Source Jouranl of CSCD
Source Journal of Chinese Scientific and Technical Papers
Included as T2 Level in the High-Quality Science and Technology Journals in the Field of Environmental Science
Core Journal of RCCSE
Included in the CAS Content Collection
Included in the JST China
Indexed in World Journal Clout Index (WJCI) Report
Volume 40 Issue 11
Nov.  2022
Turn off MathJax
Article Contents
Abstract
References
Article Navigation >  ENVIRONMENTAL ENGINEERING  > 2022  >  40(11): 61-68
LIU Jun, PAN Tianqi, ZHAO Huihui, GUO Yan, CHEN Guanyi, HOU Li'an. A MODEL OF CARBON EMISSION REDUCTION CALCULATION FOR AEROBIC REMEDIATION PROCESS IN MSW LANDFILLS BASED ON PRINCIPAL COMPONENT ANALYSIS[J]. ENVIRONMENTAL ENGINEERING , 2023, 41(9): 133-139. doi: 10.13205/j.hjgc.202309016
Citation: ZHANG Lijun, YAN Qun, ZHOU Zilin, CHEN Yan, CHEN Jinfu. NANOPARTICLES SUPPORTED BY DIATOMITE FOR REMOVAL OF ORANGE Ⅱ THROUGH ACTIVATING PMS[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(11): 61-68. doi: 10.13205/j.hjgc.202211009
shu

NANOPARTICLES SUPPORTED BY DIATOMITE FOR REMOVAL OF ORANGE Ⅱ THROUGH ACTIVATING PMS

doi: 10.13205/j.hjgc.202211009

  • 1. School of Resources and Environmental Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, China;

  • 2. School of Civil and Surveying&Mapping Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, China;

  • 3. Research Center for Water Quality Security Technology at Ganjiang River Basin, Jiangxi University of Science and Technology, Ganzhou 341000, China

  • Received Date: 2022-03-08
    Available Online: 2023-03-24
    Abstract
  • Diatomite/MnFe2O4 composite catalyst (DMF) was rationally synthesized by sol-gel method. The performance and reaction mechanism of DMF activated peroxymonosulfate (PMS) were degraded with orange Ⅱ as the target pollutant. The results showed that:1) MnFe2O4 particles were uniformly loaded on diatomite and DMF had better dispersion and stability; 2) DMF had a better catalytic activity to PMS than MnFe2O4 so that the degradation rate of DMF/PMS system for orange Ⅱ removal was 2.16 times that of MnFe2O4 system, the reaction process could be fitted by the pseudo-first-order kinetic pattern. A degradation rate of 93.1% could be achieved within 40 min for 50 mg/L AO2 by 0.5 g/L DMF and 0.5 mmol/L PMS; 3) there were four active radicals ·OH、SO4-·、1O2 and ·O2- in the reaction system, and OH and SO4- play the main role; 4) DMF had better structural stability and its metal ion dissolution was much lower than MnFe2O4. This study paved a way for the practical application of the new PMS activators in industrial wastewater treatment.
    • FullText(HTML)
    • References(29)
  • [1]
    MERCYRAN B, HERNANDEZ-MAYA R, SOLÍS-LÓPEZ1 M, et al. Photocatalytic degradation of Orange G using TiO2/Fe3O4 nanocomposites[J]. Journal of Materials Science:Materials in Electronics, 2018, 29(8):15436-15444.
    [2]
    HU L X, DENG G H, LU W C, et al. Peroxymonosulfate activation by Mn3O4/metal-organic framework for degradation of refractory aqueous organic pollutant rhodamine B[J]. Chinese Journal of Catalysis, 2017, 38(8):1360-1372.
    [3]
    OLMEZ-HANCI T, ARSLAN-ALATON I. Comparison of sulfate and hydroxyl radical based advanced oxidation of phenol[J].Chemical Engineering Journal, 2013, 224(1):10-16.
    [4]
    XU Y, AI J, ZHANG H. The mechanism of degradation of bisphenol A using the magnetically separable CuFe2O4/peroxymonosulfate heterogeneous oxidation process[J]. Journal of Hazardous Materials, 2016, 309:87-96.
    [5]
    SHAO S, QIAN L, ZHAN X, et al. Transformation and toxicity evolution of amlodipine mediated by cobalt ferrite activated peroxymonosulfate:effect of oxidant concentration[J]. Chemical Engineering Journal, 2020, 382:123005.
    [6]
    XIONG C Y, REN Q F, CHEN S H, et al. A multifunctional Ag3PO4/Fe3O4/Diatomite composites:photocatalysis, adsorption and sterilization[J]. Materials Today Communications, 2021, 28:102695.
    [7]
    KHRAISHEH M A, AL-GHOUTI M A, ALLEN S J. Effect of OH and silanol groups in the removal of dyes from aqueous solution using diatomite[J]. Water Research, 2005, 39(5):922-932.
    [8]
    DONG X D, SUN Z M, ZHANG X W, et al. Synthesis and enhanced solar light photocatalytic activity of a C/N Co-doped TiO2/diatomite composite with exposed (001) facets[J]. Australian Journal of Chemistry, 2018, 71:315-324.
    [9]
    WANG B, ZHANG G X, LENG X, et al, Characterization and improved solar light activity of vanadium doped TiO2/diatomite hybrid catalysts[J]. Journal of Hazardous Materials, 2015, 285:212-220.
    [10]
    TAN C Q, GAO N Y, FU D F, et al. Efficient degradation of paracetamol with nanoscaled magnetic CoFe2O4 and MnFe2O4 as a heterogeneous catalyst of peroxymonosulfate[J]. Separation and Purification Technology, 2017, 175:47-57.
    [11]
    石清清,蒲生彦,杨犀.纳米Cu0@Fe3O4活化PMS降解对-硝基苯酚的协同反应机制[J]. 环境科学, 2020, 41(10):4616-4625.
    [12]
    ZHANG Z L, WANG Y, TAN Q Q, et al. Facile solvothermal synthesis of mesoporous manganese ferrite (MnFe2O4) microspheres as anode materials for lithium-ion batteries[J]. Journal of Colloid and Interface Science, 2013, 398:185-192.
    [13]
    TAN C Q, GAO N Y, DENG Y, et al. Radical induced degradation of acetaminophen with Fe3O4 magnetic nanoparticles as heterogeneous activator of peroxymonosulfate[J]. Journal of Hazardous Materials, 2014, 276:442-460.
    [14]
    DATSKO T Y, ZELENTSOV V I, DATSKO E E, et al. Physicochemical and adsorption-structural properties of diatomite modified with aluminum compounds[J]. Surface Engineering and Applied Electrochemistry, 2011, 47(6):530-539.
    [15]
    HU Z B, ZHENG S L, JIA M Z, et al. Preparation and characterization of novel diatomite/ground calcium carbonate composite humidity control material[J]. Separation and Purification Technology. Advanced Powder Technology, 2017, 28(5):1372-1381.
    [16]
    FENG Y, WU D L, DENG Y, et al. Sulfate radical-mediated degradation of sulfadiazine by CuFeO2 rhombohedral crystal-catalyzed peroxymonosulfate:synergistic effects and mechanisms[J]. Environmental Science & Technology, 2016, 50(6):3119-3127.
    [17]
    LIN C H, SHI D J, WU Z T, et al. CoMn2O4 catalyst prepared using the sol-gel method for the activation of peroxymonosulfate and degradation of UV filter 2-phenylbenzimidazole-5-sulfonic acid(PBSA)[J]. Nanomaterials, 2019, 9(5):774.
    [18]
    TAN Y, LI C Q, SUN Z M, et al. Natural diatomite mediated spherically monodispersed CoFe2O4 nanoparticles for efficient catalytic oxidation of bisphenol A through activating peroxymonosulfate[J]. Chemical Engineering Journal, 2020, 388:124386.
    [19]
    GUAN Y H, MA J, REN Y M, et al. Efficient degradation of atrazine by magnetic porous copper ferrite catalyzed peroxymonosulfate oxidation via the formation of hydroxyl and sulfate radicals[J]. Water Reseach, 2013, 47(14):5431-5438.
    [20]
    HUANG G X, WANG C Y, YANG C W, et al. Degradation of bisphenol a by peroxymonosulfate catalytically activated with Mn1.8Fe1.2O4 nanospheres:synergism between Mn and Fe[J]. Environmental Science & Technology, 2017, 51(21):12611-12618.
    [21]
    PAN Y, SU H R, ZHU Y T, et al. CaO2 based Fenton-like reaction at neutral pH:accelerated reduction of ferric species and production of superoxide radicals[J]. Water Research, 2018, 145:731-740.
    [22]
    DUAN P J, MA T F, YUE Y. Fe/Mn nanoparticles encapsulated in nitrogen-doped carbon nanotubes as a peroxymonosulfate activator for acetamiprid degradation[J]. Environmental Science:Nano, 2019, 6(6):1799-1811.
    [23]
    YANG S S, WUA P X, LIU J Q, et al. Efficient removal of bisphenol A by superoxide radical and singlet oxygen generated from peroxymonosulfate activated with Fe0-montmorillonite[J]. Chemical Engineering Journal, 2018, 350:484-495.
    [24]
    DONG X B, REN B X, SUN Z M, et al. Monodispersed CuFe2O4 nanoparticles anchored on natural kaolinite as highly efficient peroxymonosulfate catalyst for bisphenol A degradation[J]. Applied Catalysis B:Environmental, 2019, 253:206-217.
    [25]
    DENG J, FENG S F, MA X Y, et al. Heterogeneous degradation of Orange Ⅱ with peroxymonosulfate activated by ordered mesoporous MnFe2O4[J]. Separation and Purification Technology, 2016, 167:181-189.
    [26]
    GUAN Y H, MA J, LI X C, et al. Influence of pH on the Formation of Sulfate and Hydroxyl Radicals in the UV/Peroxymonosulfate System[J]. Environmental Science & Technology, 2011, 45(21):9308-9314.
    [27]
    FU H C, MA S L, ZHAO P, et al. Activation of peroxymonosulfate by graphitized hierarchical porous biochar and MnFe2O4 magnetic nanoarchitecture for organic pollutants degradation:structure dependence and mechanism[J]. Chemical Engineering Journal, 2019, 360:157-170.
    [28]
    MA W J, WANG N, DU Y C, et al. One-step synthesis of novel Fe3C@nitrogen-doped carbon nanotubes/graphene nanosheets for catalytic degradation of Bisphenol A in the presence of peroxymonosulfate[J]. Chemical Engineering Journal, 2019, 356:1022-1031.
    [29]
    ANIPSITAKIS G P, DIONYSIOU D D, GONZALEZ M A. Cobalt-mediated activation of peroxymonosulfate and sulfate radical attack on phenolic compounds:implications of chloride ions[J]. Environmental Science & Technology, 2006, 40(3):1000-1007.
    • Relative Articles

  • Relative Articles

    [1]HE Xi, LIU Chen, LI Jinglu, CHEN Ming, B. Larry LI. PERFORMANCE AND MECHANISM OF CSB-BOC ACTIVATED PMS FOR REMOVAL OF TETRACYCLINE HYDROCHLORIDE IN WATER IN SLOW-GATHERING AREAS OF RIVER[J]. ENVIRONMENTAL ENGINEERING , 2024, 42(2): 82-96. doi: 10.13205/j.hjgc.202402010
    [2]XU Zhenyang, FANG Qinglu, GU Wenwen, LI Zhiying, ZHANG Yimei, WANG Fei. PERFORMANCE OF Bi2WO6@MXenes-NS ACTIVATED PERMONOSULFATE IN DEGRADING BISPHENOL A[J]. ENVIRONMENTAL ENGINEERING , 2023, 41(4): 10-17,62. doi: 10.13205/j.hjgc.202304002
    [3]ZHANG Shicheng, LI Simin, ZHU Jia. DEGRADATION OF METHYL ORANGE BY CuO/g-C3N4 ACTIVATED PEROXODISULFATE[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(10): 40-48. doi: 10.13205/j.hjgc.202210006
    [4]ZHA Wengui, WANG Xueye, WANG Zhiwei. PILOT-SCALE STUDY ON MEMBRANE-CATHODE ELECTRO-FENTON PROCESS FOR PRETREATMENT OF SEMICONDUCTOR WASTEWATER[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(4): 153-158,208. doi: 10.13205/j.hjgc.202204022
    [5]SUN Su-yun, LI Bao-lei, KONG De-yong, HOU Ya-nan, MA Jin-feng, GUO Jian-bo, SONG Yuan-yuan. ADSORPTION AND TRANSFORMATION OF CHLOROPYRIDINE: RESEARCH ADVANCES AND CHALLENGES[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(5): 227-236. doi: 10.13205/j.hjgc.202205032
    [6]ZHOU Kang, WANG Zhen-kai, ZHANG Gui-cheng, CHEN Xin-an, CHENG Yan, LUO Gang, SUN Sheng-peng. BIODEGRADATION AND TERTIARY TREATMENT EFFICIENCIES OF TYPICAL PHARMACEUTICAL MICROPOLLUTANTS BY MBBR AND UVC-BASED ADVANCED OXIDATION PROCESSES[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(5): 37-43. doi: 10.13205/j.hjgc.202205006
    [7]LIAO Xiaoshu, ZHU Chengyu, CHOU Yue, ZHONG Min, ZHOU Bingling, ZHANG Qian. PERSULFATE ACTIVATION VIA NANOSCALE ZERO-VALENT IRON BASED BIOCHAR FOR OXYTETRACYCLINE DEGRADATION[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(8): 118-124,95. doi: 10.13205/j.hjgc.202208016
    [8]GUO Zhi-wei, ZHAO Bao-long, ZHENG Zhi-hong, HONG Fei-yu, XIN Si-yuan, WANG Xiao-wei, WANG Xing-xiao, ZHANG Zhen-zhen, NIU Fang, LI Guo-ting. PREPARATION OF MODIFIED DIATOMITE VIA CARBONIZATION AND ITS ADSORPTION PERFORMANCE ON TETRACYCLINE[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(5): 44-52. doi: 10.13205/j.hjgc.202205007
    [9]ZHU Tong, YANG Shi-peng, TAN Wei-qiang, WANG Kai-jun. DEGRADATION OF 2,4,6-TRICHLOROPHENOL BY UV/O3/TiO2 COUPLING PROCESS[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(3): 7-13. doi: 10.13205/j.hjgc.202103002
    [10]CAO Yuan, LI Xiao-dong, PENG Chang-sheng, SUN Zong-quan, SHEN Jia-lun, MA Fu-jun, GU Qing-bao. REMOVAL OF 2,4-DINITROTOLUENE BY PERSULFATE ACTIVATED WITH IRON MODIFIED BIOCHAR PREPARED BY DIPPING-PYROLYSIS PROCESS[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(11): 135-142,178. doi: 10.13205/j.hjgc.202111017
    [11]CHEN Yong-kang, LU Bin, CHAI Xiao-li, CHANG Fei. PILOT TEST OF TREATING SEWAGE FROM PUMPING STATION WITH A BIO-DIATOMITE REACTOR[J]. ENVIRONMENTAL ENGINEERING , 2020, 38(12): 6-12. doi: 10.13205/j.hjgc.202012002
    • Supplements(0)
    • Cited By

  • Cited by

    Periodical cited type(3)

    1. 刘克琼，王福浩，占美丽，张国栋，王亚楠，夏正启，付友先，孙英杰. 膜浓缩液蒸发母液回灌填埋场对渗滤液水质及处理系统的影响研究. 给水排水. 2024(02): 39-44 .
    2. 韦艺佳，张金冉，朱润泽，孙治国，夏正启，占美丽，刘克琼. 絮凝预处理对垃圾浓缩液有机物去除影响研究. 山东化工. 2024(17): 270-273 .
    3. 李硕晨，李学刚，贺志鹏，宋金明，刘珊珊，王志博. 基于钙添加的海水无机碳移除的增汇潜力研究. 中国环境科学. 2024(10): 5912-5920 .

    Other cited types(1)

  • Created with Highcharts 5.0.7Amount of accessChart context menuAbstract Views, HTML Views, PDF Downloads StatisticsAbstract ViewsHTML ViewsPDF Downloads2024-052024-062024-072024-082024-092024-102024-112024-122025-012025-022025-032025-0402.557.51012.515
    Created with Highcharts 5.0.7Chart context menuAccess Class DistributionFULLTEXT: 17.1 %FULLTEXT: 17.1 %META: 82.5 %META: 82.5 %PDF: 0.4 %PDF: 0.4 %FULLTEXTMETAPDF
    Created with Highcharts 5.0.7Chart context menuAccess Area Distribution其他: 13.7 %其他: 13.7 %临汾: 0.4 %临汾: 0.4 %兰州: 0.9 %兰州: 0.9 %北京: 0.9 %北京: 0.9 %南京: 0.9 %南京: 0.9 %台州: 0.9 %台州: 0.9 %合肥: 0.4 %合肥: 0.4 %嘉兴: 0.4 %嘉兴: 0.4 %天津: 0.9 %天津: 0.9 %常州: 0.4 %常州: 0.4 %常德: 0.9 %常德: 0.9 %张家口: 0.9 %张家口: 0.9 %成都: 0.4 %成都: 0.4 %新乡: 1.3 %新乡: 1.3 %昆明: 1.7 %昆明: 1.7 %晋城: 0.9 %晋城: 0.9 %朝阳: 0.4 %朝阳: 0.4 %杭州: 1.3 %杭州: 1.3 %武汉: 1.3 %武汉: 1.3 %济南: 0.4 %济南: 0.4 %济源: 0.4 %济源: 0.4 %温州: 0.4 %温州: 0.4 %漯河: 1.7 %漯河: 1.7 %芒廷维尤: 37.2 %芒廷维尤: 37.2 %芝加哥: 0.4 %芝加哥: 0.4 %衡阳: 0.4 %衡阳: 0.4 %衢州: 0.4 %衢州: 0.4 %西宁: 22.6 %西宁: 22.6 %贵阳: 0.4 %贵阳: 0.4 %运城: 3.4 %运城: 3.4 %遵义: 0.4 %遵义: 0.4 %郑州: 0.4 %郑州: 0.4 %长沙: 0.9 %长沙: 0.9 %长治: 1.3 %长治: 1.3 %阿什本: 0.4 %阿什本: 0.4 %其他临汾兰州北京南京台州合肥嘉兴天津常州常德张家口成都新乡昆明晋城朝阳杭州武汉济南济源温州漯河芒廷维尤芝加哥衡阳衢州西宁贵阳运城遵义郑州长沙长治阿什本

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索
    Get Citation
    PDF
    XML

    Article Metrics

    Article views (193) PDF downloads(1) Cited by(4)
    Proportional views
    Related

    Journal Online

    Authors' Center

    Links

    Copyright © 《工业建筑》杂志社有限公司 京ICP备11033253号-1

    Supported by: Beijing Renhe Information Technology Co. Ltd     百度统计

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return