Source Jouranl of CSCD
Source Journal of Chinese Scientific and Technical Papers
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DU Xiaoli, CHI Zhongwen, YIN Zijie, ZHAO Meng. ATTENUATION ON CONTROL EFFECT OF HEAVY METALS IN RUNOFF BY PERMEABLE BRICK DURING THE WHOLE PROCESS OF BLOCKAGE[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(7): 1-8. doi: DOI:10.13205/j.hjgc.202207001
Citation: YANG Zhenxing, XIE Wenyu, LI Dehao, YAN Guangxu, GUO Shaohui. SYNTHESIS,CHARACTERIZATION AND PERFORMANCE EVALUATION OF Ru-Ir ELECTRODE FOR ELECTROCATALYTIC TREATMENT FOR AMMONIA-NITROGEN WASTEWATER WITH HIGH CHLORIDE CONTENT[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(7): 165-171. doi: DOI:10.13205/j.hjgc.202207024

SYNTHESIS,CHARACTERIZATION AND PERFORMANCE EVALUATION OF Ru-Ir ELECTRODE FOR ELECTROCATALYTIC TREATMENT FOR AMMONIA-NITROGEN WASTEWATER WITH HIGH CHLORIDE CONTENT

doi: DOI:10.13205/j.hjgc.202207024
  • Received Date: 2021-08-31
    Available Online: 2022-09-02
  • In this paper,the effect of the molar ratios of ruthenium (Ru)-iridium (Ir) on the microstructure,chemical properties,electrochemical performance,and denitrification performance of high ammonia-chloride wastewater were investigated.The results illustrated that Ru-Ir solid solution was a rutile crystal with uniform grain distribution and tight connection.The electrochemical performances of the electrodes were tested by electrochemical techniques.And the electrochemical performance of the Ru-Ir electrode first increased and then decreased with the increase of the molar ratio of Ir.The electrochemical properties of Ru2/3Ir1/3O2 electrodes were the best when the molar ratio of Ru-Ir was 2:1.The chlorine evolution potential,corrosion current density,and conductivity of Ru2/3Ir1/3O2 electrode were 0.998,0.755,and 1.816 times those of RuO2,respectively.In the removal process of ammonia-nitrogen in high chloride ammonia-nitrogen simulated wastewater,the electrode with the best removal effect of ammonia-nitrogen was Ru2/3Ir1/3O2 electrode,and when the current was 0.5 A,the ammonia-nitrogen removal rate could reach 75.2% in 50 minutes.This paper proved that electrocatalytic technology could effectively treat high chloride ammonia-nitrogen wastewater.
  • [1]
    周银芳. SBR工艺处理高含盐采油废水试验研究[D].西安:长安大学, 2010.
    [2]
    RIBEIRO J, ALVES P D, DE Andrade A R. Effect of the preparation methodology on some physical and electrochemical properties of Ti/Ir<i>xSn(1-x)O2 materials[J]. Journal of materials science, 2007,42(22):9293-9299.
    [3]
    ESCALANTE G I, DURON T S, CRUZ J, et al. Electrochemical characterization of IrO2-Pt and RuO2-Pt mixtures as bifunctional electrodes for unitized regenerative fuel cells[J]. Journal of New Matetials for Electrochemical Systems, 2010,13:227-233.
    [4]
    CRUZ J, HERNÁNDEZ A R, GUERRA B M, et al. Electrochemical evaluation of a Ir-Ru binary oxide for oxygen evolution reaction[J]. International Journal of Electrochemical Science, 2012,7(9):7866-7876.
    [5]
    CRUZ J, BAGLIO V, SIRACUSANO S, et al. Nanosized IrO2 electrocatalysts for oxygen evolution reaction in an SPE electrolyzer[J]. Journal of Nanoparticle Research, 2011,13(4):1639-1646.
    [6]
    AUDICHON T, MAYOUSSE E, MORISSET S, et al. Electroactivity of RuO2-IrO2 mixed nanocatalysts toward the oxygen evolution reaction in a water electrolyzer supplied by a solar profile[J]. International Journal of Hydrogen Energy, 2014,39(30):16785-16796.
    [7]
    MENZEL N, ORTEL E, METTE K, et al. Dimensionally stable Ru/Ir/TiO2-anodes with tailored mesoporosity for efficient electrochemical chlorine evolution[J]. ACS Catalysis, 2013,3(6):1324-1333.
    [8]
    SANTANA M H P, DE F L A. Oxygen and chlorine evolution on RuO2+TiO2+CeO2+Nb2O5 mixed oxide electrodes[J]. Electrochimica Acta, 2006,51(17):3578-3585.
    [9]
    WANG S W, XU H L, YAO P D, et al. Ti/RuO2-IrO2-SnO2-Sb2O5 anodes for Cl2 evolution from seawater[J]. Electrochemistry, 2012,80(7):507-511.
    [10]
    RUAN Y, LU C, GUO X, et al. Electrochemical treatment of recirculating aquaculture wastewater using a Ti/RuO2-IrO2 anode for synergetic total ammonia nitrogen and nitrite removal and disinfection[J]. Transactions of the ASABE, 2016,59(6):1831-1840.
    [11]
    WANG H, YANG Y, LIU X, et al. Decomposition of ammonia nitrogen from biologically pretreated coking wastewater with electrochemical three-dimensional Ti/RuO2/IrO2 electrodes[J]. Nature Environment and Pollution Technology, 2016,15(3):881-886.
    [12]
    HE S L, HUANG Q, ZHANG Y, et al. Investigation on direct and indirect electrochemical oxidation of ammonia over Ru-Ir/TiO2 anode[J]. Industrial&Engineering Chemistry Research, 2015,54(5):1447-1451.
    [13]
    WANG B, HOU S Z, HAN Y, et al. Recent status of development of metal oxide coated anode for antifouling by electrolyzing seawater[J]. Development&Application of Materials, 1998,13(1):42.
    [14]
    LI L, LIU Y. Ammonia removal in electrochemical oxidation:mechanism and pseudo-kinetics[J]. Journal of Hazardous Materials, 2009,161(2/3):1010-1016.
    [15]
    WANG J. Preparation of the ordered spherical Ru-RuO2 and electrocatalysis toward chlorine evolution reaction[J]. International Journal of Electrochemical Science, 2019:10187-10197.
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