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汾渭平原PM2.5-O3复合污染特征及输送路径分析

宋晓伟 孔媛 郝永佩 朱晓东 张晓龙 韩越梅 高宁馨

宋晓伟, 孔媛, 郝永佩, 朱晓东, 张晓龙, 韩越梅, 高宁馨. 汾渭平原PM2.5-O3复合污染特征及输送路径分析[J]. 环境工程, 2025, 43(12): 129-140. doi: 10.13205/j.hjgc.202512015
引用本文: 宋晓伟, 孔媛, 郝永佩, 朱晓东, 张晓龙, 韩越梅, 高宁馨. 汾渭平原PM2.5-O3复合污染特征及输送路径分析[J]. 环境工程, 2025, 43(12): 129-140. doi: 10.13205/j.hjgc.202512015
SONG Xiaowei, KONG Yuan, HAO Yongpei, ZHU Xiaodong, ZHANG Xiaolong, HAN Yuemei, GAO Ningxin. Characteristics and transport pathways of PM2.5-O3 compound pollution in Fenwei Plain[J]. ENVIRONMENTAL ENGINEERING , 2025, 43(12): 129-140. doi: 10.13205/j.hjgc.202512015
Citation: SONG Xiaowei, KONG Yuan, HAO Yongpei, ZHU Xiaodong, ZHANG Xiaolong, HAN Yuemei, GAO Ningxin. Characteristics and transport pathways of PM2.5-O3 compound pollution in Fenwei Plain[J]. ENVIRONMENTAL ENGINEERING , 2025, 43(12): 129-140. doi: 10.13205/j.hjgc.202512015

汾渭平原PM2.5-O3复合污染特征及输送路径分析

doi: 10.13205/j.hjgc.202512015
基金项目: 

国家自然科学基金项目(72104132);教育部人文社会科学基金项目(21YJCZH136); 山西省社科联重点课题研究项目 (SSKLZDKT2024089);2024年山财学者学术拔尖骨干人才科研项目(BY-Z01059)

详细信息
    作者简介:

    宋晓伟(1987—),男,博士,副教授, 主要研究方向为大气污染控制模拟。xiaoweicool9418@126.com

    通讯作者:

    宋晓伟(1987—),男,博士,副教授, 主要研究方向为大气污染控制模拟。xiaoweicool9418@126.com

Characteristics and transport pathways of PM2.5-O3 compound pollution in Fenwei Plain

  • 摘要: 随着PM2.5和O3复合污染现象频发,其危害性逐渐显现。基于此,开展大气污染防控重点区域之一的汾渭平原PM2.5-O3复合污染时空分布特征及其与气象因素关联性研究。结果显示:1)2014—2021年汾渭平原PM2.5年均浓度呈下降趋势,PM2.5污染集中分布于西安市、洛阳市和临汾市,O3污染却表现出波动上升的趋势,O3污染分布集中于汾渭平原东南部城市洛阳市、三门峡市、运城市和临汾市;汾渭平原PM2.5浓度日变化特征表现出“U”型趋势,而O3浓度日均值变化呈“倒U”型特征。2)研究期间,汾渭平原各年份PM2.5-O3复合污染天数和PM2.5单污染天数均出现下降趋势,年内4至10月出现复合污染天数较为集中,复合污染天数空间分布呈由东南角向两翼递减的特征,而汾渭平原PM2.5和O3相关系数总体呈“夏正冬负”趋势。3)汾渭平原PM2.5-O3的复合污染易出现于气温为13~29.7 ℃,相对湿度为35%~75%,偏东风,风速为1.5~3.1 m/s的气象条件下。4)后向轨迹聚类分析发现,汾渭平原西南部城市复合污染受来自于东南方向短路径气流影响显著,中部地区城市气流输送路径来自新疆和内蒙古部分区域,而来自西北和东北方向的长距离气流则影响东南部及北部城市。
  • [1] LU X,ZHANG S J,XING J,et al. Progress of air pollution control in China and its challenges and opportunities in the ecological civilization era[J]. Engineering,https://doi.org/10.1016/j.eng.2020.03.014.
    [2] KONG X R,CHEN M,CHEN H R,et al. Variation characteristics and influence factors of surface ozone concentration in Lanzhou in 2018-2019[J]. Environmental Engineering,2022,40(7):69-75. 孔祥如,陈敏,陈恒蕤,等. 2018—2019年兰州市近地面臭氧浓度变化特征及其影响因素分析[J]. 环境工程,2022,40(7):69-75.
    [3] JIANG H,GAO J,LI H,et al. Preliminary research on theoretical framework of cooperative control of air pollution in China[J]. Research of Environmental Sciences,2022,35(3):601-610. 姜华,高健,李红,等. 我国大气污染协同防控理论框架初探[J]. 环境科学研究,2022,35(3):601-610.
    [4] WANG F Y,QIU X H,CAO J Y,et al. Policy-driven changes in the health risk of PM2.5 and O3 exposure in China during 2013—2018[J]. Science of the Total Environment,2021,757,143775.
    [5] ZHOU J,FU S H,PENG L,et al. Effect of ozone and PM2.5 on chronic obstructive pulmonary disease deaths and the effect modification by the air temperature[J]. China Environmental Science,2021,41(12):5904-5911. 周骥,付世华,彭丽,等. 臭氧和 PM2.5对慢阻肺死亡影响及气温修饰效应[J]. 中国环境科学,2021,41(12):5904-5911.
    [6] CHEN J,PENG J L,XU Y S. Spatiotemporal distribution and health impacts of PM2.5 and O3 in Beijing,from 2014 to 2020[J]. Environmental Science,2021,42(9):4071-4082. 陈菁,彭金龙,徐彦森. 北京市2014—2020年PM2.5和O3时空分布与健康效应评估[J]. 环境科学,2021,42(9):4071-4082.
    [7] ZHANG H,JIANG H,GAO J,et al. Formation mechanism and management strategy of cooperative control of PM2.5 and O3[J]. Research of Environmental Sciences,2022,35(3):611-620. 张涵,姜华,高健,等. PM2.5与臭氧污染形成机制及协同防控思路[J]. 环境科学研究,2022,35(3):611-620.
    [8] WANG P,ZHU S Q,ZHANG M Y,et al. Atmospheric oxidation capacity and its contribution to secondary pollutants formation[J]. Chinese Science Bulletin,2022,67(18):2069-2078. 王芃,朱盛强,张梦媛,等. 大气氧化性及其对二次污染物形成的贡献[J]. 科学通报,2022,67(18):2069-2078.
    [9] ZHANG X Y,XU X D,DING Y H,et al. The impact of meteorological changes from 2013 to 2017 on PM2.5 mass reduction in key regions in China[J]. Science China Earth Sciences,2020,50(4):483-500. 张小曳,徐祥德,丁一汇,等. 2013—2017年气象条件变化对中国重点地区 PM2.5质量浓度下降的影响[J]. 中国科学:地球科学,2020,50(4):483-500.
    [10] WANG Z S,ZHANG D W,Li Y T,et al. Different air pollution situations of O3 and PM2.5 during summer in Beijing[J]. Environmental Science,2016,37(3):807-815. 王占山,张大伟,李云婷,等. 北京市夏季不同O3和PM2.5污染状况研究[J]. 环境科学,2016,37(3):807-815.
    [11] ZHAO S T,WANG L T,QI M Y,et al. Study on the characteristics and mutual influence of PM2.5-O3 complex pollution in Handan[J]. Acta Scientiae Circumstantiae,2021,41(6):2250-2261. 赵淑婷,王丽涛,齐孟姚,等. 邯郸市 PM2.5-O3复合污染特征及相互影响研究[J]. 环境科学学报,2021,41(6):2250-2261.
    [12] DAI H B,ZHU J,LIAO H,et al. Co-occurrence of ozone and PM2.5 pollution in the Yangtze River Delta over 2013—2019 spatiotemporal distribution and meteorological conditions[J]. Atmospheric Research,2021,249,105363.
    [13] NIU X X,ZHONG Y M,YANG L,et al. Spatiotemporal evolution characteristics of PM2.5-O3 compound pollution in Chinese cities from 2015 to 2020[J]. Environmental Science,2023,44(4):1830-1840. 牛笑笑,钟艳梅,杨璐,等. 2015—2020年中国城市PM2.5-O3复合污染时空演变特征[J]. 环境科学,2023,44(4):1830-1840.
    [14] SONG X H,YAN L,LIU W,et al. Spatiotemporal distribution characteristics of co-pollution of PM2.5 and Ozone over BTH with surrounding area from 2015 to 2021[J]. Environmental Science,2023,44(4):1841-1851. 宋小涵,燕丽,刘伟,等. 2015—2021 年京津冀及周边地区 PM2.5和臭氧复合污染时空特征分析[J]. 环境科学,2023,44(4):1841-1851.
    [15] LIU M H,YU C T,FANG X Y,et al. Analysis of PM2.5-O3 compound pollution characteristics and meteorological causes in Henan Province from 2014 to 2020[J]. Research of Environmental Sciences,2023,36(2):285-293. 刘淼晗,于宸涛,房祥玉,等. 2014—2020年河南省PM2.5-O3复合污染特征及气象成因分析[J]. 环境科学研究,2023,36(2):285-293.
    [16] HE Y P,LI L,WANG H L,et al. A cold front induced co-occurrence of O3 and PM2.5 pollution in a Pearl River Delta city:Temporal variation,vertical structure,and mechanism[J]. Environmental Pollution,2022,306,DOI:10.1016/j.envpol.2022.119464.
    [17] XIAO Z M,XU H,GAO J Y,et al. Characteristics and Sources of PM2.5-O3 Compound Pollution in Tianjin[J]. Environmental Science,2022,43(3):1140-1150. 肖致美,徐虹,高璟贇,等. 天津市PM2.5-O3复合污染特征及来源分析[J]. 环境科学,2022,43(3):1140-1150.
    [18] ZHANG Z D,SHAO T J,HUANG X G,et al. Characteristics and potential sources of PM2.5 pollution in Beijing-Tianjin-Hebei region in 2017[J]. Environmental Engineering,2020,38(2):99-109. 张忠地,邵天杰,黄小刚,等. 2017年京津冀地区PM2.5污染特征及潜在来源分析[J]. 环境工程,2020,38(2):99-109.
    [19] BIAN J T,HUANG L,LI H L,et al. Evaluation of the effectiveness of multiple emission reduction pathways during a concurrent PM2.5 and ozone pollution in Shanghai[J]. Research of Environmental Sciences,2023,36(2):314-324. 卞锦婷,黄凌,李红丽,等. 上海市PM2.5和臭氧复合污染期多路径减排效果评估[J]. 环境科学研究,2023,36(2):314-324.
    [20] YU C,ZHANG Y X,CHEN W. The transport pathways and potential source regions of PM2.5 in Yinchuan,China[J]. China Environmental Science,2021,41(7):3055-3065. 余创,张玉秀,陈伟. 银川市PM2.5的输送路径及潜在源解析[J]. 中国环境科学,2021,41(7):3055-3065.
    [21] SONG X W,HAO Y P,ZHU X D,et al. Variations in Ozone pollution and their meteorological influences and transmission sources in Linfen City of China[J]. China Environmental Science,2022,42(8):3626-3634. 宋晓伟,郝永佩,朱晓东,等. 临汾市臭氧污染变化特征、气象影响及输送源分析[J]. 中国环境科学,2022,42(8):3626-3634.
    [22] ZHANG G,XU H H,QI B,et al. Characterization of atmospheric trace gases and particulate matter in Hangzhou,China[J]. Atmospheric Chemistry and Physics,2018,18(3):1705-1728.
    [23] ZHAO H,ZHENG Y F,LI C. Spatiotemporal distribution of PM2.5 and O3 and their interaction during the summer and winter seasons in Beijing,China[J]. Sustainability,2018,10(12):4519.
    [24] QIN M M,HU A Q,MAO J J,et al. PM2.5 and O3 relationships affected by the atmospheric oxidizing capacity in the Yangtze River Delta,China[J]. Science of the Total Environment,2022,810:152268.
    [25] HUA C,JIANG Q,CHI X Y,et al. Meteorological characteristics of PM2.5-O3 air combined pollution in central and eastern China in the summer half years of 2015—2020[J]. Research of Environmental Sciences,2022,35(3):650-658. 花丛,江琪,迟茜元,等. 我国中东部地区2015—2020年夏半年PM2.5和臭氧复合污染气象特征分析[J]. 环境科学研究,2022,35(3):650-658.
    [26] ZHANG Y J,LEI R Y,CUI S J,et al. Spatiotemporal trends and impact factors of PM2.5 and O3 pollution in major cities in China during 2015—2020[J]. Chinese Science Bulletin,2022,67(18):2029-2042. 张运江,雷若媛,崔世杰,等. 2015—2020年我国主要城市PM2.5和O3污染时空变化趋势和影响因素[J]. 科学通报,2022,67(18):2029-2042.
    [27] ZHANG R T,CHEN C M,WU H C,et al. Research on the impact of“coal-to-electricity” policy on the improvement of PM2.5 concentration in Beijing-Tianjin-Hebei region[J]. China Environmental Science,2022,42(3):1022-1031. 张茹婷,陈传敏,吴华成,等. 京津冀“煤改电”对 PM2.5浓度改善影响研究[J]. 中国环境科学,2022,42(3):1022-1031.
    [28] ZHANG H Y,WANG Y,LU Y L,et al. Identification of ozone pollution control zones and types in China[J]. China Environmental Science,2021,41(9):4051-4059. 张鸿宇,王媛,卢亚灵,等. 我国臭氧污染控制分区及其控制类型识别[J]. 中国环境科学,2021,41(9):4051-4059.
    [29] JIA M W,ZHAO T L,CHENG X H,et al. Inverse relations of PM2.5 and O3 in air compound pollution between cold and hot seasons over an urban area of East China[J]. Atmosphere,2017,8(59). doi:10.3390/atmos8030059.
    [30] PAN W Q,XIAO G J,MENG L X,et al. Characteristics of ozone pollution and analysis of meteorological causes in Hangzhou city[J]. Journal of Chengdu University of Information Technology,2019,34(6):664-670. 潘文琪,肖国杰,孟林夕,等. 杭州市臭氧污染特征及其气象成因分析[J]. 成都信息工程大学学报,2019,34(6):664-670.
    [31] LIU H J,TIAN H Z,ZHANG K,et al. Seasonal variation,formation mechanisms and potential sources of PM2.5 in two typical cities in the Central Plains Urban Agglomeration,China[J]. Science of the Total Environment,2019,657:657-670.
    [32] ZHANG H,YIN S S,BAI L,et al. Establishment and evaluation of anthropogenic black and organic carbon emissions over Central Plain,China[J]. Atmospheric Environment,2020,226:117406.
    [33] MAO Z C,XU J M,YANG D D,et al. Analysis of characteristics and meteorological causes of PM2.5-O3 compound pollution in Shanghai[J]. China Environmental Science,2019,39(7):2730-2738. 毛卓成,许建明,杨丹丹,等. 上海地区 PM2.5-O3复合污染特征及气象成因分析[J]. 中国环境科学,2019,39(7):2730-2738.
    [34] ZHANG Z R,HU M,SHANG D J,et al. The evolution trend and typical process characteristics of atmospheric PM2.5 and O3 pollution in Beijing from 2013 to 2020[J]. Chinese Science Bulletin,2022,67(18):1995-2007. 张子睿,胡敏,尚冬杰,等. 2013—2020年北京大气PM2.5和O3污染演变态势与典型过程特征[J]. 科学通报,2022,67(18):1995-2007.
    [35] XIAO Z M,LI Y,KONG J,et al. Characteristics and meteorological factors of PM2.5-O3 compound pollution in Tianjin[J]. Environmental Science,2022,43(6):2928-2936. 肖致美,李源,孔君,等. 天津市PM2.5-O3复合污染特征及气象影响分析[J]. 环境科学,2022,43(6):2928-2936.
    [36] LI X R,WANG Y S,GUO X Q,et al. Seasonal variation and source apportionment of organic and inorganic compounds in PM2.5 and PM10 particulates in Beijing,China[J]. Journal of Environmental Sciences,2013,25(4):741-750.
    [37] CHEN Y Z,ZHAO D,CHAI F H,et al. Correlation between the atmospheric visibility and aerosol fine particle concentrations in Guangzhou and Beijing[J]. China Environmental Science,2010,30(7):967-971. 陈义珍,赵丹,柴发合,等. 广州市与北京市大气能见度与颗粒物质量浓度的关系[J]. 中国环境科学,2010,30(7):967-971.
    [38] XU K,LIU Z H,HE M Q,et al. Meteorological characteristics of O3 pollution near the ground in summer of Chengdu[J]. Environmental Monitoring in China,2018,34(5):36-45. 徐锟,刘志红,何沐全,等. 成都市夏季近地面臭氧污染气象特征[J]. 中国环境监测,2018,34(5):36-45.
    [39] WANG L,LIU D Y,YAN W L,et al. Spatio-temporal distribution,transport characteristics and synoptic patterns of ozone pollution near surface in Jiangsu province,China[J]. Atmospheric Pollution Research,2022,13(12):101616.
    [40] GONG C,LIAO H,ZHANG L,et al. Persistent ozone pollution episodes in North China exacerbated by regional transport[J]. Environmental Pollution,2020,265:115056.
    [41] LIU H,XIA D S,CHEN H,et al. Simulation analysis of sources and transmission characteristics of air pollutants in Lanzhou city in 2017[J]. Research of Environmental Sciences,2019,32(6):993-1000. 刘慧,夏敦胜,陈红,等. 2017年兰州市大气污染物输送来源及传输特征模拟分析[J]. 环境科学研究,2019,32(6):993-1000.
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  • 收稿日期:  2024-04-17
  • 录用日期:  2024-05-25
  • 修回日期:  2024-05-11
  • 网络出版日期:  2026-01-09

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