Source Journal of CSCD
Source Journal for Chinese Scientific and Technical Papers
Core Journal of RCCSE
Included in JST China
Volume 40 Issue 10
Oct.  2022
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Article Contents
JIANG Yuzhu, HUI Helong, LIU Hongyi, DING Guangchao, LU Wenyi, LI Songgeng. STUDY ON THE EFFECTIVENESS OF TEXTILE DYING SLUDGE BIOCHAR IN TREATING REFRACTORY ORGANIC WASTEWATER[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(10): 32-39. doi: 10.13205/j.hjgc.202210005
Citation: JIANG Yuzhu, HUI Helong, LIU Hongyi, DING Guangchao, LU Wenyi, LI Songgeng. STUDY ON THE EFFECTIVENESS OF TEXTILE DYING SLUDGE BIOCHAR IN TREATING REFRACTORY ORGANIC WASTEWATER[J]. ENVIRONMENTAL ENGINEERING , 2022, 40(10): 32-39. doi: 10.13205/j.hjgc.202210005

STUDY ON THE EFFECTIVENESS OF TEXTILE DYING SLUDGE BIOCHAR IN TREATING REFRACTORY ORGANIC WASTEWATER

doi: 10.13205/j.hjgc.202210005
  • Received Date: 2022-01-16
  • The sludge-based carbon (SC) was prepared from textile dyeing sludge, and the impact of carbonization temperature and reaction time on the adsorption capacity of SC treating refractory industrial wastewater were investigated. Simultaneously the adsorption preference of SC and commercial activated carbon (CAC) was compared and studied. The results indicate that the SC derived from higher carbonization temperature can own more specific surface area, pore volume and deeper graphitization degree which facilitate its adsorption capacity. The SC-900℃ owns more than 90% mesoporous pore volume and it's specific surface area reaches 140.65 m2/g. The chemical oxygen demand (COD) removal rate of SC-900℃ treating coking wastewater and digest filtrate is as effective as 70% that of CAC. Besides, the SC-900℃(89.56%)present superior decolorizing effect than CAC(16.70%)when treating high chromaticity digestion filtrate. The macromolecular pollutants can be rapidly adsorbed by SC, the adsorption equilibrium time of SC-900℃(≤ 120 min) treating digestion filtrate is significantly lower than that of CAC(>24 h); Especially, the humus-like macromolecular compounds containing chromogenic functional groups could be selectively absorbed in the mesoporous (3.8~5.4 nm) of SC. At last, some guidance suggestions for industrialization application of SC to treat refractory industrial wastewater are put forward based on above research results.
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  • [1]
    WEN Q H,CHEN H M,WEI J J,et al. Preparation of nitrogen-doped porous carbon by urea-formaldehyde resin for the construction of membrane adsorption reactor to remove refractory pollutant[J]. Separation and Purification Technology,2021,282:120105.
    [2]
    熊富忠,温东辉. 难降解工业废水高效处理技术与理论的新进展[J]. 环境工程,2021,39(11):1-16.
    [3]
    LI Y H,CHANG F M,HUNAG B,et al. Activated carbon preparation from pyrolysis char of sewage sludge and its adsorption performance for organic compounds in sewage[J]. Fuel,2020,266:117053.
    [4]
    林旭萌,宿程远,黄纯萍,等. 污泥质生物炭对2,4-二氯苯酚的吸附性能[J]. 环境工程,2019,37(8):154-158.
    [5]
    ZHOU H,WEI C H,ZHANG F Z,et al. A comprehensive evaluation method for sludge pyrolysis and adsorption process in the treatment of coking wastewater[J]. Journal of Environmental Management,2019,235:423-431.
    [6]
    LIU H D,XU G R,LI G B. The characteristics of pharmaceutical sludge-derived biochar and its application for the adsorption of tetracycline[J]. Science of the Total Environment,2020,747:141492.
    [7]
    RAVENNI G,CAFAGGI G,SAROSSY Z,et al. Waste chars from wood gasification and wastewater sludge pyrolysis compared to commercial activated carbon for the removal of cationic and anionic dyes from aqueous solution[J]. Bioresource Technology Reports,2020,10:100421.
    [8]
    LIU X Q,DING H S,WANG Y Y,et al. Pyrolytic temperature dependent and ash catalyzed formation of sludge char with ultra-high adsorption to 1-naphthol[J]. Environmental Science & Technology,2016,50(5):2602-2609.
    [9]
    CHEN X H,NING X A,LAI X J,et al. Chlorophenols in textile dyeing sludge:pollution characteristics and environmental risk control[J].Journal of Hazardous Materials,2021,416:125721.
    [10]
    SEREDYCH M,BANDOSZ T J. Sewage sludge as a single precursor for development of composite adsorbents[J]. Chemical Engineering Journal,2007,128(1):59-67.
    [11]
    LI L F,AI J,ZHANG W J,et al. Relationship between the physicochemical properties of sludge-based carbons and the adsorption capacity of dissolved organic matter in advanced wastewater treatment:effects of chemical conditioning[J]. Chemosphere,2020,243:125333.
    [12]
    LI M,TANG Y Y,REN N N,et al. Effect of mineral constituents on temperature-dependent structural characterization of carbon fractions in sewage sludge-derived biochar[J]. Journal of Cleaner Production,2018,172:3342-3350.
    [13]
    MOSKO J,POHORELY M,SKOBLIA S,et al. Structural and chemical changes of sludge derived pyrolysis char prepared under different process temperatures[J]. Journal of Analytical and Applied Pyrolysis,2021,156:105085.
    [14]
    王旭,张乐瑶,张昊轩,等. 中空孔结构对W掺杂MFI分子筛丙酮吸附行为的研究[J]. 化工学报,2022(3):1194-1206.
    [15]
    ZHAO Z M,SUN W J,RAY M B. Adsorption isotherms and kinetics for the removal of algal organic matter by granular activated carbon[J]. Science of the Total Environment,2022,806:150885.
    [16]
    杨招艺,陶家林,等. 热解温度对污泥碳基材料表面性质及吸附性能的影响[J]. 环境工程学报,2019,13(11):2711-2721.
    [17]
    曹臣,韦朝海,等. 废水处理生物出水中COD构成的解析:以焦化废水为例[J]. 环境化学,2012,31(10):1494-1501.
    [18]
    SHI Y J,HU H D,REN H Q. Dissolved organic matter (DOM) removal from biotreated coking wastewater by chitosan-modified biochar:adsorption fractions and mechanisms[J]. Bioresource Technology,2020,297:122281.
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