MIXED SORPTION OF THREE AQUEOUS SULFONAMIDES ONTO THE BIOCHAR DERIVED FROM POPLAR WOOD CHIPS

ZHOU Jun; LI Yan; GUAN Yi-dong; HUANG Li-dong; JIN Hong-mei; XIAO Qiong; SONG Jiang-sheng

doi:10.13205/j.hjgc.202103001

Volume 39 Issue 3

Jul. 2021

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ZHOU Jun, LI Yan, GUAN Yi-dong, HUANG Li-dong, JIN Hong-mei, XIAO Qiong, SONG Jiang-sheng. MIXED SORPTION OF THREE AQUEOUS SULFONAMIDES ONTO THE BIOCHAR DERIVED FROM POPLAR WOOD CHIPS[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(3): 1-6,13. doi: 10.13205/j.hjgc.202103001

Citation:

ZHOU Jun, LI Yan, GUAN Yi-dong, HUANG Li-dong, JIN Hong-mei, XIAO Qiong, SONG Jiang-sheng. MIXED SORPTION OF THREE AQUEOUS SULFONAMIDES ONTO THE BIOCHAR DERIVED FROM POPLAR WOOD CHIPS[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(3): 1-6,13. doi: 10.13205/j.hjgc.202103001

Citation:

ZHOU Jun, LI Yan, GUAN Yi-dong, HUANG Li-dong, JIN Hong-mei, XIAO Qiong, SONG Jiang-sheng. MIXED SORPTION OF THREE AQUEOUS SULFONAMIDES ONTO THE BIOCHAR DERIVED FROM POPLAR WOOD CHIPS[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(3): 1-6,13. doi: 10.13205/j.hjgc.202103001

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MIXED SORPTION OF THREE AQUEOUS SULFONAMIDES ONTO THE BIOCHAR DERIVED FROM POPLAR WOOD CHIPS

doi: 10.13205/j.hjgc.202103001

1. Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China;
2. Key Laboratory of Environment Remediation and Ecological Health, Ministry of Education, College of Environmental & Resource Sciences, Zhejiang University, Hangzhou 310058, China;
3. College of Applied Meteorology, Nanjing University of Information Science & Technology, Nanjing 210044, China;
4. Circular Agriculture Research Center, Jiangsu Academy of Agricultural Sciences, Nanjing 210014, China

Received Date: 2020-04-20
Available Online: 2021-07-19

Abstract

Abstract

Discharge of sulfonamides (SAs) poses seriously potential ecological risk on the aquatic environment. In this paper, the biochar derived from poplar wood chips (PWCs) was produced under three pyrolysis temperatures to investigate the sorption mechanism of SAs in the aqueous solution. The experiment result showed that the pore channel of BC350 and BC500-BC650 was dominated by the macropores and mesopores, respectively. The increase of pyrolysis temperature enhanced the polycyclic aromatic surface of the biochars. The pseudo-secondary-order kinetic model and the Freundlich model could be applied to describe the kinetics and isothermal process of biochar sorption, respectively. The maximum sorption capacity of SAs of BC650 was about 2.6 to 104 times on herb-residue biochars. Based on the calculation of thermodynamics, the sorption of PWC involved the physical and chemical sorption simultaneously, but dominated by chemical sorption. The sorption affinity of three SAs was in the descending order of SPD>SMZ>SDZ, thanked to the support from their molecular morphology analysis.
- biochar,
- sulfonamide,
- sorption,
- thermodynamics

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References(31)

References

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