PREPARATION OF PHOSPHORUS REMOVAL MATERIAL BY CALCINATION OF WATER TREATMENT PLANT SLUDGE AND RIVER SILT AND ITS PERFORMANCE

JIN Hongyi; Tang Xueping; Zhuang Mazhan; Gong Chunming; Wu Xiaohai; LI Fei; ZHOU Zhenming

doi:10.13205/j.hjgc.202308027

Volume 41 Issue 8

Aug. 2023

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Article Navigation > ENVIRONMENTAL ENGINEERING > 2023 > 41(8): 209-217

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JIN Hongyi, Tang Xueping, Zhuang Mazhan, Gong Chunming, Wu Xiaohai, LI Fei, ZHOU Zhenming. PREPARATION OF PHOSPHORUS REMOVAL MATERIAL BY CALCINATION OF WATER TREATMENT PLANT SLUDGE AND RIVER SILT AND ITS PERFORMANCE[J]. ENVIRONMENTAL ENGINEERING , 2023, 41(8): 209-217. doi: 10.13205/j.hjgc.202308027

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PREPARATION OF PHOSPHORUS REMOVAL MATERIAL BY CALCINATION OF WATER TREATMENT PLANT SLUDGE AND RIVER SILT AND ITS PERFORMANCE

doi: 10.13205/j.hjgc.202308027

1. College of Civil Engineering, Huaqiao University, Xiamen 361021, China;
2. Xiamen Institute of Environmental Science, Xiamen 361021, China;
3. CCCC First Highway Xiamen Engineering Co., Ltd., Xiamen 361000, China

Received Date: 2022-11-28
Available Online: 2023-11-15

Abstract

Abstract

In order to explore a new way of resource utilization of water treatment plant sludge and river silt, this paper studied the feasibility of preparing phosphorus removal material (C-WTPS/RS) by calcination of their mixture. The mixing ratio of raw materials and calcination temperature were optimized, the main influencing factors of phosphorus removal performance of C-WTPS/RS were analyzed, and the adsorption mechanism of C-WTPS/RS for phosphorus removal was discussed. The results of optimization experiments showed that when the calcination time was 1h, the optimal mixing ratio (dry weight) of WTPS to RS was 5∶5, the optimal calcination temperature was 600 ℃, then the phosphorus adsorption capacity of C-WTPS/RS reached 0.707 mg/g (with an initial concentration of orthophosphate of 2 mg/L), and C-WTPS/RS did not release ammonia nitrogen and organic matter into the water. The phosphorus adsorption capacity of C-WTPS/RS increased with the increase in dosage. When the reaction temperature was within 15 to 25 ℃, the phosphorus adsorption capacity of C-WTPS/RS increased with the increase of the reaction temperature. When the reaction temperature was within 25 to 35 ℃, the phosphorus adsorption capacity of C-WTPS/RS was less affected by the reaction temperature. The phosphorus adsorption capacity of WTPS/RS was stable when the solution pH was 3~9, and the phosphorus adsorption capacity of WTPS/RS showed a downward trend when the solution pH was higher than 9. SO₄^2-, Cl^- and NO₃^- had little effect on the phosphorus adsorption of C-WTPS/RS, and HCO₃^- had a certain inhibitory effect on the phosphorus removal performance of C-WTPS/RS. Thermodynamic analysis showed that the adsorption of phosphorus by C-WTPS/RS was a spontaneous endothermic process, The phosphorus adsorption kinetics of C-WTPS/RS was more consistent with the quasi-second-order kinetic model, and the adsorption isotherms were consistent with the Langmuir adsorption isotherm model, indicating that the phosphorus removal process by C-WTPS/RS was mainly monolayer chemisorption, accompanied by physical adsorption, and the theoretical saturated phosphorus adsorption capacity was 6.26 mg/g.
- phosphorus removal,
- water treatment plant sludge,
- river sludge,
- calcination,
- adsorption

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References(29)

References

[1]	SOK K,YUN H P,JAE B L,et al.Phosphorus adsorption behavior of industrial waste biomass-based adsorbent,esterified polyethylenimine-coated polysulfone-Escherichia coli biomass composite fibers in aqueous solution[J].Journal of Hazardous Materials,2020,400:123217.
[2]	YANG B,LIN H,Bartlett S L,et al.Partitioning and transformation of organic and inorganic phosphorus among dissolved,colloidal and particulate phases in a hypereutrophic freshwater estuary[J].Water Research,2021,196:117025.
[3]	尹炜,王超,张洪,等.长江流域总磷问题思考[J].人民长江,2022,53(4):44-52.
[4]	宋勇军,戚菁,刘立恒,等.程海湖夏冬季浮游植物群落结构与富营养化状况研究[J].环境科学学报,2019,39(12):4106-4113.
[5]	BROWN P,IKUMA K,ONG S K,et al.Biological phosphorus removal and its microbial community in a modified full-scale activated sludge system under dry and wet weather dynamics[J].Water Research,2022,217:118338.
[6]	MA H,GAO X L,CHEN Y H,et al.Fe(Ⅱ) enhances simultaneous phosphorus removal and denitrification in heterotrophic denitrification by chemical precipitation and stimulating denitrifiers activity[J].Environmental Pollution,2021,287:118338.
[7]	MA G S,CHEN J.Removal effects on nitrogen,phosphorus and COD in water body of Shanghu Lake ecological wetland in Taihu Lake watershed[J].Procedia Environmental Sciences,2011,10:2665-2670.
[8]	REN Y,ZHENG W,DUAN X,et al.Recent advances in electrochemical removal and recovery of phosphorus from water:a review[J].Environmental Functional Materials,2022,1(1):10-20.
[9]	ZHENG W,SUN Y,GU Y.Catalysis and adsorption of Zr-doped Fe₃O₄ nanoparticles provide a new strategy for diazinon removal and phosphorus recovery from aqueous solution[J].Journal of Environmental Chemical Engineering,2022,10(2):107153.
[10]	仇付国,孙瑶,陈丽霞,等.给水厂铝污泥特性分析及吸附氮磷性能试验[J].环境工程,2016,34(4):54-59.
[11]	朱元中,陶红,顾竹珺,等.底泥制备免烧结多孔材料对原水中磷的去除[J].净水技术,2017,36(2):78-82.
[12]	刘啟迪,周真明,张红忠,等.煅烧改性净水厂污泥制备除磷材料工艺参数优化[J].华侨大学学报(自然科学版),2018,39(1):51-56.
[13]	WU H F,WANG J P,DUAN E G,et al.Study on the preparation of granular alum sludge adsorbent for phosphorus removal[J].Water Sci Technol,2019,79(12):2378-2386.
[14]	肖继波,陈玉莹,瞿倩,等.高效除磷型底泥陶粒对水体中磷的去除特性[J].环境污染与防治,2018,40(10):1122-1125.
[15]	国家环境保护总局.水和废水监测分析方法[M].4版.北京:中国环境科学出版社,2002.
[16]	LIU C J,LI Y Z,LUAN Z K,et al.Adsorption removal of phosphate from aqueous solution by active red mud[J].Journal of Environmental Sciences,2007,19(10):1166-1170.
[17]	TANTAWY M A.Characterization and pozzolanic properties of calcined alum sludge[J].Materials Research Bulletin,2015,61(1):415-421.
[18]	向速林,龚聪远,楚明航,等.Mg-Al-Cl^-LDH对磷的吸附性能及其机理[J].环境工程学报,2021,15(12):3865-3874.
[19]	李迎春,董良飞,仝驰,等.稀土改性凹凸棒土对低浓度磷的吸附性能[J].环境工程学报,2021,15(10):3214-3222.
[20]	ZHANG S P,DING J,TIAN D Y.Incorporation of MIL-101 (Fe or Al) into chitosan hydrogel adsorbent for phosphate removal:performance and mechanism[J].Journal of Solid State Chemistry,2022,306:122709.
[21]	简志强,周高婷,龚斌,等.微米零价铁去除磷酸盐效果与机理研究[J].环境工程技术学报,2021,11(5):927-934.
[22]	ASWIN K I,JEYASEELAN A,VISWANATHAN N,et al.Fabrication of lanthanum linked trimesic acid as porous metal organic frameworks for effective nitrate and phosphate adsorption[J].Journal of Solid State Chemistry,2021:122446.
[23]	熊承旺,段宁,陶敏,等.氢氧化镧大孔水凝胶对磷的吸附特征研究[J].环境科学与技术,2021,44(9):58-63.
[24]	段宁,吴依远,张银凤,等.硅藻土/沸石复合颗粒吸附材料脱氮除磷的吸附动力学及热力学分析[J].硅酸盐通报,2014,33(12):3151-3158.
[25]	王新宇,张卫民,王玉罡,等.活性炭负载纳米零价铁-羟基磷灰石的制备及其对Mn(Ⅱ)的吸附性能[J].有色金属(冶炼部分),2022(11):97-104.
[26]	曾凤美,孙丰文,孙恩惠,等.Fe₂O₃/PC功能化复合多孔炭材料的制备及除磷机理[J].环境科学学报,2021,41(9):3487-3496.
[27]	郑凯,蒋善庆,武福平,等.给水厂污泥陶粒制备及其对氮磷吸附研究[J].环境污染与防治,2020,42(1):35-38.
[28]	耿雅妮,任雪盈,巨龙,等.热改性铝污泥吸附除磷的动力学和热力学研究[J].应用化工,2018,47(7):1377-1381.
[29]	刘艳芳,高玮,尹思婕,等.铁、锆改性生物炭对水中磷的吸附特性及机理研究[J].工业水处理,2022,42(11):153-161.

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