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Volume 44 Issue 3
Mar.  2026
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Article Contents
YOU Wei, LIU Dingxin, ZHANG Weiliang, MA Zhichen, ZHOU Lü, LUO Jingyang, LIU Jianchao. Pollution characteristics and priority substance screening of PFASs in typical drinking water systems of the lower Yangtze River[J]. ENVIRONMENTAL ENGINEERING , 2026, 44(3): 112-124. doi: 10.13205/j.hjgc.202603010
Citation: YOU Wei, LIU Dingxin, ZHANG Weiliang, MA Zhichen, ZHOU Lü, LUO Jingyang, LIU Jianchao. Pollution characteristics and priority substance screening of PFASs in typical drinking water systems of the lower Yangtze River[J]. ENVIRONMENTAL ENGINEERING , 2026, 44(3): 112-124. doi: 10.13205/j.hjgc.202603010

Pollution characteristics and priority substance screening of PFASs in typical drinking water systems of the lower Yangtze River

doi: 10.13205/j.hjgc.202603010
  • Received Date: 2025-12-30
    Available Online: 2026-04-11
  • Publish Date: 2026-03-01
  • Per- and polyfluoroalkyl substances (PFASs) are frequently detected at elevated concentrations in water bodies of the lower Yangtze River, posing risks to drinking water safety and human health. This study investigated the occurrence of 23 typical PFASs in source water, treated water, and tap water from eight drinking water treatment plants (DWTPs) in the lower reaches of the Yangtze River. The removal efficiency of PFASs by the treatment processes and their priority for control were also assessed. The results revealed the presence of 19 PFASs across the eight DWTPs, with total concentrations ranging from 32.02 to 167.68 ng/L and an average of 85.86 ng/L. Among these, 14 long-chain and 5 short-chain PFASs were identified, contributing 35.7% and 64.3% to the total concentration, respectively, indicating that short-chain PFASs were the predominant pollutants. The major contaminant monomers were perfluorooctanoic acid (PFOA), perfluorobutanoic acid (PFBA), perfluorobutanesulfonic acid (PFBS), and perfluorohexanoic acid (PFHxA). The overall removal efficiency of PFASs by the drinking water treatment processes was 17.8%, with a removal efficiency of 22.2% for long-chain and 15.1% for short-chain congeners. Notably, concentrations of 14 PFASs increased during distribution from the treatment plant to the tap, resulting in an overall rebound rate of 39.6%. PFBA, PFOA, and PFBS were the primary contributors, accounting for over 92.8% of this concentration increase. Modeling assessment identified PFOA, perfluorononanoic acid (PFNA), perfluorododecanoic acid (PFDoA), and perfluorooctanesulfonic acid (PFOS) as priority PFASs requiring enhanced monitoring and control measures.
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  • [1]
    QIN X,ZHUANG Y,SHI B. PFAS promotes disinfection byproduct formation through triggering particle-bound organic matter release in drinking water pipes[J]. Water Research,2024,254:121339.
    [2]
    SADIA M,NOLLEN I,HELMUS R,et al. Occurrence,fate,and related health risks of PFAS in raw and produced drinking water[J]. Environmental Science& Technology,2023,57(8):3062-3074.
    [3]
    PAULETTO P S,BANDOSZ T J. Activated carbon versus metal-organic frameworks:a review of their PFAS adsorption performance[J]. Journal of Hazardous Materials,2022,425:127810.
    [4]
    PENNOYER E H,FILLMAN T,HEIGER-BERNAYS W,et al. Exposure to legacy per-and polyfluoroalkyl substances from diet and drinking water in California Adults,2018-2020[J]. Environmental Science& Technology,2025,59(20):9896-9906.
    [5]
    ZHONG T T,LIN T,LIU W. Distribution,tansformation,and fate of per-and polyfluoroalkyl substances in drinking water treatment[J]. Environmental Science,2023,44(5):2613-2621. 钟婷婷,林涛,刘威. 饮用水处理过程中全氟化合物的分布、转化及去向[J]. 环境科学,2023,44(5):2613-2621.
    [6]
    CHANG W,XU S D,LIU T,et al. Risk prioritization and experimental validation of per-and polyfluoroalkyl substances(PFAS)in Chaohu Lake:Based on nontarget and target analyses[J]. Journal of Hazardous Materials,2025,492:138179.
    [7]
    ZHENG P,LIU M,YIN H,et al. Analysis of 58 poly-/perfluoroalkyl substances and their occurrence in surface water in a high-technology industrial park[J]. Environmental Pollution,2020,267:115381.
    [8]
    ARINAITWE K,KELTSCH N,TAABU-MUNYAHO A,et al. Perfluoroalkyl substances(PFASs)in the Ugandan waters of Lake Victoria:Spatial distribution,catchment release and public exposure risk via municipal water consumption[J]. Science of the Total Environment,2021,783:146970.
    [9]
    FANG X Y,WU Y P,LI T R,et al. Advanced purification of per-and polyfluoroalkyl substances in drinking water:status and challenges[J]. Environmental Science,2025,46(6):3440-3449. 方晓雅,吴颖鹏,李汤睿,等. 饮用水中全氟及多氟烷基化合物的深度净化:现状与挑战[J]. 环境科学,2025,46(6):3440-3449.
    [10]
    WEE S Y,ARIS A Z. Revisiting the“forever chemicals”,PFOA and PFOS exposure in drinking water[J]. NPJ Clean Water,2023,6(1):57.
    [11]
    HU X C,ANDREWS D Q,LINDSTROM A B,et al. Detection of poly-and perfluoroalkyl substances(PFASs)in U.S. drinking water linked to industrial sites,military fire training areas,and wastewater treatment plants[J]. Environmental Science& Technology Letters,2016,3(10):344-350.
    [12]
    LENKA S P,KAH M,PADHYE L P. Occurrence and fate of poly-and perfluoroalkyl substances(PFAS)in urban waters of New Zealand[J]. Journal of Hazardous Materials,2022,428:128257.
    [13]
    LI S,GOODRICH J A,COSTELLO E,et al. Examining disparities in PFAS plasma concentrations:Impact of drinking water contamination,food access,proximity to industrial facilities and superfund sites[J]. Environmental Research,2025,264:120370.
    [14]
    LI Y,WAN F F,ZHANG W L. Development trend and strategy of efficient utilization of water resources for industrial parks in Yangtze River Delta Region[J]. Journal of Hohai University(Natural Sciences),2023,51(3):1-9. 李轶,万芬芬,张文龙. 长三角地区工业园区水资源高效利用的发展趋势与策略[J]. 河海大学学报(自然科学版),2023,51(3):1-9.
    [15]
    SHAO G,JIANG N,LIU T,et al. Target and non-target screening of per-and polyfluoroalkyl substances(PFAS)in drinking water:Focus on alternatives and health risks[J]. Environmental Research,2025,285:122581.
    [16]
    LIU J,OUYANG T,LU G,et al. Ecosystem risk-based prioritization of micropollutants in wastewater treatment plant effluents across China[J]. Water Research,2024,263:122168.
    [17]
    ZHONG M,WANG T,ZHAO W,et al. Emerging organic contaminants in Chinese surface water:identification of priority pollutants[J]. Engineering,2022,11:111-125.
    [18]
    LIN Z T,YOU W,LIU J C,et al. A proposed multi-media exposure and risk assessment method for screening for organic micropollutants in shallow lakes:a case study of Lake Taihu[J]. Journal of Lake Sciences,2025,37(6):2050-2065. 林梓涛,尤为,刘建超,等. 基于多介质暴露与危害风险评估的浅水湖泊中优控有机微污染物筛查:以太湖为例[J]. 湖泊科学,2025,37(6):2050-2065.
    [19]
    ZHAO J,HOU S,ZHANG H,et al. Spatiotemporal variations and priority ranking of emerging contaminants in nanwan reservoir:A case study from the agricultural region in huaihe river basin in China[J]. Journal of Environmental Management,2024,368:122195.
    [20]
    GONG X,XIONG L,XING J,et al. Implications on freshwater lake-river ecosystem protection suggested by organic micropollutant(OMP)priority list[J]. Journal of Hazardous Materials,2024,461:132580.
    [21]
    HUANG F,CHEN L,ZHANG C,et al. Prioritization of antibiotic contaminants in China based on decennial national screening data and their persistence,bioaccumulation and toxicity[J]. Science of the Total Environment,2022,806:150636.
    [22]
    DVORAKOVA D,JURIKOVA M,SVOBODOVA V,et al. Complex monitoring of perfluoroalkyl substances(PFAS)from tap drinking water in the Czech Republic[J]. Water Research,2023,247:120764.
    [23]
    ADEOGUN A O,CHUKWUKA A V,IBOR O R,et al. Occurrence,bioaccumulation and trophic dynamics of per-and polyfluoroalkyl substances in two tropical freshwater lakes[J]. Environmental Pollution,2024,346:123575.
    [24]
    TAO Y,PANG Y,LUO M,et al. Multi-media distribution and risk assessment of per-and polyfluoroalkyl substances in the Huai River Basin,China[J]. Science of the Total Environment,2024,914:169581.
    [25]
    SöRENGåRD M,BERGSTRöM S,MCCLEAF P,et al. Long-distance transport of per-and polyfluoroalkyl substances(PFAS)in a Swedish drinking water aquifer[J]. Environmental Pollution,2022,311:119981.
    [26]
    LLEWELLYN M J,GRIFFIN E K,CASPAR R J,et al. Identification and quantification of novel per-and polyfluoroalkyl substances(PFAS)contamination in a Great Lakes urban-dominated watershed[J]. Science of the Total Environment,2024,941:173325.
    [27]
    GRUNG M,HJERMANN D Ø,RUNDBERGET T,et al. Low levels of per-and polyfluoroalkyl substances(PFAS)detected in drinking water in Norway,but elevated concentrations found near known sources[J]. Science of the Total Environment,2024,947:174550.
    [28]
    MUNOZ G,LIU M,VO DUY S,et al. Target and nontarget screening of PFAS in drinking water for a large-scale survey of urban and rural communities in Québec,Canada[J]. Water Research,2023,233:119750.
    [29]
    CSERBIK D,REDONDO-HASSELERHARM P E,FARRé M J,et al. Human exposure to per-and polyfluoroalkyl substances and other emerging contaminants in drinking water[J]. npj Clean Water,2023,6(1):16.
    [30]
    VON BEHREN J,REYNOLDS P,BRADLEY P M,et al. Per-and polyfluoroalkyl substances(PFAS)in drinking water in Southeast Los Angeles:Industrial legacy and environmental justice[J]. Science of the Total Environment,2024,953:176067.
    [31]
    FU Y,JI Y,TIAN Y,et al. Unveiling priority emerging PFAS in Taihu Lake using integrated nontarget screening,target analysis,and risk characterization[J]. Environmental Science& Technology,2024,58(42):18980-18991.
    [32]
    KANG J-K,KIM M-G,J-E OH. Occurrence and removal of 42 legacy and emerging per-and polyfluoroalkyl substances(PFAS)in drinking water treatment plants in South Korea[J]. Water Research X,2025,29:100329.
    [33]
    ZHU H,XIA Y,ZHANG Y,et al. Distribution characteristics and transformation mechanism of per-and polyfluoroalkyl substances in drinking water sources:a review[J]. Science of the Total Environment,2024,916:169566.
    [34]
    CHENG H,JIN H,LU B,et al. Emerging poly-and perfluoroalkyl substances in water and sediment from Qiantang River-Hangzhou Bay[J]. Science of the Total Environment,2023,875:162687.
    [35]
    SONG D,QIAO B,YAO Y,et al. Target and nontarget analysis of per-and polyfluoroalkyl substances in surface water,groundwater and sediments of three typical fluorochemical industrial parks in China[J]. Journal of Hazardous Materials,2023,460:132411.
    [36]
    CAPPELLI F,BAMAI Y AIT,VAN HOEY K,et al. Occurrence of short-and ultra-short chain PFAS in drinking water from Flanders(Belgium)and implications for human exposure[J]. Environmental Research,2024,260:119753.
    [37]
    MCCLEAF P,STEFANSSON W,AHRENS L. Drinking water nanofiltration with concentrate foam fractionation—a novel approach for removal of per-and polyfluoroalkyl substances(PFAS)[J]. Water Research,2023,232:119688.
    [38]
    HONG Y,DING Q,YANG T,et al. Per-and polyfluoroalkyl substances(PFAS)in drinking water systems in the lower Yangtze River:source,fate,and health risk assessment[J]. Environmental Geochemistry and Health,2025,47(6):197.
    [39]
    JIAO E,ZHU Z,YIN D,et al. A pilot study on extractable organofluorine and per-and polyfluoroalkyl substances(PFAS)in water from drinking water treatment plants around Taihu Lake,China:what is missed by target PFAS analysis?[J]. Environmental Science:Processes& Impacts,2022,24(7):1060-1070.
    [40]
    PREST E I,SCHAAP P G,BESMER M D,et al. Dynamic hydraulics in a drinking water distribution system influence suspended particles and turbidity,but not microbiology[J]. Water Research,2021,13(1):109.
    [41]
    SZABO J,WITT S,SOJDA N,et al. Flushing home plumbing pipes contaminated with aqueous film-forming foam containing per-and polyfluoroalkyl substances[J]. Journal of Environmental Engineering,2023,149(9):05023007.
    [42]
    CHEN R,LI G,YU Y,et al. Occurrence and transport behaviors of perfluoroalkyl acids in drinking water distribution systems[J]. Science of the Total Environment,2019,697:134162.
    [43]
    MOHAMMADI A,DOBARADARAN S,SCHMIDT T C,et al. Emerging contaminants migration from pipes used in drinking water distribution systems:a review of the scientific literature[J]. Environmental Science and Pollution Research,2022,29(50):75134-75160.
    [44]
    YU C H,WEISEL C P,ALIMOKHTARI S,et al. Biomonitoring:a tool to assess PFNA body burdens and evaluate the effectiveness of drinking water intervention for communities in New Jersey[J]. International Journal of Hygiene and Environmental Health,2021,235:113757.
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