Source Journal of CSCD
Source Journal for Chinese Scientific and Technical Papers
Core Journal of RCCSE
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Volume 39 Issue 11
Jan.  2022
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ZHANG Zhuo-ran, LIU Qing-hua, WANG Wei-gang, RONG Jing, CAO Rui-jie, LUO Wen-tao, LIU Chao, WANG Ya-yi. EFFECT OF PYROLYSIS TEMPERATURE ON THE PHYSICAL AND CHEMICAL CHARACTERISTICS OF BAMBOO-BASED BIOCHAR[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(11): 96-102,126. doi: 10.13205/j.hjgc.202111012
Citation: ZHANG Zhuo-ran, LIU Qing-hua, WANG Wei-gang, RONG Jing, CAO Rui-jie, LUO Wen-tao, LIU Chao, WANG Ya-yi. EFFECT OF PYROLYSIS TEMPERATURE ON THE PHYSICAL AND CHEMICAL CHARACTERISTICS OF BAMBOO-BASED BIOCHAR[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(11): 96-102,126. doi: 10.13205/j.hjgc.202111012

EFFECT OF PYROLYSIS TEMPERATURE ON THE PHYSICAL AND CHEMICAL CHARACTERISTICS OF BAMBOO-BASED BIOCHAR

doi: 10.13205/j.hjgc.202111012
  • Received Date: 2021-08-04
    Available Online: 2022-01-26
  • As a new environmental functional material, biochar showed application prospects in environmental pollution remediation, soil improvement, greenhouse gas emission reduction, and enhanced biological nitrogen removal from wastewater. Biochars were prepared from bamboo powder at different pyrolysis temperatures, and their electron exchange capacity, surface functional groups, and elemental composition were characterized to explore the effect of pyrolysis temperatures on the physicochemical characteristics of bamboo-based biochar. The results showed that while the pyrolysis temperature increased from 300℃ to 700℃, the electron donating capacity (EDC) of biochars generally increased first and then decreased. The highest EDC was obtained in the biochars prepared at 300℃ and 400℃ with the value of 0.33 e-/g Biochar and 0.35 e-/g Biochar, respectively, had higher potential in improving biological nitrogen removal; and the lowest EDC was obtained in the biochars prepared at 600℃ with the value of 0.07 e-/g Biochar. Accordingly, the average oxidation degree Cox calculated from the elemental content was corresponding to the results of EDC. With the increase of pyrolysis temperature, the Cox of biochars changed from negative to positive. When the pyrolysis temperature was 300℃ or 400℃, the Cox of the biochars was negative, indicating that the biochars was more reductive and less oxidizable than those prepared at 500~700℃, i.e., higher electron donating capacity (EDC) and lower electron accepting capacity (EAC). In addition, Fourier transform infrared spectroscopy showed that the hydroxyl content of the biochars was highest at 300℃ and 400℃, which was consistent with their highest EDC.
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  • [1]
    LEHMANN J, JOSEPH S. Biochar for Environmental Management:Science, Technology and Implementation[M]. Taylor and Francis, 2015.
    [2]
    MAHTAB A, et al. Biochar as a sorbent for contaminant management in soil and water:a review[J]. Chemosphere, 2014, 99:19-33.
    [3]
    刘玉学,刘微,吴伟祥,等.土壤生物质炭环境行为与环境效应[J].应用生态学报,2009,20(4):977-982.
    [4]
    张东升,江泽慧,任海青,等.竹炭微观构造形貌表征[J].竹子研究汇刊,2006(4):1-8.
    [5]
    CORNELISSEN G,GUSTAFSSON,BUCHELI T D,et al.Extensive sorption of organic compounds to black carbon,coal,and kerogen in sediments and soils:mechanisms and consequences for distribution,bioaccumulation,and biodegradation[J].Environmental Science & Technology,2005,39(18):6881-6895.
    [6]
    LIANG B,LEHMANN J,SOLOMON D,et al.Black carbon increase cation exchange capacity in soils[J].Soil Science Society of America Journal,2006,70(5):1719-1730.
    [7]
    DONG X L, MA L Q, LI Y C. Characteristics and mechanisms of hexavalent chromium removal by biochar from sugar beet tailing[J]. Journal of Hazardous Materials, 2011, 190(1/2/3):909-915.
    [8]
    XU X Y, HUANG H, ZHANG Y, et al. Biochar as both electron donor and electron shuttle for the reduction transformation of Cr(Ⅵ) during its sorption[J]. Environmental Pollution, 2019, 244:423-430.
    [9]
    KAPPLER A, WUESTNER M L, RUECKER A, et al. Biochar as an electron shuttle between bacteria and Fe(Ⅲ) minerals[J]. Environmental Science & Technology Letters, 2014, 1(8):339-344.
    [10]
    QIAN L B, SHANG X, ZHANG B, et al. Enhanced removal of Cr(Ⅵ) by silicon rich biochar-supported nanoscale zero-valent iron[J]. Chemosphere, 2019, 215:739-745.
    [11]
    OH S, SEO Y, RYU K. Reductive removal of 2,4-dinitrotoluene and 2,4-dichlorophenol with zero-valent iron-included biochar[J]. Bioresource Technology, 2016, 216:1014-1021.
    [12]
    AHMED A, KURIAN J, RAGHAVAN V. Biochar influences on agricultural soils, crop production, and the environment:a review[J]. Environmental Reviews, 2016, 24(4):495-502.
    [13]
    KONG L L, GAO Y Y, ZHOU Q X, et al. Biochar accelerates PAHs biodegradation in petroleum-polluted soil by biostimulation strategy[J]. Journal of Hazardous Materials, 2018, 343:276-284.
    [14]
    VITHANAGE M, HERATH I, ALMAROAI Y A, et al. Effects of carbon nanotube and biochar on bioavailability of Pb, Cu and Sb in multi-metal contaminated soil[J]. Environmental Geochemistry and Health, 2018, 40(1):565.
    [15]
    Van der ZEE F R, CERVANTES F J. Impact and application of electron shuttles on the redox (bio)transformation of contaminants:a review[J]. Biotechnology Advances, 2009, 27(3):256-277.
    [16]
    FRANCISCO J, CHACÓN, et al. Understanding, measuring and tuning the electrochemical properties of biochar for environmental applications[J]. Reviews in Environmental Science and Bio/Technology, 2017, 16(4):695-715.
    [17]
    KLVPFEL LAURA, et al. Redox properties of plant biomass-derived black carbon (biochar)[J]. Environmental Science & Technology, 2014, 48(10):5601-5611.
    [18]
    CHEN S S, et al. Promoting interspecies electron transfer with biochar[J]. Scientific Reports, 2014, 4:5019.
    [19]
    ANTAL M J,GRONLI M.The art,science,and technology of charcoal production[J].Ind Eng Chem Res,2003,42(8):1619-1640.
    [20]
    LEHMANN J,JOSEPH S.Biochar for environmental management:science and technology[M].London:Earthscan,2009:1-29,107-157.
    [21]
    LEE J W,KIDDER M,EVANS B R.Characterization of biochars produced from cornstovers for soil amendment[J].Environmental Science & Technology,2010,44(20):7970-7974.
    [22]
    HOSSAIN M K,STREZOV V,CHAN K Y,et al.Influence of pyrolysis temperature on production and nutrient properties of wastewater sludge biochar[J].Journal of Environmental Management,2011,92(1):223-228.
    [23]
    CAO X D,HARRIS W.Properties of dairy-manure-derived biochar pertinent to its potential use in remediation[J].Bioresource Technology,2010,101(14):5222-5228.
    [24]
    SARAN S,ELISA L C,EVELYN K,et al.Biochar,climate change and soil:a review to guide future research[R].CSIRO Land and WaterScience Report,2009:5-6.
    [25]
    KUPPUSAMY S, YI L, EDMOND S. Electrochemical behavior of biochar and its effects on microbial nitrate reduction:role of extracellular polymeric substances in extracellular electron transfer[J]. Chemical Engineering Journal, 2020, 395:125077.
    [26]
    XU J J, WU X H, ZHU N W et al. Anammox process dosed with biochars for enhanced nitrogen removal:role of surface functional groups[J]. Science of the Total Environment, 2020, 748:141367.
    [27]
    LIU D L, LI J, ZHANG S S, et al. Leaf spot disease of Orychophragmus violaceus caused by Alternaria tenuissima in China[J]. Plant Disease, 2021.
    [28]
    CHEN Y, HALLER C, LIU W, et al. GaN buffer growth temperature and efficiency of InGaN/GaN quantum wells:the critical role of nitrogen vacancies at the GaN surface[J]. Applied Physics Letters, 2021, 118(11):.
    [29]
    MUTHANNA J. Ahmed and SAMAR K. Theydan. Physical and chemical characteristics of activated carbon prepared by pyrolysis of chemically treated date stones and its ability to adsorb organics[J]. Powder Technology, 2012, 229:237-245.
    [30]
    CHUN Y, SHENG G Y, CHIOU C T, et al. Compositions and sorptive properties of crop residue-derived chars[J]. Environmental Science & Technology, 2004, 38(17):4649-4655.
    [31]
    NOVAK J M, CANTRELL K B, WATTS D W, et al. Designing relevant biochars as soil amendments using lignocellulosic-based and manure-based feedstocks[J]. Journal of Soils and Sediments, 2014, 14(2):330-343.
    [32]
    LI N, RAO F, HE L L, et al. Evaluation of biochar properties exposing to solar radiation:a promotion on surface activities[J]. Chemical Engineering Journal, 2020, 384:123353.
    [33]
    WANG G J, LI Q, DZAKPASU M, et al. Impacts of different biochar types on hydrogen production promotion during fermentative co-digestion of food wastes and dewatered sewage sludge[J]. Waste Management, 2018, 80:73-80.
    [34]
    PFAFFENEDER-KMEN M, CASAS I F, NAGHILOU A, et al. A multivariate curve resolution evaluation of an in-situ ATR-FTIR spectroscopy investigation of the electrochemical reduction of graphene oxide[J]. Electrochimica Acta, 2017, 255:160-167.
    [35]
    WU Z S, XU F, YANG C, et al. Highly efficient nitrate removal in a heterotrophic denitrification system amended with redox-active biochar:a molecular and electrochemical mechanism[J]. Bioresource Technology, 2019, 275:297-306.
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