Core Chinese Journal
Source Journal of CSCD(Core Version)
Source Journal for Chinese Scientific and Technical Papers
Core Journal of RCCSE
Included in JST China
Volume 40 Issue 1
Mar.  2022
Turn off MathJax
Article Contents
MA Yan, ZHANG Dading, ZHANG Fan, CHENG Lu, MA Yue, GUO Jianda. INFLUENTING FACTORS OF CHITOSAN-MODIFIED ZEOLITE AND ITS STABILIZATION EFFECT ON MULTI METAL CONTAMINATED SOIL[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(1): 94-101,116. doi: 10.13205/j.hjgc.202201014
Citation: MA Yan, ZHANG Dading, ZHANG Fan, CHENG Lu, MA Yue, GUO Jianda. INFLUENTING FACTORS OF CHITOSAN-MODIFIED ZEOLITE AND ITS STABILIZATION EFFECT ON MULTI METAL CONTAMINATED SOIL[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(1): 94-101,116. doi: 10.13205/j.hjgc.202201014

INFLUENTING FACTORS OF CHITOSAN-MODIFIED ZEOLITE AND ITS STABILIZATION EFFECT ON MULTI METAL CONTAMINATED SOIL

doi: 10.13205/j.hjgc.202201014
  • Received Date: 2021-05-08
    Available Online: 2022-03-30
  • Publish Date: 2022-03-30
  • In this study, Pb-, Zn-, and Cd-contaminated soil was stabilized by chitosan-modified zeolite. Scanning electron microscopy, X-ray photoelectron spectroscopy, X-ray diffraction, and toxicity characteristic leaching procedure extraction methods were used to analyze the composition of the modified materials and their stabilizing effect on multi-metal-contaminated soil. In addition, the effect of the modified material dosages, soil water content, and pH on the stabilization of the contaminated soil were investigated.Resultsshowed that the surface of the modified material had a clear fibrous structure and a uniform synaptic structure. The characteristic peak of N1 s was increased at a binding energy of approximately 400 eV, confirming that chitosan was loaded onto the surface of the zeolite and calcium silicate particles had a modifying effect. The stabilization effect reached its maximum when the maximum dosage was 10%. With the increase in water content, the leaching concentration increased slightly. Under different water content, the competition on Pb stabilization of Zn and Cd was not evident. When the soil environment was weakly acid-base or neutral, Zn and Cd showed no competitive advantage in Pb stabilization, but Zn and Cd had a stronger competitive advantage under strong acid or strong alkali environment, thereby inhibiting the stabilization of Pb. This study developed a novel and efficient soil stabilization material, providing a basis for the remediation of polymetallic contaminated sites.
  • loading
  • [1]
    DIACONU M,PAVEL L V,HLIHOR R,et al.Characterization of heavy metal toxicity in some plants and microorganisms:a preliminary approach for environmental bioremediation[J].New Biotechnology,2020,56:130-139.
    [2]
    LI Z Y,MA Z W,van der KUIJP T J,et al.A review of soil heavy metal pollution from mines in China:pollution and health risk assessment[J].Science of the Total Environment,2014,468/469:843-853.
    [3]
    APPEL C,MA L Q,RHUE R D,et al.Sequential sorption of lead and cadmium in three tropical soils[J].Environmental Pollution,2007,155(1):132-140.
    [4]
    GOPALAPILLAI Y,HALE B.Internal versus external dose for describing ternary metal mixture (Ni,Cu,Cd) chronic toxicity to lemna minor[J].Environmental Science & Technology,2017,51(9):5233-5241.
    [5]
    WATERLOT C,BIDAR G,PELFRÊNE A,et al.Contamination,fractionation and availability of metals in urban soils in the vicinity of former lead and zinc smelters,france[J].Pedosphere,2013,23(2):143-159.
    [6]
    CHEN X,CUI J,XU X R,et al.Bacterial cellulose/attapulgite magnetic composites as an efficient adsorbent for heavy metal ions and dye treatment[J].Carbohydrate Polymers,2020,229:115512.
    [7]
    SABOLC P,JELENA R,SNEŽANA T,et al.Evaluation of the adsorption potential of eco-friendly activated carbon prepared from cherry kernels for the removal of Pb2+,Cd2+and Ni2+from aqueous wastes[J].Journal of environmental management,2016,184(Pt 2):297-306.
    [8]
    FERRI M,CAMPISI S,SCAVINI M,et al.In-depth study of the mechanism of heavy metal trapping on the surface of hydroxyapatite[J].Applied Surface Science,2019,475:397-409.
    [9]
    NIMIRCIAG R.Heavy metals in the soils of Rodna mining area,Romania and Zeolite efficiency for remediation[J].Environmental Engineering and Management Journal,2012,11(2):421-426.
    [10]
    李明遥,张妍,杜立宇,等.生物炭与沸石混施对土壤Cd形态转化的影响[J].水土保持学报,2014,28(3):248-252.
    [11]
    马玮艺,张彦峰,姜英男,等.不同改良剂对镉污染土壤的化学固定修复的比较研究[J].中国科技博览,2009,(32):136-137.
    [12]
    王永强,肖立中,李伯威,等.骨炭+沸石对重金属污染土壤的修复效果及评价[J].农业环境与发展,2010,27(3):90-93.
    [13]
    OSTROSKI I C,BARROS M,SILVA E A,et al.A comparative study for the ion exchange of Fe(Ⅲ)and Zn(Ⅱ)on zeolite NaY[J].Journal of Hazardous Materials,2009,161 (2/3):1404-1412.
    [14]
    XAVIER Q,ANDRÉS A,NATÀLIA M,et al.Immobilization of heavy metals in polluted soils by the addition of zeolitic material synthesized from coal fly ash[J].Chemosphere,2006,62(2):171-180.
    [15]
    HAMIDPOUR M,AFYUNI M,KALBASI M,et al.Mobility and plant-availability of Cd(Ⅱ)and Pb(Ⅱ)adsorbed on zeolite and bentonite[J].Applied Clay Science,2010,48(3):342-348.
    [16]
    TURAN N G,ELEVLI S,MESCI B.Adsorption of copper and zinc ions on illite:determination of the optimal conditions by the statistical design of experiments[J].Applied Clay Science,2011,52(4):392-399.
    [17]
    SANDHYA B,TONNI A K.Low-cost adsorbents for heavy metals uptake from contaminated water:a review[J].Journal of Hazardous Materials,2003,97(1):219-243.
    [18]
    KUMPIENE J,LAGERKVIST A,MAURICE C.Stabilization of As,Cr,Cu,Pb and Zn in soil using amendments:a review[J].Waste Management (New York,N.Y.),2006,28(1):215-225.
    [19]
    李晔,肖文浚,彭长琪.沸石改性及其对氨氮废水处理效果的研究[J].非金属矿,2003,26(2):53-55.
    [20]
    叶玲,张敬阳.蒙脱石的电动电位调控及其对重金属离子吸附性能的影响[J].矿物学报,2013,33(1):19-24.
    [21]
    PANNEERSELVAM P,THINAKARAN N,THIRUVENKATARAVI KV,et al.Phosphoric acid modified-Y zeolites:a novel,efficient and versatile ion exchanger[J].Journal of Hazardous Materials,2008,159(2/3):427-434.
    [22]
    程婷.酸改性沸石处理含磷废水的制备条件研究[J].山西大同大学学报(自然科学版),2017,33(1):35-37.
    [23]
    思宇,张建民,张涛,等.改性沸石对水中氨氮的去除效果[J].西安工程大学学报,2014,28(3):329-332.
    [24]
    SHAHEEN S M,EISSA F I,GHANEM K M,et al.Heavy metals removal from aqueous solutions and wastewaters by using various byproducts[J].Journal of Environmental Management,2013,128:514-521.
    [25]
    宋俊颖,何绪文,黄占斌.壳聚糖及其衍生物对土壤重金属的稳定化效应[J].化工进展,2019,38(9):4308-4319.
    [26]
    EPA.Method 1311-Toxicity Characteristic Leaching Procedure[S].Washington DC:EPA,1992.
    [27]
    郜玉楠,周历涛,王静,等.壳聚糖/沸石分子筛复合吸附颗粒的制备与性能[J].复合材料学报,2019,36(3):701-707.
    [28]
    FIGUEIREDO H,QUINTELAS C.Tailored zeolites for the removal of metal oxyanions:overcoming intrinsic limitations of zeolites[J].Journal of Hazardous Materials,2014,274:287-299.
    [29]
    ABBAS T,GHANAVATI N S,NIAZ V,et al.Chitosan/Zeolite Y/Nano ZrO2nanocomposite as an adsorbent for the removal of nitrate from the aqueous solution[J].International Journal of Biological Macromolecules,2016,93:254-266.
    [30]
    石岩.改性沸石对微污染灌溉水中Cd(Ⅱ)的吸附机理研究[D].北京:中国农业科学院,2017.
    [31]
    AMAL D,AMINE M,MIKE R,et al.Sorption of Cu(Ⅱ)ions on chitosan-zeolite X composites:impact of gelling and drying conditions[J].Molecules,2016,21(1):E109.
    [32]
    JIA W,ZENG G M.Chemical and biological assessment of Cdpolluted sediment for land use:the effect of stabilization using chitosan-coated zeolite[J].Journal of Environmental Management,2018,212:46-53.
    [33]
    杨宾,罗会龙,刘士清,等.淹水对土壤重金属浸出行为的影响及机制[J].环境工程学报,2019,13(4):936-943.
    [34]
    杨宾.水分调控下冶金污染土壤重金属形态变化及其驱动机制[D].北京:北京师范大学,2019.
    [35]
    王崇臣,王鹏.pH值对土壤中Pb、Cd释放量的影响[J].安徽农业科学,2009,37(5):2170-2171.
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索

    Article Metrics

    Article views (107) PDF downloads(8) Cited by()
    Proportional views
    Related

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return