INFLUENCE OF PROPERTIES OF TEXTILE DYEING SLUDGE ON DISTRIBUTION AND DEGRADATION OF PAHs AFTER THE TREATMENT OF US-Fenton

WU Junji; NING Xunan

doi:10.13205/j.hjgc.202202017

Volume 40 Issue 2

Apr. 2022

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WU Junji, NING Xunan. INFLUENCE OF PROPERTIES OF TEXTILE DYEING SLUDGE ON DISTRIBUTION AND DEGRADATION OF PAHs AFTER THE TREATMENT OF US-Fenton[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(2): 106-112. doi: 10.13205/j.hjgc.202202017

Citation:

WU Junji, NING Xunan. INFLUENCE OF PROPERTIES OF TEXTILE DYEING SLUDGE ON DISTRIBUTION AND DEGRADATION OF PAHs AFTER THE TREATMENT OF US-Fenton[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(2): 106-112. doi: 10.13205/j.hjgc.202202017

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INFLUENCE OF PROPERTIES OF TEXTILE DYEING SLUDGE ON DISTRIBUTION AND DEGRADATION OF PAHs AFTER THE TREATMENT OF US-Fenton

doi: 10.13205/j.hjgc.202202017

WU Junji,
NING Xunan^,

Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control, School of Environment Science and Engineering,Guangdong University of Technology, Guangzhou 510006, China

Received Date: 2020-12-18
Available Online: 2022-04-02
Publish Date: 2022-04-02

Abstract

Abstract

The physicochemical properties of four kinds of textile dyeing sludge were investigated, including the levels of metal, nonmetal, organic matter and 16 polycyclic aromatic hydrocarbons(Σ₁₆PAHs). Furthermore, the relationship between the degradation efficiency of PAHs after the treatment of ultrasonic Fenton technology(US-Fenton) and the physicochemical properties of the sludge were discussed. The results showed that the concentration of Σ₁₆PAHs in sludge was 983.52~2942.34 ng/g, and that of the low molecular weight PAHs was 570.47~1919.97 ng/g, which was the main component of Σ₁₆PAHs, accounting for more than 50% by mass weight. After the US-Fenton treatment, the degradation rate of Σ₁₆PAHs was 35.24%~61.80% and the degradation rate of lower molecular weight PAHs was higher than that of the higher molecular weight PAHs, about 28.22%~40.48% and 11.76%~24.04%, respectively. The results indicated that the characteristics of the sludge had a great impact on the degradation of PAHs, among which, C, Fe and organic matter content had a negative correlation with the degradation of PAHs, respectively. Ca content in sludge had a positive correlation with the degradation rate of PAHs. And their correlation coefficient R² were all more than 0.90. This study would provide a theoretical basis for the degradation of PAHs and other organic pollutants in sludge by US-Fenton.
- textile dyeing sludge,
- PAHs,
- physicochemical properties,
- organic matter,
- US-Fenton degradation

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References(24)

References

[1]	LIANG X,NING X A,CHEN G X,et al.Concentrations and speciation of heavy metals in sludge from nine textile dyeing plants[J].Ecotoxicol and Environmental Safety,2013,98(Dec.1):128-134.
[2]	NING X A,LIN M Q,SHEN L Z,et al.Levels,composition profiles and risk assessment of polycyclic aromatic hydrocarbons (PAHs) in sludge from ten textile dyeing plants[J].Environmental Research,2014,132:112-118.
[3]	NING X A,LIANG J Y,LI R J,et al.Aromatic amine contents,component distributions and risk assessment in sludge from 10 textile-dyeing plants[J].Chemosphere,2015,134:367-373.
[4]	HWANG I K,KANG H H,LEE I S,et al.Assessment of characteristic distribution of PCDD/Fs and BFRs in sludge generated at municipal and industrial wastewater treatment plants[J].Chemosphere,2012,88(7):888-894.
[5]	ZHOU X,ZHOU Y X,LIU J S,et al.Study on the pollution characteristics and emission factors of PCDD/Fs from disperse dye production in China[J].Chemosphere,2019,228(AUG.):328-334.
[6]	LIN M,NING X A,AN T,et al.Degradation of polycyclic aromatic hydrocarbons (PAHs) in textile dyeing sludge with ultrasound and Fenton processes:effect of system parameters and synergistic effect study[J].Journal of Hazardous Materials,2016,307:7-16.
[7]	ZHANG J H,ZOU H Y,NING X A,et al.Combined ultrasound with Fenton treatment for the degradation of carcinogenic polycyclic aromatic hydrocarbons in textile dying sludge[J].Environmental Geochemistry & Health,2017(1):1-10.
[8]	BOULANGE M,C.LORGEOUX,C.BIACHE,et al.Fenton-like and potassium permanganate oxidations of PAH-contaminated soils:impact of oxidant doses on PAH and polar PAC (polycyclic aromatic compound) behavior[J].Chemosphere,2019,224(JUN.):437-444.
[9]	ZHANG H,ZHEN W J.Performance,rheological behavior and enzymatic degradation of poly(lactic acid)/modified fulvic acid composites[J].International Journal of Biological Macromolecules,2019,139:181-190.
[10]	KE Y W,NING X A,LIANG J Y,et al.Sludge treatment by integrated ultrasound-Fenton process:characterization of sludge organic matter and its impact on PAHs removal[J].Journal of Hazardous Materials,2017,343:191-199.
[11]	ZHAO Y P,TAN Y Y,GUO Y,et al.Interactions of tetracycline with Cd (Ⅱ),Cu (Ⅱ) and Pb (Ⅱ) and their cosorption behavior in soils[J].Environmental Pollution,2013,180(sep.):206-213.
[12]	NCUBE S,KUNENE P,TAVENGWA N T,et al.Synthesis and characterization of a molecularly imprinted polymer for the isolation of the 16 US-EPA priority polycyclic aromatic hydrocarbons (PAHs) in solution[J].Journal of Environmental Management,2017,199(sep.1):192-200.
[13]	陈涛,孙水裕,刘敬勇,等.城市污水污泥焚烧二次污染物控制研究进展[J].化工进展,2010,29(1):157-162.
[14]	陈剑峰.印染污泥元素分析及干化焚烧方案[J].化学工程与装备,2017(9):343-346.
[15]	吴浩亮,杜伟志,陈繁忠,等.关于佛山市印染污泥现状分析及焚烧处理的研究[J].化纤与纺织技术,2015,34 (1):23-30.
[16]	MAN Y B,CHOW K L,CHENG Z,et al.Profiles and removal efficiency of polycyclic aromatic hydrocarbons by two different types of sewage treatment plants in Hong Kong[J].Journal of Environmental Sciences,2017,53(3):196-206.
[17]	王靖宇.印染废水处理过程中芳香烃化合物的污染特征和去除特性研究[D].广州:广东工业大学,2015.
[18]	CHEN C F,JU Y R,LIM Y C,et al.Determination of polycyclic aromatic hydrocarbons in sludge from water and wastewater treatment plants by GC-MS[J].International Journal of Environmental Research and Public Health,2019,16(14):2604.
[19]	黄兴如,张彩文,张瑞杰,等.多环芳烃降解菌的筛选、鉴定及降解特性[J].微生物学通报,2016,43(5):965-973.
[20]	LIN M Q,NING X A,AN T C,et al.Degradation of polycyclic aromatic hydrocarbons (PAHs) in textile dyeing sludge with ultrasound and Fenton processes:effect of system parameters and synergistic effect study[J].Journal of Hazardous Materials,2016,307:7-16.
[21]	ADEOLA A O,FORBES P B C.Influence of natural organic matter fractions on PAH sorption by stream sediments and a synthetic graphene wool adsorbent[J].Environmental Technology & Innovation,2020,21:101202.
[22]	程琳.孔道结构铁矿物的改性及其在污染治理中的应用[D].扬州:扬州大学,2017.
[23]	POURAN S R,RAMAN A A A,WAN M A W D.Review on the application of modified iron oxides as heterogeneous catalysts in Fenton reactions[J].Journal of Cleaner Production,2014,64(2):24-35.
[24]	GAURAV G K,MEHMOOD T,KUMAR M,et al.Review on polycyclic aromatic hydrocarbons (PAHs) migration from wastewater-Science Direct[J].Journal of Contaminant Hydrology,2021,236:103715.