STUDY ON HUMAN HEALTH AND WATER QUALITY CRITERIA OF ARSENIC IN TIELING SECTION OF LIAOHE RIVER
-
摘要: 砷(As)是一种持久性、毒性强的致癌污染物。近年来我国As污染事件频发,故制定As的人体健康水质基准具有重要意义。以辽河铁岭段为研究对象,采集并分析水样和不同营养级的鱼样中As含量。结合文献调研,确定As的污染物毒性参数与辽河铁岭段饮水相关的部分人群暴露参数;基于线上问卷调查,计算本地居民人均第2、3、4营养级鱼类摄入量分别为0.0268,0.0323,0.0027 kg/d,进而推导出当地代表性鱼类As的第2、3、4营养级国家生物累积因子为8.256,9.281,10.197 L/kg。根据以上参数计算出辽河铁岭段As的人体健康水质基准值为1.976×10-5 mg/L,研究结果可为辽河流域制定水质标准提供参考,为更加科学有效地管控污染物排放和保护人体健康提供依据。Abstract: Arsenic is a persistent and toxic carcinogen pollutant.In recent years,arsenic pollution incidents occur frequently in China.It is of great significance to establish human health water quality criteria for arsenic in China.Taking the Tieling Section of Liaohe River as the research object,the content of arsenic in water samples and fish samples of different nutritional levels were collected and analyzed.Combined with literature research,the toxicity parameters of arsenic pollutants and the exposure parameters of some people related to drinking water in the Tieling Section of Liaohe River were determined.Through the online questionnaire survey,it was calculated that the per capita fish intake of the second,third,and fourth nutritional levels of local residents was 0.0268,0.0323,and 0.0027 kg/d.Then it was derived that the second,third,and fourth trophic national bioaccumulation factors were 8.256,9.281,and 10.197 L/kg of local representative fishes.According to the above parameters,it was calculated that the reference value of human health water quality criteria of arsenic in the Tieling Section of Liaohe River was 1.976×10-5 mg/L,which provided a reference for the formulation of water quality standards in Liaohe River Basin,and a basis for scientific and effective pollution control and protection of human health.
-
[1] United States Environmental Protection Agency Office of Water. Methodology for deriving ambient water quality criteria for the protection of human health (2000)[R]. U.S. Environmental Protection Agency Washington, 2000, DC 20460. [2] European Communities. No.27 technical guidance for deriving environmental quality standards[R]. Common Implementation Strategy for the Water Framework Directive (2000/60/EC), 2011. [3] ORGANIZATION W H. Guidelines for drinking-water quality fourth edition[M]. Paris:World Health Organization, 2011. [4] Canadian Council of Ministers of the Environment. Summary of a protocol for the derivation of environmental and human health soil quality guidelines (CCME 2006)[R]. Canadian Council of Ministers of the Environment, 2006. [5] 金银龙,梁超轲,何公理,等.中国地方性砷中毒分布调查(总报告)[J].卫生研究,2003,32(6):519-540. [6] 张娟,闫振广,高富,等.不同形态的砷水生生物基准探讨及在辽河流域的初步应用[J].环境科学学报,2015,35(4):1164-1173. [7] 杨晶.铁岭市控制单元水生态系统健康评价[J].黑龙江农业科学,2017(7):28-30. [8] 环境保护部.人体健康水质基准制定技术指南:HJ 837-2017[S].北京:环境保护部,2017. [9] 段小丽.中国人群暴露参数手册(成人卷)[M].北京:中国环境出版社,2013. [10] 陈金,王晓南,李霁,等.太湖流域双酚AF和双酚S人体健康水质基准的研究[J].环境科学学报,2019,39(8):2764-2770. [11] 王晓南,崔亮,李霁,等.人体健康水质基准特征参数研究及应用[J].环境科学研究,2021,34(7):1553-1561. [12] 丁蕊,陈景文,于洋,等.基于集成学习算法构建有机化学品鱼体生物富集因子的QSAR预测模型[J].环境化学,2021,40(5):1295-1304. [13] 《2019中国渔业统计年鉴》[M].北京:中国农业出版社,2019. [14] 国家卫生和计划生育委员会.食品安全国家标准食品中总砷及无机砷的测定:GB 5009.11-2014[S].北京:国家卫生和计划生育委员会,2015. [15] 李佳凡.上海市黄浦江重金属和典型新兴污染物的健康风险评价及水质基准研究[D].上海:上海交通大学,2019. [16] United States Environmental Protection Agency Office of Water. National recommended water quality criteria[R]. Washington, DC 20210, 2012. [17] 杨晓云,温勇,陈晓燕,等.重金属在北江鱼类和底栖动物体内的富集及污染评价[J].环境科学与技术,2010,33(6):194-198. [18] 周淑婷,罗莹华,胡金妹,等.韶关北江河水质重金属污染调查与评价[J].安徽农业科学,2015,43(3):277-279. [19] 汪晓静,刁飞燕,张静,等.济南市售食用鱼铅、镉、砷含量调查及污染状况评价[J].山东大学学报(医学版),2011,49(5):153-155. [20] 潘恒健.小清河济南段水质主因子分析[J].济南大学学报(自然科学版),2008,22(1):107-109. [21] 纪登云,郭少为,张晓枫,等.石墨炉原子吸收法测定鱼中砷[J].光谱学与光谱分析,1992,(5):101-102,100. [22] 曹文杰.基于人体健康的湘江砷、铅水质基准研究[D].湘潭:湘潭大学,2016. [23] 余杨.三峡水库蓄水初期鱼类中重金属污染研究[D].北京:中国水利水电科学研究院,2013. [24] 徐青.重金属污染在不同水体淡水鱼中的分布特征及健康风险评估[D].上海:上海大学,2013. [25] 夏青.水质标准手册[M].北京:中国环境科学出版社,1990. [26] 国家环境保护总局科技标准司.地表水环境质量标准:GB 3838-2002[S].北京:中国标准出版社,2002. [27] 中华人民共和国卫生部中国国家标准化管理委员会.生活饮用水卫生标准:GB 5749-2006[S].北京:中国标准出版社,2006. [28] 苏海磊,李信茹,陶艳茹,等.美国水质标准制定研究及其对中国的借鉴意义[J].生态环境学报,2021,30(11):2267-2274. [29] 何珊,郭渊,王琛,等.镍的环境生物地球化学与毒性效应研究进展[J].中国环境科学,2022,46(5):2239-2351.
点击查看大图
计量
- 文章访问数: 110
- HTML全文浏览量: 22
- PDF下载量: 2
- 被引次数: 0