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LIU Wei, ZHONG Zhaoping, LIU Jin, ZHOU Yuguo, YU Shunyao. CFD-BASED FLOW FIELD OPTIMIZATION AND BAG LEAKAGE SIMULATION OF FABRIC BAGHOUSE FILTERS[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(11): 84-91,142. doi: 10.13205/j.hjgc.202211012
Citation: ZHAO Bin, YANG Yang, QIU Fengtao, SU Yan, QU Zhenhe, HUANG Qian, JIANG Qi, XU Hao. PREPARATION OF STAINLESS STEEL-BASED Sb-SnO2/PbO2 ELECTRODE AND EFFECT OF ELECTRODEPOSITION FACTORS ON ITS PERFORMANCE[J]. ENVIRONMENTAL ENGINEERING , 2023, 41(4): 26-31,39. doi: 10.13205/j.hjgc.202304004

PREPARATION OF STAINLESS STEEL-BASED Sb-SnO2/PbO2 ELECTRODE AND EFFECT OF ELECTRODEPOSITION FACTORS ON ITS PERFORMANCE

doi: 10.13205/j.hjgc.202304004
  • Received Date: 2022-05-27
    Available Online: 2023-05-26
  • Publish Date: 2023-04-01
  • In this paper, the stainless steel-based lead dioxide (PbO2) electrode with antimony-doped tin dioxide (Sb-SnO2) interlayer was prepared using 316L stainless steel as the substrate, and used for the decolorization of Acid Red G (ARG). The morphology, crystal structure, stability and catalytic performance of the electrode were characterized by scanning electron microscopy (SEM), X-ray diffraction (XRD), enhanced lifetime test, and linear scan test (LSV). Based on this, orthogonal experiments were used to optimize four typical factors (lead ion concentration, temperature, current density and electrodeposition time) that had a strong influence on stability of the electrode. The results showed that the β-PbO2 layer was successfully prepared on the stainless steel substrate with a typical conical structure of β-PbO2 in its morphology. The results of the enhanced lifetime test indicated that the failure mechanism of the stainless steel-based PbO2 electrode was mainly pitting corrosion, which was different from the uniform corrosion of the titanium-based oxide electrode. The LSV test, hydroxyl radical (·OH) yield test and electrocatalytic degradation test were used to demonstrate the better catalytic performance of the stainless steel-based PbO2 electrode, after optimizing the conditions in orthogonal experiments. The successful preparation of stainless steel-based PbO2 electrode is expected to provide a new choice for electrocatalytic oxidation anode materials.
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