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Volume 40 Issue 11
Nov.  2022
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Article Navigation >  ENVIRONMENTAL ENGINEERING  > 2022  >  40(11): 61-68
ZHANG Lijun, YAN Qun, ZHOU Zilin, CHEN Yan, CHEN Jinfu. NANOPARTICLES SUPPORTED BY DIATOMITE FOR REMOVAL OF ORANGE Ⅱ THROUGH ACTIVATING PMS[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(11): 61-68. doi: 10.13205/j.hjgc.202211009
Citation: ZHANG Lijun, YAN Qun, ZHOU Zilin, CHEN Yan, CHEN Jinfu. NANOPARTICLES SUPPORTED BY DIATOMITE FOR REMOVAL OF ORANGE Ⅱ THROUGH ACTIVATING PMS[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(11): 61-68. doi: 10.13205/j.hjgc.202211009
shu

NANOPARTICLES SUPPORTED BY DIATOMITE FOR REMOVAL OF ORANGE Ⅱ THROUGH ACTIVATING PMS

doi: 10.13205/j.hjgc.202211009

  • 1. School of Resources and Environmental Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, China;

  • 2. School of Civil and Surveying&Mapping Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, China;

  • 3. Research Center for Water Quality Security Technology at Ganjiang River Basin, Jiangxi University of Science and Technology, Ganzhou 341000, China

  • Received Date: 2022-03-08
    Available Online: 2023-03-24
    Abstract
  • Diatomite/MnFe2O4 composite catalyst (DMF) was rationally synthesized by sol-gel method. The performance and reaction mechanism of DMF activated peroxymonosulfate (PMS) were degraded with orange Ⅱ as the target pollutant. The results showed that:1) MnFe2O4 particles were uniformly loaded on diatomite and DMF had better dispersion and stability; 2) DMF had a better catalytic activity to PMS than MnFe2O4 so that the degradation rate of DMF/PMS system for orange Ⅱ removal was 2.16 times that of MnFe2O4 system, the reaction process could be fitted by the pseudo-first-order kinetic pattern. A degradation rate of 93.1% could be achieved within 40 min for 50 mg/L AO2 by 0.5 g/L DMF and 0.5 mmol/L PMS; 3) there were four active radicals ·OH、SO4-·、1O2 and ·O2- in the reaction system, and OH and SO4- play the main role; 4) DMF had better structural stability and its metal ion dissolution was much lower than MnFe2O4. This study paved a way for the practical application of the new PMS activators in industrial wastewater treatment.
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    • References(29)
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