[J].Process Safety and Environmental Protection,2022,164:91-108.
[87]	GARG S,WANG J,KUMAR P,et al.Remediation of water from per-/poly-fluoroalkyl substances (PFAS)-Challenges and perspectives[J].Journal of Environmental Chemical Engineering,2021,9(4):105784.
[88]	XU B T,LIU S,ZHOU J L,et al.PFAS and their substitutes in groundwater:occurrence,transformation and remediation[J].Journal of Hazardous Materials,2021,412:125159.
[89]	MASTROPIETRO T F,BRUNO R,PARDO E,et al.Reverse osmosis and nanofiltration membranes for highly efficient PFASs removal:overview,challenges and future perspectives[J].Dalton Transactions,2021,50(16):5398-5410.
[90]	WANNINAYAKE D M.Comparison of currently available PFAS remediation technologies in water:a review[J].Journal of Environmental Management,2021,283:111977.
[91]	KIM T H,LEE S H,KIM H Y,et al.Decomposition of perfluorooctane sulfonate (PFOS) using a hybrid process with electron beam and chemical oxidants[J].Chemical Engineering Journal,2019,361:1363-1370.
[92]	MERINO N,QU Y,DEEB R A,et al.Degradation and removal methods for perfluoroalkyl and polyfluoroalkyl substances in water[J].Environmental Engineering Science,2016,33(9):615-649.
[93]	HORI H,NAGAOKA Y,MURAYAMA M,et al.Efficient decomposition of perfluorocarboxylic acids and alternative fluorochemical surfactants in hot water[J].Environmental Science &Technology,2008,42(19):7438-7443.
[94]	AHMED M B,ALAM M M,ZHOU J L,et al.Advanced treatment technologies efficacies and mechanism of per- and poly-fluoroalkyl substances removal from water[J].Process Safety and Environmental Protection,2020,136:1-14.
[95]	TIMSHINA A,ARISTIZABAL-HENAO J J,da SILVA B F,et al.The last straw:characterization of per- and polyfluoroalkyl substances in commercially-available plant-based drinking straws[J].Chemosphere,2021,277:130238.
[96]	朱翔,汪宣,徐文君,等.包装印刷材料全氟烷基化合物检测方法研究[J].绿色包装,2022(9):26-31.
[97]	BENOTTI M J,FERNANDEZ L A,PEASLEE G F,et al.A forensic approach for distinguishing PFAS materials[J].Environmental Forensics,2020,21(3/4):319-333.
[98]	王振聚,罗忻,梁生康,等.高分辨质谱技术在全氟多氟化合物分析中的应用研究进展[J].分析测试学报,2022,41(6):931-940.
[99]	VON ABERCRON E,FALK S,STAHL T,et al.Determination of adsorbable organically bound fluorine (AOF) and adsorbable organically bound halogens as sum parameters in aqueous environmental samples using combustion ion chromatography (CIC)[J].Science of the Total Environment,2019,673:384-391.
[100]	FANG C,CHEN Z,MEGHARAJ M,et al.Potentiometric detection of AFFFs based on MIP[J].Environmental Technology & Innovation,2016,5:52-59.
[101]	WALLACE S,LAMBRAKOS S G,SHABAEV A,et al.On using DFT to construct an IR spectrum database for PFAS molecules[J].Structural Chemistry,2022,33(1):247-256.
[102]	FANG C,MEGHARAJ M,NAIDU R.Surface-enhanced Raman scattering (SERS) detection of fluorosurfactants in firefighting foams[J].RSC Advances,2016,6(14):11140-11145.
[103]	FANG C,ZHANG X,DONG Z M,et al.Smartphone app-based/portable sensor for the detection of fluoro-surfactant PFOA[J].Chemosphere,2018,191:381-388.
[104]	MCDONOUGH C A,LI W,BISCHEL H N,et al.Widening the lens on PFASs:direct human exposure to perfluoroalkyl acid precursors (pre-PFAAs)[J].Environmental Science & Technology,2022:6004-6013.
[105]	WANG Y,CHANG W G,WANG L,et al.A review of sources,multimedia distribution and health risks of novel fluorinated alternatives[J].Ecotoxicology and Environmental Safety,2019,182:109402.
[106]	COGGAN T L,ANUMOL T,PYKE J,et al.A single analytical method for the determination of 53 legacy and emerging per- and polyfluoroalkyl substances (PFAS) in aqueous matrices[J].Analytical and Bioanalytical Chemistry,2019,411(16):3507-3520.
[107]	CHEN L,DAI Y Y,ZHOU C,et al.Robust matrix effect-free method for simultaneous determination of legacy and emerging per- and polyfluoroalkyl substances in crop and soil matrices[J].Journal of Agricultural and Food Chemistry,2020,68(30):8026-8039.
[108]	杨愿愿,李偲琳,赵建亮,等.超高效液相色谱-串联质谱法同时测定水、沉积物和生物样品中57种全/多氟化合物[J].分析化学,2022,50(8):1243-1251.