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LU Ping, LIU Kai, YANG Hong-yi, MENG Hong-ju, LIU Ya-lei. REMOVAL OF SO2 AND HCl FROM SIMULATED FLUE GAS BY CEMENT CLINKER[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(12): 128-134. doi: 10.13205/j.hjgc.202112019
Citation: LU Ping, LIU Kai, YANG Hong-yi, MENG Hong-ju, LIU Ya-lei. REMOVAL OF SO2 AND HCl FROM SIMULATED FLUE GAS BY CEMENT CLINKER[J]. ENVIRONMENTAL ENGINEERING , 2021, 39(12): 128-134. doi: 10.13205/j.hjgc.202112019

REMOVAL OF SO2 AND HCl FROM SIMULATED FLUE GAS BY CEMENT CLINKER

doi: 10.13205/j.hjgc.202112019
  • Received Date: 2021-01-02
    Available Online: 2022-03-30
  • Publish Date: 2022-03-30
  • The co-processing of municipal solid waste(MSW) with dry cement kiln has been paid attention all over the world because of its advantages such as high reaction temperature, low renovation cost, good comprehensive treatment performance and no secondary pollution. The removal characteristics of SO2 and HCl by cement clinker in simulated flue gas was investigated at 700~1000 ℃ in a fixed-bed experimental reactor. The adsorption mechanism of SO2 and HCl was discussed on the basis of physiochemical properties of original and spent cement clinker samples. The results indicated that the removal efficiency of SO2 by cement clinker increased rapidly as the reaction temperature increased from 700 ℃ to 1000 ℃, and the maximum unit adsorption capacity of SO2 reached 4.9 mg/g while only SO2 was present in simulated flue gas. The opposite was that the removal efficiency of HCl by cement clinker decreased as reaction temperature increased from 700 ℃ to 1000 ℃, and the corresponding unit adsorption capacity of HCl decreased from 8.40 mg/g to 4.8 mg/g while only HCl was present in the simulated flue gas. The initial adsorption rates of SO2 or HCl were determined by its concentration, and the adsorption rate of HCl was significantly larger than that of SO2. When SO2 and HCl were present in simulated flue gas, the removal performance of HCl by cement clinker decreased slightly, but existing HCl could significantly promote the SO2 removal performance and its adsorption reaction rate, and resulting in the unit adsorption capacity of SO2 at 700 ℃ and 1000 ℃ increased from 1.8 mg/g and 4.9 mg/g to 4.5 mg/g and 7.8 mg/g, respectively. The main reason of above results was the migration of chloride ions in spent cement clinker. These results provide a reference for the industrial application of a new co-processing technology using dry cement clinker to treat municipal solid waste incineration flue gas.
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