MECHANOCHEMICAL REMEDIATION OF NON-DEGRADABLE PYRENE CONTAMINATED SOIL

HAN Han; WANG Xiao; YIN Mengqiuzi; ZHANG Qiwu; HE Xiaoman

doi:10.13205/j.hjgc.202202016

Volume 40 Issue 2

Apr. 2022

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HAN Han, WANG Xiao, YIN Mengqiuzi, ZHANG Qiwu, HE Xiaoman. MECHANOCHEMICAL REMEDIATION OF NON-DEGRADABLE PYRENE CONTAMINATED SOIL[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(2): 100-105,112. doi: 10.13205/j.hjgc.202202016

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MECHANOCHEMICAL REMEDIATION OF NON-DEGRADABLE PYRENE CONTAMINATED SOIL

doi: 10.13205/j.hjgc.202202016

School of Resources and Environmental Engineering, Wuhan University of Technology, Wuhan 430070, China

Received Date: 2021-03-06
Available Online: 2022-04-02
Publish Date: 2022-04-02

Abstract

Abstract

Mechanochemical methods were used to remediate polycyclic aromatic hydrocarbons(PAHs) contaminated soil. The effects of ball-milling time and ball-milling speed on the removal rate of pyrene in soil were studied. When the milling time was 6 h and the milling speed was 500 r/min, the removal rate of pyrene in the soil was 93.78%. The synthetic soil samples using SiO₂ before and after ball milling were analyzed by GC-MS, FT-IR spectra and Raman spectra. The degradation pathway and mechanism of pyrene were revealed as follows: the benzene rings of pyrene were destroyed, and some of the intermediate products were PAHs with fewer benzene rings and alkanes with shorter carbon chains, and some were carbonized into graphite and amorphous carbon. The residual concentration of pyrene and fluoranthene in soil was 21.45, 35.68 mg/kg when the site contaminated soil was remediation by mechanochemical method. Mechanochemical method provides a possible method and considerable application prospect in remediation of PAHs contaminated soil.
- mechanochemical methods,
- PAHs,
- soil remediation,
- degradation pathway

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References

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