RESPONSE SURFACE OPTIMIZATION OF GRAPHENE OXIDE PREPARATION USING MUNICIPAL SLUDGE AS THE SUBSTRATE

ZHANG Tingting; KONG Xiangqing; FU Ying; ZHANG Zhenbin; ZHAO Fei; YUAN Dan; ZHOU Yuanming

doi:DOI:10.13205/j.hjgc.202207004

Volume 40 Issue 7

Sep. 2022

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Article Navigation > ENVIRONMENTAL ENGINEERING > 2022 > 40(7): 25-30,51

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ZHANG Tingting, KONG Xiangqing, FU Ying, ZHANG Zhenbin, ZHAO Fei, YUAN Dan, ZHOU Yuanming. RESPONSE SURFACE OPTIMIZATION OF GRAPHENE OXIDE PREPARATION USING MUNICIPAL SLUDGE AS THE SUBSTRATE[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(7): 25-30,51. doi: DOI:10.13205/j.hjgc.202207004

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RESPONSE SURFACE OPTIMIZATION OF GRAPHENE OXIDE PREPARATION USING MUNICIPAL SLUDGE AS THE SUBSTRATE

doi: DOI:10.13205/j.hjgc.202207004

1. School of Chemical and Environmental Engineering, Liaoning University of Technology, Jinzhou 121001, China;
2. Songshan Lake Materials Laboratory, Dongguan 523000, China;
3. Huawei (Liaoning) Resources and Environment Technology Co., Ltd, Jinzhou 121000, China;
4. Jinzhou City Product Quality Supervision and Inspection Institute (National Photovoltaic Material Quality Supervision and Inspection Center), Jinzhou 121001, China

Received Date: 2021-07-26
Available Online: 2022-09-02

Abstract

Abstract

Municipal sludge is rich in organic matter,which can provide carbon source for the preparation of graphene oxide (GO).In this paper,GO was prepared from municipal sludge by modified Hummers method.Response surface methodology (RSM) was used to optimize GO preparation conditions,including toner dosage,potassium permanganate dosage,concentrated sulfuric acid dosage,and ultrasonic time,based on single factor experiment.The optimized preparation conditions of GO-based on municipal sludge were carbon powder of 3.22 g,potassium permanganate of 4.12 g,concentrated sulfuric acid of 22.63 mL and ultrasonic time of 7.61 h.Scanning electron microscopy and infrared spectroscopy analysis showed that GO prepared under the optimum experimental conditions had obvious lamellar structure,with O-H (hydroxyl) characteristic peaks at about 3400 cm^-1 and 1400 cm^-1,C=O (carbonyl) characteristic peaks at about 1700 cm^-1,and C-O (epoxy) characteristic peaks at about 1200 cm^-1.It was consistent with the properties of GO prepared with the traditional materials.Thus,a new direction and theoretical basis were provided for the utilization of municipal sludge by preparing GO.
- municipal sludge,
- graphene oxide,
- response surface methodology,
- resource utilization

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References

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