Source Jouranl of CSCD
Source Journal of Chinese Scientific and Technical Papers
Included as T2 Level in the High-Quality Science and Technology Journals in the Field of Environmental Science
Core Journal of RCCSE
Included in the CAS Content Collection
Included in the JST China
Indexed in World Journal Clout Index (WJCI) Report
Volume 41 Issue 9
Sep.  2023
Turn off MathJax
Article Contents
XU Zhilong, YU Naichuan, SUN Huijie, WANG Qunhui. MECHANISM AND TOXICITY ANALYSIS OF SULFAMETHAZINE DEGRADATION BY ELECTRO-FENTON SYSTEM USING NATURAL TOURMALINE AS THE CATALYST[J]. ENVIRONMENTAL ENGINEERING , 2023, 41(9): 89-95. doi: 10.13205/j.hjgc.202309011
Citation: XU Zhilong, YU Naichuan, SUN Huijie, WANG Qunhui. MECHANISM AND TOXICITY ANALYSIS OF SULFAMETHAZINE DEGRADATION BY ELECTRO-FENTON SYSTEM USING NATURAL TOURMALINE AS THE CATALYST[J]. ENVIRONMENTAL ENGINEERING , 2023, 41(9): 89-95. doi: 10.13205/j.hjgc.202309011

MECHANISM AND TOXICITY ANALYSIS OF SULFAMETHAZINE DEGRADATION BY ELECTRO-FENTON SYSTEM USING NATURAL TOURMALINE AS THE CATALYST

doi: 10.13205/j.hjgc.202309011
  • Received Date: 2023-05-24
    Available Online: 2023-11-15
  • Sulfadimethymidine (SMT) is a kind of antibiotic with a good antibacterial effect, which is widely used in the treatment of human and livestock diseases globally. But because it cannot be completely absorbed in the animal body, it will be excreted with feces, and then pollute the natural water body. In this study, natural tourmaline was used as a catalyst to form an electro-Fenton reaction system. Hydrogen peroxide (H2O2) was generated in situ by the cathode. In this paper, the effects of different pH, initial SMT concentration, temperature, current density, and tourmaline dosage on the degradation of SMT were investigated.
  • loading
  • [1]
    ZHANG M L, JIANG Z W, LI D Q, et al. Oral antibiotic treatment induces skin microbiota dysbiosis and influences wound healing[J]. Microbial Ecology, 2015, 69(2):415-421.
    [2]
    XIE Z X, TANG J, WU X W, et al. Bioconcentration and ecotoxicity of sulfadiazine in the aquatic midge Chironomus riparius[J]. Environmental Toxicology and Pharmacology, 2019, 66:69-74.
    [3]
    宋亚丽, 李帅斌, 李紫燕, 等. Ag/g-C3N4复合材料可见光降解磺胺甲基嘧啶的效能及机理研究[J]. 郑州轻工业学院学报(自然科学版), 2021, 036(6):102-109.
    [4]
    XU J, ZHANG Y, ZHOU C B, et al. Distribution, sources and composition of antibiotics in sediment, overlying water and pore water from Taihu Lake, China[J]. Science of the Total Environment, 2014, 498:267-273.
    [5]
    XIE H J, WANG X P, CHEN J W, et al. Occurrence, distribution and ecological risks of antibiotics and pesticides in coastal waters around Liaodong Peninsula, China[J]. Science of the Total Environment, 2019, 656:946-951.
    [6]
    黄春年, 李学德, 花日茂. 磺胺二甲嘧啶在水溶液中的光化学降解[J]. 环境污染与防治, 2011, 33(12):59-64.
    [7]
    NIU B H, WANG N F, CHEN Y M, et al. Tourmaline synergized with persulfate for degradation of sulfadiazine:influencing parameters and reaction mechanism[J]. Separation and Purification Technology, 2021, 257:117893.
    [8]
    张立东, 付文贤, 霍思月, 等. CuFeO2@PVP的制备及其基于光电芬顿降解氧氟沙星[J].环境工程学报, 2023, 17(2):416-430.
    [9]
    NAKAMURA T. Tourmaline group crystals reaction with water[J]. Ferroelectrics, 1992, 137(4):13-21.
    [10]
    孙振亚, 祝春水, 龚文琪. 铁(氢)氧化物矿物对有机污染物的光催化氧化作用[J]. 矿物学报, 2003(4):341-348.
    [11]
    殷丹阳, 余梦琳, 史静, 等. 电气石对恩诺沙星的吸附特性[J]. 环境工程学报, 2017, 11(4):2183-2189.
    [12]
    李艳. 天然铁电气石Fenton反应降解甲基橙的效能与机理研究[D]. 哈尔滨:哈尔滨理工大学, 2012.
    [13]
    舒诚, 于晓枫, 程建华, 等. 甲酸刻蚀缺陷MOFs电芬顿高效降解磺胺甲恶唑[J].环境工程学报, 2022, 16(9):2828-2837.
    [14]
    WANG C P, ZHANG Y W, Yu L, et al. Oxidative degradation of azo dyes using tourmaline[J]. Journal of Hazardous Materials, 2013, 260:851-859.
    [15]
    DIAO Z H, LIU J J, HU Y X, et al. Comparative study of Rhodamine B degradation by the systems pyrite/H2O2 and pyrite/persulfate:reactivity, stability, products and mechanism[J]. Separation & Purification Technology, 2017, 184:374-383.
    [16]
    XUE X F, HANNA K, ABDELMOULA M, et al. Adsorption and oxidation of PCP on the surface of magnetite:kinetic experiments and spectroscopic investigations[J]. Applied Catalysis B Environmental, 2009, 89(3/4):432-440.
    [17]
    张婧懿, 向琦, 雷炜东, 等. N掺杂多孔生物炭材料的制备及电Fenton法降解染料X3B[J]. 武汉大学学报(理学版), 2021, 67(4):359-366.
    [18]
    江淑文, 韦士程, 王婷, 等.类芬顿催化剂Cu-Co-Fe金属氧化物的制备及其对典型难降解有机物的去除[J].环境工程, 2021, 39(11):77-82

    ,118.
    [19]
    陈作云. 旅客列车集便器废水中抗生素的光芬顿催化降解分析[J]. 环境工程, 2020,38(10):128-133

    ,139.
  • 加载中

Catalog

    通讯作者: 陈斌, bchen63@163.com
    • 1. 

      沈阳化工大学材料科学与工程学院 沈阳 110142

    1. 本站搜索
    2. 百度学术搜索
    3. 万方数据库搜索
    4. CNKI搜索

    Article Metrics

    Article views (129) PDF downloads(3) Cited by()
    Proportional views
    Related

    /

    DownLoad:  Full-Size Img  PowerPoint
    Return
    Return