Source Journal of CSCD
Source Journal for Chinese Scientific and Technical Papers
Core Journal of RCCSE
Included in JST China
Volume 41 Issue 10
Oct.  2023
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SHAN Changgong, WANG Wei, XIE Yu, WU Peng, ZENG Xiangyu, ZHU Qianqian, LIANG Bin, ZHA Lingling, LIU Cheng. TOTAL COLUMN CONCENTRATION OBSERVATION OF CO2 AND CH4 BY A PORTABLE GROUND-BASED FTIR SPECTROMETER[J]. ENVIRONMENTAL ENGINEERING , 2023, 41(10): 14-19,140. doi: 10.13205/j.hjgc.202310003
Citation: SHAN Changgong, WANG Wei, XIE Yu, WU Peng, ZENG Xiangyu, ZHU Qianqian, LIANG Bin, ZHA Lingling, LIU Cheng. TOTAL COLUMN CONCENTRATION OBSERVATION OF CO2 AND CH4 BY A PORTABLE GROUND-BASED FTIR SPECTROMETER[J]. ENVIRONMENTAL ENGINEERING , 2023, 41(10): 14-19,140. doi: 10.13205/j.hjgc.202310003

TOTAL COLUMN CONCENTRATION OBSERVATION OF CO2 AND CH4 BY A PORTABLE GROUND-BASED FTIR SPECTROMETER

doi: 10.13205/j.hjgc.202310003
  • Received Date: 2023-07-20
    Available Online: 2023-12-26
  • Ground-based Fourier transform infrared spectroscopy (FTIR) has become an important technology for monitoring greenhouse gas column concentration, due to its high spatiotemporal resolution and sensitivity to changes in surface atmospheric concentrations. This paper was based on the solar spectrum observed by a portable Fourier transform infrared spectrometer (EM27/SUN) to retrieve the CO2 and CH4 total column concentrations in Beijing. By comparing with high-resolution FTIR observation, the accuracy and reliability of EM27/SUN observation were verified. At the same time, the observation accuracy was calculated by using the concentration results of CO2 and CH4 column observations at noon. The accuracy of CO2 was 0.16×10-6, and the accuracy of CH4 was 1.4×10-9. Finally, the time series changes of CO2 and CH4 were presented, and the variation of CO2 and CH4 were more consistent during the observation period. This study shows that portable FTIR can accurately determine CO2 and CH4 column concentration.
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  • [1]
    ALLEN, M R, DUBE O P, SOLECKI W, et al.Framing and Context.In:Global Warming of 1.5℃[R].An IPCC Special Report on the Impacts of Global Warming of 1.5℃ Above Pre-Industrial Levels and Related Global Greenhouse Gas Emission Pathways, in the Context of Strengthening the Global Response to the Threat of Climate Change, Sustainable Development, and Efforts to Eradicate Poverty.2018.
    [2]
    蔡兆男, 成里京, 李婷婷, 等.碳中和目标下的若干地球系统科学和技术问题分析[J].中国科学院院刊, 2021, 36(5):602-613.
    [3]
    IPCC, 2021:Climate Change 2021:The Physical Science Basis.Contribution of Working Group I to the Sixth Assessment Report of the Intergovernmental Panel on Climate Change[R].Cambridge University Press, Cambridge and New York:2391.doi: 10.1017/9781009157896.
    [4]
    FENG L, PALMER P I, BÖSCH H, et al.Consistent regional fluxes of CH4 and CO2 inferred from GOSAT proxy XCH4:XCO2 retrievals, 2010-2014[J].Atmos Chem Phys, 2017, 17:4781-4797.
    [5]
    WUNCH D, WENNBERG P O, OSTERMAN G, et al.Comparisons of the Orbiting Carbon Observatory-2(OCO-2) XCO2 measurements with TCCON[J].Atmos Meas Tech Discuss, 2017, doi:10.5194/amt-2016-227, in review.
    [6]
    de MAZIÈRE M, THOMPSON A M, KURYLO M J, et al.The network for the detection of atmospheric composition change (NDACC):history, status and perspectives[J].Atmospheric Chemistry and Physics, 2018, 18(7):4935-4964.
    [7]
    POLYAKOV A V, TIMOFEYEV Y M, Virolainen Y A, et al.Ground-based measurements of the total column of freons in the atmosphere near St.Petersburg (2009-2017)[J].Izvestiya, Atmospheric and Oceanic Physics, 2018, 54(5):487-494.
    [8]
    WUNCH D, TOON G C, BLAVIER J F L, et al.The total carbon column observing network[J].Philosophical Transactions of the Royal Society A:Mathematical, Physical and Engineering Sciences, 2011, 369(1943):2087-2112.
    [9]
    刘丹丹, 黄印博, 孙宇松, 等.对流层顶高对拉萨地区温室气体柱浓度反演的影响[J].物理学报, 2020, 69(13):130201.
    [10]
    查玲玲.基于便携式FTIR光谱技术的城市大气CO2和CH4时空分布的研究[D].合肥:合肥学院, 2022.
    [11]
    FREY M.Characterisation and Application of Portable Solar Absorption Spectrometers for the Detection of Greenhouse Gas Emissions from Regional Anthropogenic Sources[D].Karlsruhe:Karlsruhe Institute for Technolgy (KIT), 2018.
    [12]
    ZHOU M, NI Q, CAI Z, et al.Ground-based atmospheric CO2, CH4, and CO column measurements at golmud in the Qinghai-Tibetan Plateau and comparisons with TROPOMI/S5P Satellite Observations[J].Advances in Atmospheric Sciences, 2023, 40(2):223-234.
    [13]
    TU Q, HASE F, BLUMENSTOCK T, et al.Intercomparison of atmospheric CO2 and CH4 abundances on regional scales in boreal areas using copernicus atmosphere monitoring service (CAMS) analysis, collaborative carbon column observing network (COCCON) spectrometers, and sentinel-5 precursor satellite observations[J] Atmos Meas Tech, 2020, 13:4751-4771.
    [14]
    GORDON I E, ROTHMAN L S, HARGREAVES R J, et al.The HITRAN2020 molecular spectroscopic database[J].Journal of Quantitative Spectroscopy and Radiative Transfer, 2022, 277:107949.
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