Core Chinese Journal
Source Journal of CSCD(Core Version)
Source Journal for Chinese Scientific and Technical Papers
Core Journal of RCCSE
Included in JST China
Volume 40 Issue 9
Nov.  2022
Turn off MathJax
Article Contents
LI Yan-xue, ZHANG Meng-zhu, SHU Sha-sha, ZOU Jun-han, JIAO Wei, ZHOU Jun-yu. QUANTITATIVE IDENTIFICATION OF ANTHROPOGENIC HEAVY METAL SOURCES IN FARMLAND SOIL BASED ON ENRICHMENT FACTOR AND MLR-APCS MODEL[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(9): 173-177,232. doi: 10.13205/j.hjgc.202209023
Citation: LI Yan-xue, ZHANG Meng-zhu, SHU Sha-sha, ZOU Jun-han, JIAO Wei, ZHOU Jun-yu. QUANTITATIVE IDENTIFICATION OF ANTHROPOGENIC HEAVY METAL SOURCES IN FARMLAND SOIL BASED ON ENRICHMENT FACTOR AND MLR-APCS MODEL[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(9): 173-177,232. doi: 10.13205/j.hjgc.202209023

QUANTITATIVE IDENTIFICATION OF ANTHROPOGENIC HEAVY METAL SOURCES IN FARMLAND SOIL BASED ON ENRICHMENT FACTOR AND MLR-APCS MODEL

doi: 10.13205/j.hjgc.202209023
  • Received Date: 2021-11-19
    Available Online: 2022-11-09
  • An accurate and quantitative identification of anthropogenic heavy metal sources in farmland soil is vital for the subsequent implementation of more precise prevention and control. In this study, soil samples were collected from a typical agricultural area, and the anthropogenic sources of heavy metals in the surface soils were quantitatively identified by using the enrichment factor(EF) and multiple linear regression of absolute principal component scores(MLR-APCS) model.Resultsshowed that heavy metals like Pb, Cu, Zn, Cr and Ni in the surface soil have been affected by anthropogenic sources to different extents. The average increases rates in Pb, Cu, Zn, Cr and Ni were 112.37%, 71.21%, 59.38%, 69.67% and 64.54% respectively, when comparing their total contents in the surface soils with the contents in the local background soils. The EF values of heavy metals decreased with the order of Pb, Cu, Cr, Ni and Zn. Among them, Pb reached a medium enrichment level, and its anthropogenic content was more than 50% of the total content. Based on the anthropogenic heavy metal contents, atmospheric deposition and livestock manure were identified as the two main anthropogenic heavy metal sources. The MLR-APCS simulation results showed that atmospheric deposition could contribute on average 42.41%, 37.58% and 37.26% of total Pb, Cr and Ni contents, respectively, while livestock manure contributed 41.67% of total Cu and 39.39% of total Zn contents. In general, this study provided a reliable method for quantitative identification of anthropogenic heavy metal sources in farmland soil, which can be applied in other similar areas.
  • loading
  • [1]
    SHAO D W,ZHAN Y,ZHOU W J,et al.Current status and temporal trend of heavy metals in farmland soil of the Yangtze River Delta Region:field survey and meta-analysis[J].Environmental Pollution,2016,219:329-336.
    [2]
    窦韦强,安毅,秦莉,等.农田土壤重金属垂直分布迁移特征及生态风险评价[J].环境工程,2021,39(2):166-172.
    [3]
    郑影怡,刘杰,蒋萍萍,等.河池市某废弃冶炼厂周边农田土壤重金属污染特征及风险评价[J].环境工程,2021,39(5):238-245.
    [4]
    TOTH G,HERMANN T,da SILVA M R,et al.Heavy metals in agricultural soils of the European Union with implications for food safety[J].Environment International,2016,88:299-309.
    [5]
    安外尔·艾力,麦麦提吐尔逊·艾则孜,靳万贵,等.新疆焉耆盆地农田土壤重金属环境容量分析[J].环境工程,2020,38(3):168-173.
    [6]
    周江明.中国耕地重金属污染现状及其人为污染源浅析[J].中国土壤与肥料,2020(2):83-92.
    [7]
    JIAO W,NIU Y,NIU Y,et al.Spatial assessment of the anthropogenic impact on trace metal accumulation in farmland soils from a rapid industrializing region,East China[J].International Journal of Environmental Research and Public Health,2018,15:2052.
    [8]
    章明奎,王浩,张慧敏.浙东海积平原农田土壤重金属来源辨识[J].环境科学学报,2008,28(10):1946-1954.
    [9]
    李瑞平,郝英华,李光德,等.泰安市农田土壤重金属污染特征及来源解析[J].农业环境科学学报,2011,30(10):2012-2017.
    [10]
    MICO C,RECATALA L,PERIS A,et al.Assessing heavy metal sources in agricultural soils of an European Mediterranean area by multivariate analysis[J].Chemosphere,2006,65(5):863-872.
    [11]
    陈雅丽,翁莉萍,马杰,等.近十年中国土壤重金属污染源解析研究进展[J].农业环境科学学报,2019,38(10):2219-2238.
    [12]
    李娇,吴劲,蒋进元,等.近十年土壤污染物源解析研究综述[J].土壤通报,2018,49(1):232-242.
    [13]
    SHI D Q,LU X W.Accumulation degree and source apportionment of trace metals in smaller than 63 μm road dust from the areas with different land uses:a case study of Xi’an,China[J].Science of the Total Environment,2018,636:1211-1218.
    [14]
    霍明珠,高秉博,乔冬云,等.基于APCS-MLR受体模型的农田土壤重金属源解析[J].农业环境科学学报,2021,40(5):978-986.
    [15]
    史文昌,古正刚,冯燕,等.基于APCS-MLR的宝象河沉积物重金属污染源解析[J].环境科学与技术,2020,43(10):51-59.
    [16]
    YANG Y,CHRISTAKOS G,GUO M W,et al.Space-time quantitative source apportionment of soil heavy metal concentration increments[J].Environmental Pollution,2017,223:560-566.
    [17]
    N’GUESSAN Y M,PROBST J L,BUR T,et al.Trace elements in stream bed sediments from agricultural catchments (Gascogne region,S-W France):where do they come from[J].Science of the Total Environment,2009,407:2939-2952.
    [18]
    中华人民共和国农业部.农田土壤环境质量监测技术规范:NY/T 395—2012 [S].北京:中国农业出版社,2012.
    [19]
    中华人民共和国环境保护部.土壤和沉积物金属元素总量的消解微波消解法:HJ 832—2017[S].北京:中国环境出版社,2017.
    [20]
    BLASER P,ZIMMERMANN S,LUSTER J,et al.Critical examination of trace element enrichments and depletions in soils:As,Cr,Cu,Ni,Pb,and Zn in Swiss forest soils[J].Science of the Total Environment,2000,249:257-280.
    [21]
    NIU L L,YANG F X,XU C,et al.Status of metal accumulation in farmland soils across China:from distribution to risk assessment[J].Environmental Pollution,2013,176:55-62.
    [22]
    中华人民共和国生态环境部.土壤环境质量农用地土壤污染风险管控标准:GB 15618—2018 (试行)[S].北京:中国环境出版社,2018.
    [23]
    SUTHERLAND R A.Bed sediment-associated trace metals in an urban stream,Oahu,Hawaii[J].Environmental geology,2000,39:611-627.
    [24]
    PALLEIRO L,PATINHA C,RODRIGUEZ-BLANCO M L,et al.Metal fractionation in topsoils and bed sediments in the Mero River rural basin:bioavailability and relationship with soil and sediment properties[J].Catena,2016,144:34-44.
    [25]
    ZHAO L S,YAN Y,YU R L,et al.Source apportionment and health risks of the bioavailable and residual fractions of heavy metals in the park soils in a coastal city of China using a receptor model combined with Pb isotopes[J].Catena,2020,194:104736.
    [26]
    焦伟,牛勇,李斌,等.基于化学形态分析的城市道路灰尘重金属健康风险评价与人为来源解析[J].生态环境学报,2018,27(12):2269-2275.
    [27]
    HU Y A,CHENG H F.A method for apportionment of natural and anthropogenic contributions to heavy metal loadings in the surface soils across large-scale regions[J].Environmental Pollution,2016,214:400-409.
    [28]
    LOCKITCH G.Perspectives on lead toxicity[J].Clinical Biochemistry,1993,26:371-381.
    [29]
    刘娟,李洋,张敏,等.滇东农田土壤铅污染健康风险评价及基准研究[J].农业工程学报,2021,37(1):241-250.
    [30]
    LUO L,MA Y B,ZHANG S Z,et al.An inventory of trace element inputs to agricultural soils in China[J].Journal of Environmental Management,2009,90:2524-2530.
    [31]
    陆平,赵雪艳,殷宝辉,等.临沂市 PM2.5和PM10中元素分布特征及来源解析[J].环境科学,2020,41(5):2036-2043.
    [32]
    张国忠,黄威,潘月鹏,等.河北典型农田大气重金属干沉降通量及来源解析[J].中国生态农业学报,2019,27(8):1245-1254.
    [33]
    DACH J,STARMANS D.Heavy metals balance in Polish and Dutch agronomy:actual state and previsions for the future[J].Agriculture,Ecosystems & Environment,2005,107:309-316.
    [34]
    JIAO W,NIU Y,NIU Y,et al.Quantitative identification of anthropogenic trace metal sources in surface river sediments from a hilly agricultural watershed,East China[J].Environmental Science and Pollution Research,2019,26:32266-32275.
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索

    Article Metrics

    Article views (104) PDF downloads(3) Cited by()
    Proportional views
    Related

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return