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Volume 39 Issue 4
Jul.  2021
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Article Navigation >  ENVIRONMENTAL ENGINEERING  > 2021  >  39(4): 50-56,106
WU Meng-yi, LONG Xin, GAO Cong-hao, QIN Xiao, CHEN Yue, TANG Yu-lin. FABRICATION OF CARBON NANOTUBE-DOPED PbO2 COMPOSITE ELECTRODE AND MECHANISM OF CATALYTIC OXIDATION OF BISPHENOL A[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(4): 50-56,106. doi: 10.13205/j.hjgc.202104009
Citation: WU Meng-yi, LONG Xin, GAO Cong-hao, QIN Xiao, CHEN Yue, TANG Yu-lin. FABRICATION OF CARBON NANOTUBE-DOPED PbO2 COMPOSITE ELECTRODE AND MECHANISM OF CATALYTIC OXIDATION OF BISPHENOL A[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(4): 50-56,106. doi: 10.13205/j.hjgc.202104009
shu

FABRICATION OF CARBON NANOTUBE-DOPED PbO2 COMPOSITE ELECTRODE AND MECHANISM OF CATALYTIC OXIDATION OF BISPHENOL A

doi: 10.13205/j.hjgc.202104009

  • 1. State Key Laboratory of Pollution Control and Resource Reuse, College of Environmental Science and Engineering, Tongji University, Shanghai 200092, China;

  • 2. National Engineering Research Center for Urban Pollution Control, Tongji University, Shanghai 200092, China;

  • 3. Hebei Construction Group Installation Engineering Co., Ltd, Baoding 071000, China

  • Received Date: 2020-03-16
    Available Online: 2021-07-21
    Abstract
  • CNT-PbO2 composite electrodes with high stability and catalytic activity were obtained by doping carbon nanotubes (CNTs) with different concentrations into PbO2 electrodes by electrochemical deposition. Scanning electron microscopy (SEM), energy dispersive spectroscopy (EDS) analysis proved that CNTs were successfully doped into the PbO2 electrode surface active layer, leading to a decline of PbO2 particle size and an increase of activity surface area. The amount of ·OH radicals generated in the degradation system of bisphenol A (BPA) by CNT-PbO2 electrodes decreased. However, the degradation effect was improved. Cyclic voltammetry (CV) curves and the accelerated life test indicated that the degradation mechanism of BPA was mainly ascribed to the stronger electrochemical direct oxidation ability and higher stability of CNT-PbO2 composite electrodes. Finally, the dominant by-products were obtained, and plausible degradation pathway of BPA was proposed by UPLC & Q-TOF MS test.
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    • References(16)
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