ADSORPTION PERFORMANCE OF P-ARSANILIC ACID IN AQUEOUS SOLUTION BY BIOCHAR SUPPORTED MANGANESE FERRATE

LI Pei-pei; ZHOU Yu-zhou; XIANG Yu-jia; ZHOU Yao-yu; ZHU Hong-mei; RONG Xiang-min

doi:10.13205/j.hjgc.202001011

Volume 38 Issue 1

Mar. 2020

Turn off MathJax

Article Contents

Article Navigation > ENVIRONMENTAL ENGINEERING > 2020 > 38(1): 75-79,86

LI Pei-pei, ZHOU Yu-zhou, XIANG Yu-jia, ZHOU Yao-yu, ZHU Hong-mei, RONG Xiang-min. ADSORPTION PERFORMANCE OF P-ARSANILIC ACID IN AQUEOUS SOLUTION BY BIOCHAR SUPPORTED MANGANESE FERRATE[J]. ENVIRONMENTAL ENGINEERING , 2020, 38(1): 75-79,86. doi: 10.13205/j.hjgc.202001011

Citation:

LI Pei-pei, ZHOU Yu-zhou, XIANG Yu-jia, ZHOU Yao-yu, ZHU Hong-mei, RONG Xiang-min. ADSORPTION PERFORMANCE OF P-ARSANILIC ACID IN AQUEOUS SOLUTION BY BIOCHAR SUPPORTED MANGANESE FERRATE[J]. ENVIRONMENTAL ENGINEERING , 2020, 38(1): 75-79,86. doi: 10.13205/j.hjgc.202001011

Citation:

LI Pei-pei, ZHOU Yu-zhou, XIANG Yu-jia, ZHOU Yao-yu, ZHU Hong-mei, RONG Xiang-min. ADSORPTION PERFORMANCE OF P-ARSANILIC ACID IN AQUEOUS SOLUTION BY BIOCHAR SUPPORTED MANGANESE FERRATE[J]. ENVIRONMENTAL ENGINEERING , 2020, 38(1): 75-79,86. doi: 10.13205/j.hjgc.202001011

PDF( 2184 KB)

ADSORPTION PERFORMANCE OF P-ARSANILIC ACID IN AQUEOUS SOLUTION BY BIOCHAR SUPPORTED MANGANESE FERRATE

doi: 10.13205/j.hjgc.202001011

College of Resources and Environment, Hunan Agricultural University, Changsha 410128, China

Received Date: 2019-01-24

Abstract

Abstract

The p-arsanilic acid adsorbent MFB-MCs was prepared by co-precipitation method with vinasse, manganese sulfate monohydrate (MnSO₄·H₂O) and ferric chloride hexahydrate (FeCl₃·6H₂O) as the raw materials. The SEM and TEM analysis and characterization of MFB-MCs were carried out. The effects of initial solution pH, adsorption dose, temperature and time on the adsorption of p-arsanilic acid were investigated. The results showed that MFB-MCs could effectively remove the p-arsanilic acid in aqueous solution; the influences of initial pH on adsorption process of MFB-MCs to p-arsanilic acid in water was greater. With the condition of temperature of 25 ℃, initial solution pH of 2.0, the adsorption dose of 1 g/L, after 1440 minutes adsorption, the removal rate of p-arsanilic acid with initial concentration of 20 mg/L reached 82.27%; the adsorption process of MFB-MCs on p-arsanilic acid conformed to the pseudo-second-order kinetic model, so it was mainly controlled by chemical adsorption. At the same time, the adsorption process conformed to the Freundlich isotherm model, which belonged to multi-layer adsorption process.
- biochar,
- ferrite,
- p-arsanilic acid,
- adsorption

FullText(HTML)

References(17)

References

刘玉坤,郑星,陈勐,等. 铝易拉罐/Fe(Ⅱ)/O₂体系降解对氨基苯胂酸的机理[J]. 环境工程学报,2017,11(3):1417-1422.

何万领,李晓丽,常会庆,等. 不同水平阿散酸粪肥对水稻生长发育及砷积累的影响[J]. 植物营养与肥料学报,2018,24(4):1088-1096.

何万领,李晓丽,杨肖娥,等. 阿散酸在土壤中的降解与形态变化[J]. 环境工程学报,2018,12(1):198-205.

WANG H L, HU Z H, TONG Z L, et al. Effect of arsanilic acid on anaerobic methanogenic process: kinetics, inhibition and biotransformation analysis[J]. Biochemical Engineering Journal,2014,91:179-185.

FISHER D J, YONKOS L T, STAVER K W. Environmental concerns of roxarsone in broiler poultry feed and litter in Maryland, USA[J]. Environmental Science and Technology,2015,49(4):1999-2012.

耿安静,王旭,陈岩,等. 有机胂阿散酸的研究现状及潜在风险[J]. 农产品质量与安全,2017(5):87-91.

CHATTERJEE S, DE S. Adsorptive removal of arsenic from groundwater using chemically treated iron ore slime incorporated mixed matrix hollow fiber membrane[J]. Separation and Purification Technology,2017,179:357-368.

HU Q S, LIU Y L, GU X Y, et al. Adsorption behavior and mechanism of different arsenic species on mesoporous MnFe₂O₄ magnetic nanoparticles[J]. Chemosphere,2017,181:328-336.

JOSHI T P, ZHANG G, JEFFERSON W A, et al. Adsorption of aromatic organo-arsenic compounds by ferric and manganese binary oxide and description of the associated mechanism[J]. Chemical Engineering Journal,2017,309:577-587.

王亚娇. 有机砷对厌氧消化的影响及其吸附去除研究[D].合肥:合肥工业大学,2016.

苏立强,尤嘉,王丽博,等. 阿散酸磁性分子印迹聚合物的制备及其应用[J]. 理化检验(化学分册),2018,54(4):373-378.

李铮,雷鸣. 铁氧体及其复合材料对水体中氨基苯胂酸去除效能的研究[J]. 中国资源综合利用,2018,36(11):11-13.

JUNG K W, LEE S, LEE Y J. Synthesis of novel magnesium ferrite (MgFe₂O₄)/biochar magnetic composites and its adsorption behavior for phosphate in aqueous solutions[J]. Bioresource Technology,2017,245:751-759.

WANG W, DING Z, CAI M, et al. Synthesis and high efficiency methylene blue adsorption of magnetic PAA/MnFe₂O₄ nanocomposites[J]. Applied Surface Science,2015,346:348-353.

ZHENG S, JIANG W J, CAI Y, et al. Adsorption and photocatalytic degradation of aromatic organoarsenic compounds in TiO₂ suspension[J]. Catalysis Today,2014,224:83-88.

LV Y C, ZHANG R S, ZENG S L, et al. Removal of p-arsanilic acid by an amino-functionalized indium-based metal-organic framework: adsorption behavior and synergetic mechanism[J]. Chemical Engineering,2018,339:359-368.

梅向阳,王耀,朱丽云,等. 氨基化锰铁氧体纳米粒子的制备及吸附Pb²⁺和Cd²⁺性能研究[J].化学通报,2019,82(2):144-150.

Relative Articles

Supplements(0)

Cited By

Proportional views